Achieving low-temperature Cu–Cu bonding platform via area-selective metal films with superior surface roughness for advanced packaging

This study addresses the critical challenge of achieving low-temperature Cu–Cu bonding for advanced packaging applications by optimizing area-selective electroless Au passivation. We demonstrate that an Ar/N2 plasma pretreatment, applied prior to Au deposition, substantially strips oxides, renders t...

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Main Authors: Mu-Ping Hsu, Chi-Yu Chen, Hsin-Chi Chang, Kuan-Neng Chen
Format: Article
Language:English
Published: Elsevier 2025-05-01
Series:Journal of Materials Research and Technology
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2238785425011950
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author Mu-Ping Hsu
Chi-Yu Chen
Hsin-Chi Chang
Kuan-Neng Chen
author_facet Mu-Ping Hsu
Chi-Yu Chen
Hsin-Chi Chang
Kuan-Neng Chen
author_sort Mu-Ping Hsu
collection DOAJ
description This study addresses the critical challenge of achieving low-temperature Cu–Cu bonding for advanced packaging applications by optimizing area-selective electroless Au passivation. We demonstrate that an Ar/N2 plasma pretreatment, applied prior to Au deposition, substantially strips oxides, renders the Cu surface amorphous and highly hydrophilic, and thus suppresses grain-boundary-selective Au displacement to form a smooth, continuous passivation layer. The resulting amorphous Cu surface layer facilitates the formation of continuous Au films without “lightning-like” patterns, enabling reliable chip-to-chip bonding at temperatures as low as 150 °C under ambient conditions. Compared to O2 or N2-only plasma treatments, the Ar/N2 approach yields stronger bonds, improved void filling by Cu diffusion, and higher electrical yields and stability. These findings underscore the importance of pretreatment engineering in electroless plating processes, paving the way for more robust, scalable, and cost-effective Cu–Cu bonding solutions in next-generation advanced packaging.
format Article
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institution Kabale University
issn 2238-7854
language English
publishDate 2025-05-01
publisher Elsevier
record_format Article
series Journal of Materials Research and Technology
spelling doaj-art-79ee7a66336d46779b775ace52eef8362025-08-20T03:52:55ZengElsevierJournal of Materials Research and Technology2238-78542025-05-01367748775410.1016/j.jmrt.2025.05.041Achieving low-temperature Cu–Cu bonding platform via area-selective metal films with superior surface roughness for advanced packagingMu-Ping Hsu0Chi-Yu Chen1Hsin-Chi Chang2Kuan-Neng Chen3Institute of Electronics, National Yang Ming Chiao Tung University, Hsinchu, TaiwanInstitute of Pioneer Semiconductor Innovation, National Yang Ming Chiao Tung University, Hsinchu, TaiwanInstitute of Electronics, National Yang Ming Chiao Tung University, Hsinchu, TaiwanInstitute of Electronics, National Yang Ming Chiao Tung University, Hsinchu, Taiwan; Institute of Pioneer Semiconductor Innovation, National Yang Ming Chiao Tung University, Hsinchu, Taiwan; Corresponding author. Institute of Electronics, National Yang Ming Chiao Tung University, Hsinchu, Taiwan.This study addresses the critical challenge of achieving low-temperature Cu–Cu bonding for advanced packaging applications by optimizing area-selective electroless Au passivation. We demonstrate that an Ar/N2 plasma pretreatment, applied prior to Au deposition, substantially strips oxides, renders the Cu surface amorphous and highly hydrophilic, and thus suppresses grain-boundary-selective Au displacement to form a smooth, continuous passivation layer. The resulting amorphous Cu surface layer facilitates the formation of continuous Au films without “lightning-like” patterns, enabling reliable chip-to-chip bonding at temperatures as low as 150 °C under ambient conditions. Compared to O2 or N2-only plasma treatments, the Ar/N2 approach yields stronger bonds, improved void filling by Cu diffusion, and higher electrical yields and stability. These findings underscore the importance of pretreatment engineering in electroless plating processes, paving the way for more robust, scalable, and cost-effective Cu–Cu bonding solutions in next-generation advanced packaging.http://www.sciencedirect.com/science/article/pii/S22387854250119503DICAdvanced packagingArea selective depositionLow temperature Cu–C bondingElectroless plating
spellingShingle Mu-Ping Hsu
Chi-Yu Chen
Hsin-Chi Chang
Kuan-Neng Chen
Achieving low-temperature Cu–Cu bonding platform via area-selective metal films with superior surface roughness for advanced packaging
Journal of Materials Research and Technology
3DIC
Advanced packaging
Area selective deposition
Low temperature Cu–C bonding
Electroless plating
title Achieving low-temperature Cu–Cu bonding platform via area-selective metal films with superior surface roughness for advanced packaging
title_full Achieving low-temperature Cu–Cu bonding platform via area-selective metal films with superior surface roughness for advanced packaging
title_fullStr Achieving low-temperature Cu–Cu bonding platform via area-selective metal films with superior surface roughness for advanced packaging
title_full_unstemmed Achieving low-temperature Cu–Cu bonding platform via area-selective metal films with superior surface roughness for advanced packaging
title_short Achieving low-temperature Cu–Cu bonding platform via area-selective metal films with superior surface roughness for advanced packaging
title_sort achieving low temperature cu cu bonding platform via area selective metal films with superior surface roughness for advanced packaging
topic 3DIC
Advanced packaging
Area selective deposition
Low temperature Cu–C bonding
Electroless plating
url http://www.sciencedirect.com/science/article/pii/S2238785425011950
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AT chiyuchen achievinglowtemperaturecucubondingplatformviaareaselectivemetalfilmswithsuperiorsurfaceroughnessforadvancedpackaging
AT hsinchichang achievinglowtemperaturecucubondingplatformviaareaselectivemetalfilmswithsuperiorsurfaceroughnessforadvancedpackaging
AT kuannengchen achievinglowtemperaturecucubondingplatformviaareaselectivemetalfilmswithsuperiorsurfaceroughnessforadvancedpackaging