High-performance self-driven broadband photoelectrochemical photodetector based on reduced graphene oxide/Bi2Te3 heterojunction

Attributed to its excellent physicochemical properties, graphene (GR) has very active applications in the fields of catalysis, optoelectronic devices, and battery electrode materials. However, until now, regulating the type and density of carriers in GR is still crucial for its practical application...

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Main Authors: Chenchen Zhao, Yangyang Liu, Dongbo Wang, Wen He, Bingke Zhang, Jingwen Pan, Zhi Zeng, Donghao Liu, Sihang Liu, Shujie Jiao, Xuan Fang, Dan Fang, Liancheng Zhao, Jinzhong Wang
Format: Article
Language:English
Published: KeAi Communications Co., Ltd. 2024-12-01
Series:Nano Materials Science
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Online Access:http://www.sciencedirect.com/science/article/pii/S2589965123000946
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author Chenchen Zhao
Yangyang Liu
Dongbo Wang
Wen He
Bingke Zhang
Jingwen Pan
Zhi Zeng
Donghao Liu
Sihang Liu
Shujie Jiao
Xuan Fang
Dan Fang
Liancheng Zhao
Jinzhong Wang
author_facet Chenchen Zhao
Yangyang Liu
Dongbo Wang
Wen He
Bingke Zhang
Jingwen Pan
Zhi Zeng
Donghao Liu
Sihang Liu
Shujie Jiao
Xuan Fang
Dan Fang
Liancheng Zhao
Jinzhong Wang
author_sort Chenchen Zhao
collection DOAJ
description Attributed to its excellent physicochemical properties, graphene (GR) has very active applications in the fields of catalysis, optoelectronic devices, and battery electrode materials. However, until now, regulating the type and density of carriers in GR is still crucial for its practical applications. Here, reduced graphene oxide (RGO)-Bi2Te3 heterojunctions doped with different contents were prepared by a simple one-step method. The Bi2Te3 materials containing different RGO were made into broadband (365–850 ​nm) photoelectrochemical-type detectors, and the effects of the doping amount of RGO on the optoelectronic behavior of the devices and the intrinsic operation mechanism of the devices were investigated in detail. The results show that the values of Iph/Idark, Ri, and D∗ of Bi2Te3/RGO heterojunction devices obtained with 1 ​mg of RGO doping are 412, 6.072 ​mA/W, and 2.406 ​× ​1010 Jones, respectively. It is anticipated that this work will provide a research basis for future quantitative tuning of the performance of micro-nano devices by GR.
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spelling doaj-art-0279b1ff986847b9927f51802203895d2025-01-04T04:56:52ZengKeAi Communications Co., Ltd.Nano Materials Science2589-96512024-12-0166741751High-performance self-driven broadband photoelectrochemical photodetector based on reduced graphene oxide/Bi2Te3 heterojunctionChenchen Zhao0Yangyang Liu1Dongbo Wang2Wen He3Bingke Zhang4Jingwen Pan5Zhi Zeng6Donghao Liu7Sihang Liu8Shujie Jiao9Xuan Fang10Dan Fang11Liancheng Zhao12Jinzhong Wang13School of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, China; Corresponding author.School of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, China; Corresponding author.School of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, ChinaChangchun University Science and Technology, Sch Sci, State Key Lab High Power Semicond Lasers, Changchun, 130022, China; Corresponding author.Changchun University Science and Technology, Sch Sci, State Key Lab High Power Semicond Lasers, Changchun, 130022, ChinaSchool of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, China; Corresponding author.School of Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, China; Corresponding author.Attributed to its excellent physicochemical properties, graphene (GR) has very active applications in the fields of catalysis, optoelectronic devices, and battery electrode materials. However, until now, regulating the type and density of carriers in GR is still crucial for its practical applications. Here, reduced graphene oxide (RGO)-Bi2Te3 heterojunctions doped with different contents were prepared by a simple one-step method. The Bi2Te3 materials containing different RGO were made into broadband (365–850 ​nm) photoelectrochemical-type detectors, and the effects of the doping amount of RGO on the optoelectronic behavior of the devices and the intrinsic operation mechanism of the devices were investigated in detail. The results show that the values of Iph/Idark, Ri, and D∗ of Bi2Te3/RGO heterojunction devices obtained with 1 ​mg of RGO doping are 412, 6.072 ​mA/W, and 2.406 ​× ​1010 Jones, respectively. It is anticipated that this work will provide a research basis for future quantitative tuning of the performance of micro-nano devices by GR.http://www.sciencedirect.com/science/article/pii/S2589965123000946PhotoelectrochemicalBi2Te3/RGO heterojunctionsDoping regulationSelf-drivenBroadband
spellingShingle Chenchen Zhao
Yangyang Liu
Dongbo Wang
Wen He
Bingke Zhang
Jingwen Pan
Zhi Zeng
Donghao Liu
Sihang Liu
Shujie Jiao
Xuan Fang
Dan Fang
Liancheng Zhao
Jinzhong Wang
High-performance self-driven broadband photoelectrochemical photodetector based on reduced graphene oxide/Bi2Te3 heterojunction
Nano Materials Science
Photoelectrochemical
Bi2Te3/RGO heterojunctions
Doping regulation
Self-driven
Broadband
title High-performance self-driven broadband photoelectrochemical photodetector based on reduced graphene oxide/Bi2Te3 heterojunction
title_full High-performance self-driven broadband photoelectrochemical photodetector based on reduced graphene oxide/Bi2Te3 heterojunction
title_fullStr High-performance self-driven broadband photoelectrochemical photodetector based on reduced graphene oxide/Bi2Te3 heterojunction
title_full_unstemmed High-performance self-driven broadband photoelectrochemical photodetector based on reduced graphene oxide/Bi2Te3 heterojunction
title_short High-performance self-driven broadband photoelectrochemical photodetector based on reduced graphene oxide/Bi2Te3 heterojunction
title_sort high performance self driven broadband photoelectrochemical photodetector based on reduced graphene oxide bi2te3 heterojunction
topic Photoelectrochemical
Bi2Te3/RGO heterojunctions
Doping regulation
Self-driven
Broadband
url http://www.sciencedirect.com/science/article/pii/S2589965123000946
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