Preparation of imidazole ligand zirconium-based UiO-66 and its application in the direct synthesis of dimethyl carbonate from CO2 and methanol

Preparation of imidazole ligand zirconium-based UiO-66 and its application in the direct synthesis of dimethyl carbonate from CO2 and methanol

In this study, imidazole carboxylate was introduced into the structure of UiO-66 as a secondary ligand. Subsequently, a novel imidazole ligand zirconium-based UiO-66-Im-X material was prepared, which was used to catalyze the direct synthesis of dimethyl carbonate (DMC) from carbon dioxide (CO2) and...

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Bibliographic Details
Main Authors: Zhongqi Zhang, Yingjie Shen, Aosen Zhang, Yuan Zhai, Ziqing Wang, Kun Jiang, Heyun Wang
Format: Article
Language:English
Published: Elsevier 2025-08-01
Series:Journal of CO2 Utilization
Subjects:
UiO-66
Carbon dioxide
Dimethyl carbonate
Defect engineering
Acidic site
Online Access:http://www.sciencedirect.com/science/article/pii/S2212982025001325
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