Crystal structure of tris(2-methyl-1H-imidazol-3-ium) benzene-1,3,5-tricarboxylate

The structure of the title salt, 3C4H7N2+·C9H3O63− (1), is reported. The compound is formed with three 2-methylimidazolium cations and a fully deprotonated trimesic acid. The structure is disordered over two orientations, which were refined using a split model (90.99: 9.01occupancy ratio). Analysis...

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Bibliographic Details
Main Authors: Weronika Łukaszczyk, Allegra Lohse, Julia Leibing, Sudem Yildizbas, Irwana Rizvanovic, Simone Techert, Jose de Jesus Velazquez-Garcia
Format: Article
Language:English
Published: International Union of Crystallography 2025-07-01
Series:Acta Crystallographica Section E: Crystallographic Communications
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Online Access:https://journals.iucr.org/paper?S2056989025004748
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Summary:The structure of the title salt, 3C4H7N2+·C9H3O63− (1), is reported. The compound is formed with three 2-methylimidazolium cations and a fully deprotonated trimesic acid. The structure is disordered over two orientations, which were refined using a split model (90.99: 9.01occupancy ratio). Analysis of bond distances and angles reveals the differences and similarities between compound 1 and the previously published 2-methyl-1H-imidazol-3-ium 3,5-dicarboxybenzoate structure [Baletska et al., (2023). Acta Cryst. E79, 1088–1092] and tris(2-methyl-1H- imidazol-3-ium) 5-carboxybenzene-1,3-dicarboxylate 3,5-dicarboxybenzoate [Asprilla-Herrera et al. (2025). Acta Cryst. E81, 303–309], as well as the neutral counterparts of the ions [Tothadi et al. (2020). ACS Appl. Mater. Interfaces, 12, 15588–15594; Hachuła et al. (2010). J. Chem. Crystallogr. 40, 201–206]. The crystal packing analysis reveals the formation of hydrogen-bonded two-dimensional networks perpendicular to the [111] vector, where neighbouring planes interact via extensive π–π stacking.
ISSN:2056-9890