Preparation and Property Study of Enzymatically Modified Octenyl Succinate Starch

Octenylsuccinic anhydride starch (OSAS) has high viscosity and low solubility in water, which often leads to low efficiency in the esterification reaction between starch and octenylsuccinic anhydride under alkaline conditions, and uneven distribution of octenylsuccinic anhydride (OSA) groups. Enzyma...

Full description

Saved in:
Bibliographic Details
Main Authors: HU Zhong-shan, ZHOU Jin-jie, CHEN Lei, HUANG Wei, FENG Tao
Format: Article
Language:English
Published: Academy of National Food and Strategic Reserves Administration 2025-03-01
Series:Liang you shipin ke-ji
Subjects:
Online Access:http://lyspkj.ijournal.cn/lyspkj/article/abstract/20250210?st=article_issue
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850050147093839872
author HU Zhong-shan
ZHOU Jin-jie
CHEN Lei
HUANG Wei
FENG Tao
author_facet HU Zhong-shan
ZHOU Jin-jie
CHEN Lei
HUANG Wei
FENG Tao
author_sort HU Zhong-shan
collection DOAJ
description Octenylsuccinic anhydride starch (OSAS) has high viscosity and low solubility in water, which often leads to low efficiency in the esterification reaction between starch and octenylsuccinic anhydride under alkaline conditions, and uneven distribution of octenylsuccinic anhydride (OSA) groups. Enzymatic hydrolysis of OSAS can solve this problem. Using waxy corn starch to prepare OSAS, the molecular weight of enzyme-modified octenylsuccinic anhydride starch (E-OSAS) decreased with the addition of pullulanase. The degree of substitution of E-OSAS was greater than that of OSAS, and as the amount of pullulanase increased, the degree of substitution of E-OSAS showed an upward trend, while the apparent viscosity decreased significantly. The smaller particle size and polydispersity index (PDI), the larger the absolute value of the zeta potential. E40-OSAS, with the smallest particle size, the best homogeneity and stability, had the smallest weight average molecular weight (1.38×106 g/mol), the smallest number average molecular weight (1.37×105 g/mol), and the largest degree of substitution of 0.019. This study provides some basis for the research of new microcapsules.
format Article
id doaj-art-a7308d1d734a4177867217631b7adfa1
institution DOAJ
issn 1007-7561
language English
publishDate 2025-03-01
publisher Academy of National Food and Strategic Reserves Administration
record_format Article
series Liang you shipin ke-ji
spelling doaj-art-a7308d1d734a4177867217631b7adfa12025-08-20T02:53:33ZengAcademy of National Food and Strategic Reserves AdministrationLiang you shipin ke-ji1007-75612025-03-01332596610.16210/j.cnki.1007-7561.2025.02.009Preparation and Property Study of Enzymatically Modified Octenyl Succinate StarchHU Zhong-shan0ZHOU Jin-jie1CHEN Lei2HUANG Wei3FENG Tao4Shanghai Peony Flavors and Fragrances Co., Ltd., Shanghai 201210, ChinaShanghai Peony Flavors and Fragrances Co., Ltd., Shanghai 201210, ChinaShanghai Peony Flavors and Fragrances Co., Ltd., Shanghai 201210, ChinaShanghai Peony Flavors and Fragrances Co., Ltd., Shanghai 201210, ChinaDepartment of Fragrant Chemistry, Shanghai Institute of Technology, Shanghai 201418, ChinaOctenylsuccinic anhydride starch (OSAS) has high viscosity and low solubility in water, which often leads to low efficiency in the esterification reaction between starch and octenylsuccinic anhydride under alkaline conditions, and uneven distribution of octenylsuccinic anhydride (OSA) groups. Enzymatic hydrolysis of OSAS can solve this problem. Using waxy corn starch to prepare OSAS, the molecular weight of enzyme-modified octenylsuccinic anhydride starch (E-OSAS) decreased with the addition of pullulanase. The degree of substitution of E-OSAS was greater than that of OSAS, and as the amount of pullulanase increased, the degree of substitution of E-OSAS showed an upward trend, while the apparent viscosity decreased significantly. The smaller particle size and polydispersity index (PDI), the larger the absolute value of the zeta potential. E40-OSAS, with the smallest particle size, the best homogeneity and stability, had the smallest weight average molecular weight (1.38×106 g/mol), the smallest number average molecular weight (1.37×105 g/mol), and the largest degree of substitution of 0.019. This study provides some basis for the research of new microcapsules.http://lyspkj.ijournal.cn/lyspkj/article/abstract/20250210?st=article_issuewaxy corn starchpullulanaseenzymolysisoctenyl succinate starchstructure characterization
spellingShingle HU Zhong-shan
ZHOU Jin-jie
CHEN Lei
HUANG Wei
FENG Tao
Preparation and Property Study of Enzymatically Modified Octenyl Succinate Starch
Liang you shipin ke-ji
waxy corn starch
pullulanase
enzymolysis
octenyl succinate starch
structure characterization
title Preparation and Property Study of Enzymatically Modified Octenyl Succinate Starch
title_full Preparation and Property Study of Enzymatically Modified Octenyl Succinate Starch
title_fullStr Preparation and Property Study of Enzymatically Modified Octenyl Succinate Starch
title_full_unstemmed Preparation and Property Study of Enzymatically Modified Octenyl Succinate Starch
title_short Preparation and Property Study of Enzymatically Modified Octenyl Succinate Starch
title_sort preparation and property study of enzymatically modified octenyl succinate starch
topic waxy corn starch
pullulanase
enzymolysis
octenyl succinate starch
structure characterization
url http://lyspkj.ijournal.cn/lyspkj/article/abstract/20250210?st=article_issue
work_keys_str_mv AT huzhongshan preparationandpropertystudyofenzymaticallymodifiedoctenylsuccinatestarch
AT zhoujinjie preparationandpropertystudyofenzymaticallymodifiedoctenylsuccinatestarch
AT chenlei preparationandpropertystudyofenzymaticallymodifiedoctenylsuccinatestarch
AT huangwei preparationandpropertystudyofenzymaticallymodifiedoctenylsuccinatestarch
AT fengtao preparationandpropertystudyofenzymaticallymodifiedoctenylsuccinatestarch