Orbital-free density functionals based on real and reciprocal space separation

Abstract We introduce a general class of orbital-free density functionals (OF-DFT) decomposed into a local part in coordinate space and a local part in reciprocal space. As a demonstration of principle, we choose for the former the Thomas-Fermi-von Weizsäcker (TFW) kinetic energy density functional...

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Bibliographic Details
Main Authors: Bishal Thapa, Tracey G. Oellerich, Maria Emelianenko, Phanish Suryanarayana, Igor I. Mazin
Format: Article
Language:English
Published: Nature Portfolio 2025-05-01
Series:npj Computational Materials
Online Access:https://doi.org/10.1038/s41524-025-01643-0
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