Analysis and optimization of electrospinning parameters for fabricating thermoplastic polyurethanes (TPU) nanofibers by response surface methodology

Thermoplastic polyurethanes (TPU) have attracted increasing attention due to their excellent flexibility, chemical stability, processability and greenness. The traditional processes generally limit them to civil and industrial applications, but electrospun TPU nanofibers with high porosity, high spe...

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Main Authors: Lu Liu, Tian Luo, Xiaoju Kuang, Xiaoqian Wan, Xinhua Liang, Gaoming Jiang, Honglian Cong, Haijun He
Format: Article
Language:English
Published: Budapest University of Technology and Economics 2024-08-01
Series:eXPRESS Polymer Letters
Subjects:
Online Access:http://www.expresspolymlett.com/letolt.php?file=EPL-0012973&mi=cd
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author Lu Liu
Tian Luo
Xiaoju Kuang
Xiaoqian Wan
Xinhua Liang
Gaoming Jiang
Honglian Cong
Haijun He
author_facet Lu Liu
Tian Luo
Xiaoju Kuang
Xiaoqian Wan
Xinhua Liang
Gaoming Jiang
Honglian Cong
Haijun He
author_sort Lu Liu
collection DOAJ
description Thermoplastic polyurethanes (TPU) have attracted increasing attention due to their excellent flexibility, chemical stability, processability and greenness. The traditional processes generally limit them to civil and industrial applications, but electrospun TPU nanofibers with high porosity, high specific surface area and superior mechanical properties are promising in emerging fields. TPU nanofibers’ properties are affected by various electrospinning parameters, such as solution concentration, applied voltage, flow rate and rotational speed. Thus, 29 sets of experiments were designed here by the efficient and low-cost response surface methodology (RSM). The analysis of variance (ANOVA) revealed that the model agrees well with experimental results, and solution concentration is the most crucial parameter affecting nanofibers’ morphology and diameter. Based on it, the impacts of solution concentration and orientation on the mechanical properties of the TPU nanofiber membrane were investigated. Benefiting from the stress transfer and network deformation, the TPU nanofiber membranes parallel to the collection direction possessed the highest stress strength (23.71 MPa), while the nanofiber membranes vertical showed the widest strain range (485%). This study provides useful guidance for the preparation of high-performance TPU nanofibers, contributing to expanding its applicability in emerging fields such as biomedical, filtration and separation, and flexible sensing.
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publishDate 2024-08-01
publisher Budapest University of Technology and Economics
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series eXPRESS Polymer Letters
spelling doaj-art-fd42639e97544a55ad447b1b741d01a22025-08-20T03:22:23ZengBudapest University of Technology and EconomicseXPRESS Polymer Letters1788-618X2024-08-0118880781810.3144/expresspolymlett.2024.60Analysis and optimization of electrospinning parameters for fabricating thermoplastic polyurethanes (TPU) nanofibers by response surface methodologyLu LiuTian LuoXiaoju KuangXiaoqian WanXinhua LiangGaoming JiangHonglian CongHaijun HeThermoplastic polyurethanes (TPU) have attracted increasing attention due to their excellent flexibility, chemical stability, processability and greenness. The traditional processes generally limit them to civil and industrial applications, but electrospun TPU nanofibers with high porosity, high specific surface area and superior mechanical properties are promising in emerging fields. TPU nanofibers’ properties are affected by various electrospinning parameters, such as solution concentration, applied voltage, flow rate and rotational speed. Thus, 29 sets of experiments were designed here by the efficient and low-cost response surface methodology (RSM). The analysis of variance (ANOVA) revealed that the model agrees well with experimental results, and solution concentration is the most crucial parameter affecting nanofibers’ morphology and diameter. Based on it, the impacts of solution concentration and orientation on the mechanical properties of the TPU nanofiber membrane were investigated. Benefiting from the stress transfer and network deformation, the TPU nanofiber membranes parallel to the collection direction possessed the highest stress strength (23.71 MPa), while the nanofiber membranes vertical showed the widest strain range (485%). This study provides useful guidance for the preparation of high-performance TPU nanofibers, contributing to expanding its applicability in emerging fields such as biomedical, filtration and separation, and flexible sensing.http://www.expresspolymlett.com/letolt.php?file=EPL-0012973&mi=cd elastomer thermoplastic elastomer fiber spinning nanofiber mechanical properties
spellingShingle Lu Liu
Tian Luo
Xiaoju Kuang
Xiaoqian Wan
Xinhua Liang
Gaoming Jiang
Honglian Cong
Haijun He
Analysis and optimization of electrospinning parameters for fabricating thermoplastic polyurethanes (TPU) nanofibers by response surface methodology
eXPRESS Polymer Letters
elastomer
thermoplastic elastomer
fiber spinning
nanofiber
mechanical properties
title Analysis and optimization of electrospinning parameters for fabricating thermoplastic polyurethanes (TPU) nanofibers by response surface methodology
title_full Analysis and optimization of electrospinning parameters for fabricating thermoplastic polyurethanes (TPU) nanofibers by response surface methodology
title_fullStr Analysis and optimization of electrospinning parameters for fabricating thermoplastic polyurethanes (TPU) nanofibers by response surface methodology
title_full_unstemmed Analysis and optimization of electrospinning parameters for fabricating thermoplastic polyurethanes (TPU) nanofibers by response surface methodology
title_short Analysis and optimization of electrospinning parameters for fabricating thermoplastic polyurethanes (TPU) nanofibers by response surface methodology
title_sort analysis and optimization of electrospinning parameters for fabricating thermoplastic polyurethanes tpu nanofibers by response surface methodology
topic elastomer
thermoplastic elastomer
fiber spinning
nanofiber
mechanical properties
url http://www.expresspolymlett.com/letolt.php?file=EPL-0012973&mi=cd
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