Rapid organic contaminants removal by Mg-/Fe-based magnetic nanosheets synthesized using the molten salt method

Abstract Mg-/Fe-based magnetic nanosheets (MMNs) were synthesized in 1 min using a simple molten salt method, which then could be employed for the effective removal of organic dyes from aqueous solutions. The MMNs displayed positive surface charges in all pH ranges, facilitating excellent adsorption...

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Main Authors: Sung-Hwa Kim, Chaeyoung Kim, Sang Moon Lee, Ha-Jin Lee
Format: Article
Language:English
Published: SpringerOpen 2025-05-01
Series:Journal of Analytical Science and Technology
Subjects:
Online Access:https://doi.org/10.1186/s40543-025-00492-2
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author Sung-Hwa Kim
Chaeyoung Kim
Sang Moon Lee
Ha-Jin Lee
author_facet Sung-Hwa Kim
Chaeyoung Kim
Sang Moon Lee
Ha-Jin Lee
author_sort Sung-Hwa Kim
collection DOAJ
description Abstract Mg-/Fe-based magnetic nanosheets (MMNs) were synthesized in 1 min using a simple molten salt method, which then could be employed for the effective removal of organic dyes from aqueous solutions. The MMNs displayed positive surface charges in all pH ranges, facilitating excellent adsorption efficiency for anionic dyes such as methyl blue (MB) and Congo red (CR) via electrostatic interactions. Remarkably, the nanosheets exhibited extremely high adsorption capacities, with maximum values reaching 2041 mg g−1 for MB and 1000 mg g−1 for CR at 308 K. The MMNs demonstrated outstanding organic dye adsorption efficiency and recyclability, both in powder form and when applied to a sponge using a simple dipping method. Additionally, the integration of Au nanoparticles into the MMN structure enabled the catalytic reduction of 4-nitrophenol to 4-aminophenol, achieving complete conversion within 10 min. Following the removal of organic contaminants, the MMNs could be retrieved effortlessly using an external magnet. The economical synthesis process and the versatile application of MMNs for organic contaminant remediation suggest significant potential for advancing wastewater treatment technologies.
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spelling doaj-art-fddb629f5d534cfda0c508ca5f9900a92025-08-20T01:53:19ZengSpringerOpenJournal of Analytical Science and Technology2093-33712025-05-0116111310.1186/s40543-025-00492-2Rapid organic contaminants removal by Mg-/Fe-based magnetic nanosheets synthesized using the molten salt methodSung-Hwa Kim0Chaeyoung Kim1Sang Moon Lee2Ha-Jin Lee3Department of Chemistry, Seoul Women’s UniversityDepartment of Chemistry, Seoul Women’s UniversityResearch Center for Materials Analysis, Korea Basic Science InstituteDepartment of Chemistry, Seoul Women’s UniversityAbstract Mg-/Fe-based magnetic nanosheets (MMNs) were synthesized in 1 min using a simple molten salt method, which then could be employed for the effective removal of organic dyes from aqueous solutions. The MMNs displayed positive surface charges in all pH ranges, facilitating excellent adsorption efficiency for anionic dyes such as methyl blue (MB) and Congo red (CR) via electrostatic interactions. Remarkably, the nanosheets exhibited extremely high adsorption capacities, with maximum values reaching 2041 mg g−1 for MB and 1000 mg g−1 for CR at 308 K. The MMNs demonstrated outstanding organic dye adsorption efficiency and recyclability, both in powder form and when applied to a sponge using a simple dipping method. Additionally, the integration of Au nanoparticles into the MMN structure enabled the catalytic reduction of 4-nitrophenol to 4-aminophenol, achieving complete conversion within 10 min. Following the removal of organic contaminants, the MMNs could be retrieved effortlessly using an external magnet. The economical synthesis process and the versatile application of MMNs for organic contaminant remediation suggest significant potential for advancing wastewater treatment technologies.https://doi.org/10.1186/s40543-025-00492-2Magnetic nanosheetsMolten salt methodDye adsorptionCatalystWastewater treatment
spellingShingle Sung-Hwa Kim
Chaeyoung Kim
Sang Moon Lee
Ha-Jin Lee
Rapid organic contaminants removal by Mg-/Fe-based magnetic nanosheets synthesized using the molten salt method
Journal of Analytical Science and Technology
Magnetic nanosheets
Molten salt method
Dye adsorption
Catalyst
Wastewater treatment
title Rapid organic contaminants removal by Mg-/Fe-based magnetic nanosheets synthesized using the molten salt method
title_full Rapid organic contaminants removal by Mg-/Fe-based magnetic nanosheets synthesized using the molten salt method
title_fullStr Rapid organic contaminants removal by Mg-/Fe-based magnetic nanosheets synthesized using the molten salt method
title_full_unstemmed Rapid organic contaminants removal by Mg-/Fe-based magnetic nanosheets synthesized using the molten salt method
title_short Rapid organic contaminants removal by Mg-/Fe-based magnetic nanosheets synthesized using the molten salt method
title_sort rapid organic contaminants removal by mg fe based magnetic nanosheets synthesized using the molten salt method
topic Magnetic nanosheets
Molten salt method
Dye adsorption
Catalyst
Wastewater treatment
url https://doi.org/10.1186/s40543-025-00492-2
work_keys_str_mv AT sunghwakim rapidorganiccontaminantsremovalbymgfebasedmagneticnanosheetssynthesizedusingthemoltensaltmethod
AT chaeyoungkim rapidorganiccontaminantsremovalbymgfebasedmagneticnanosheetssynthesizedusingthemoltensaltmethod
AT sangmoonlee rapidorganiccontaminantsremovalbymgfebasedmagneticnanosheetssynthesizedusingthemoltensaltmethod
AT hajinlee rapidorganiccontaminantsremovalbymgfebasedmagneticnanosheetssynthesizedusingthemoltensaltmethod