Radiation-resistant Ti/BN coatings: insights from 171 days exposure to space radiation and atomic oxygen in low orbit

Abstract Atmospheric Plasma Spray (APS) and Vacuum Plasma Spray (VPS) techniques were used to develop Ti/2 vol.% hBN coatings, for extreme space environments and tested aboard the International Space Station as part of the MISSE-17 (Materials International Space Station Experiments) program. The coa...

Full description

Saved in:
Bibliographic Details
Main Authors: Abhijith Kunneparambil Sukumaran, Sara Rengifo, William Scott, Annette Gray, Miria Finckenor, Rony Thomas Murickan, Justin McElderry, Matthew Mazurkivich, Michael Renfro, Sang-Hyon Chu, Cheol Park, Anna Wu, Yifei Fu, Sudipta Seal, Arvind Agarwal
Format: Article
Language:English
Published: Nature Portfolio 2025-07-01
Series:npj Materials Degradation
Online Access:https://doi.org/10.1038/s41529-025-00644-0
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849235042152218624
author Abhijith Kunneparambil Sukumaran
Sara Rengifo
William Scott
Annette Gray
Miria Finckenor
Rony Thomas Murickan
Justin McElderry
Matthew Mazurkivich
Michael Renfro
Sang-Hyon Chu
Cheol Park
Anna Wu
Yifei Fu
Sudipta Seal
Arvind Agarwal
author_facet Abhijith Kunneparambil Sukumaran
Sara Rengifo
William Scott
Annette Gray
Miria Finckenor
Rony Thomas Murickan
Justin McElderry
Matthew Mazurkivich
Michael Renfro
Sang-Hyon Chu
Cheol Park
Anna Wu
Yifei Fu
Sudipta Seal
Arvind Agarwal
author_sort Abhijith Kunneparambil Sukumaran
collection DOAJ
description Abstract Atmospheric Plasma Spray (APS) and Vacuum Plasma Spray (VPS) techniques were used to develop Ti/2 vol.% hBN coatings, for extreme space environments and tested aboard the International Space Station as part of the MISSE-17 (Materials International Space Station Experiments) program. The coatings were exposed to atomic oxygen, space radiation, and low-orbit thermal cycling. VPS coatings showed a 56% increase in microhardness, a 26% rise in elastic modulus, minimal porosity and crack density changes compared to APS coatings. The change in mechanical properties is attributed to the formation of TiO, TiO₂ and TiN from nitrogen retention, alongside radiation-induced dislocations, which enhanced surface hardening. The oxidation of titanium led to the formation of TiO and TiO₂, while boron nitride was retained and underwent transmutation in VPS coatings. XPS and EDS analyses confirmed the enhanced space-environment resistance of VPS coatings, making them ideal for long-term spacecraft protection in lunar and Martian conditions.
format Article
id doaj-art-fa6bb056c53145bcbb0294bed06828ac
institution Kabale University
issn 2397-2106
language English
publishDate 2025-07-01
publisher Nature Portfolio
record_format Article
series npj Materials Degradation
spelling doaj-art-fa6bb056c53145bcbb0294bed06828ac2025-08-20T04:02:55ZengNature Portfolionpj Materials Degradation2397-21062025-07-019111610.1038/s41529-025-00644-0Radiation-resistant Ti/BN coatings: insights from 171 days exposure to space radiation and atomic oxygen in low orbitAbhijith Kunneparambil Sukumaran0Sara Rengifo1William Scott2Annette Gray3Miria Finckenor4Rony Thomas Murickan5Justin McElderry6Matthew Mazurkivich7Michael Renfro8Sang-Hyon Chu9Cheol Park10Anna Wu11Yifei Fu12Sudipta Seal13Arvind Agarwal14Plasma Forming Laboratory, Florida International UniversityMaterials Test, Chemistry and Contamination Control Branch, National Aeronautics and Space Administration Marshall Space Flight CentreMaterials Test, Chemistry and Contamination Control Branch, National Aeronautics and Space Administration Marshall Space Flight CentreMaterials Test, Chemistry and Contamination Control Branch, National Aeronautics and Space Administration Marshall Space Flight CentreMaterials Test, Chemistry and Contamination Control Branch, National Aeronautics and Space Administration Marshall Space Flight CentrePlasma Forming Laboratory, Florida International UniversityMaterials Test, Chemistry and Contamination Control Branch, National Aeronautics and Space Administration Marshall Space Flight CentreMaterials Test, Chemistry and Contamination Control Branch, National Aeronautics and Space Administration Marshall Space Flight CentrePlasma Processes, LLCAdvanced Materials and Processing Branch, NASA Langley Research CenterAdvanced Materials and Processing Branch, NASA Langley Research CenterAdvanced Materials and Processing Branch, NASA Langley Research CenterAdvanced Materials Processing and Analysis Centre, Nanoscience Technology Center, University of Central FloridaAdvanced Materials Processing and Analysis Centre, Nanoscience Technology Center, University of Central FloridaPlasma Forming Laboratory, Florida International UniversityAbstract Atmospheric Plasma Spray (APS) and Vacuum Plasma Spray (VPS) techniques were used to develop Ti/2 vol.% hBN coatings, for extreme space environments and tested aboard the International Space Station as part of the MISSE-17 (Materials International Space Station Experiments) program. The coatings were exposed to atomic oxygen, space radiation, and low-orbit thermal cycling. VPS coatings showed a 56% increase in microhardness, a 26% rise in elastic modulus, minimal porosity and crack density changes compared to APS coatings. The change in mechanical properties is attributed to the formation of TiO, TiO₂ and TiN from nitrogen retention, alongside radiation-induced dislocations, which enhanced surface hardening. The oxidation of titanium led to the formation of TiO and TiO₂, while boron nitride was retained and underwent transmutation in VPS coatings. XPS and EDS analyses confirmed the enhanced space-environment resistance of VPS coatings, making them ideal for long-term spacecraft protection in lunar and Martian conditions.https://doi.org/10.1038/s41529-025-00644-0
spellingShingle Abhijith Kunneparambil Sukumaran
Sara Rengifo
William Scott
Annette Gray
Miria Finckenor
Rony Thomas Murickan
Justin McElderry
Matthew Mazurkivich
Michael Renfro
Sang-Hyon Chu
Cheol Park
Anna Wu
Yifei Fu
Sudipta Seal
Arvind Agarwal
Radiation-resistant Ti/BN coatings: insights from 171 days exposure to space radiation and atomic oxygen in low orbit
npj Materials Degradation
title Radiation-resistant Ti/BN coatings: insights from 171 days exposure to space radiation and atomic oxygen in low orbit
title_full Radiation-resistant Ti/BN coatings: insights from 171 days exposure to space radiation and atomic oxygen in low orbit
title_fullStr Radiation-resistant Ti/BN coatings: insights from 171 days exposure to space radiation and atomic oxygen in low orbit
title_full_unstemmed Radiation-resistant Ti/BN coatings: insights from 171 days exposure to space radiation and atomic oxygen in low orbit
title_short Radiation-resistant Ti/BN coatings: insights from 171 days exposure to space radiation and atomic oxygen in low orbit
title_sort radiation resistant ti bn coatings insights from 171 days exposure to space radiation and atomic oxygen in low orbit
url https://doi.org/10.1038/s41529-025-00644-0
work_keys_str_mv AT abhijithkunneparambilsukumaran radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT sararengifo radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT williamscott radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT annettegray radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT miriafinckenor radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT ronythomasmurickan radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT justinmcelderry radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT matthewmazurkivich radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT michaelrenfro radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT sanghyonchu radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT cheolpark radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT annawu radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT yifeifu radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT sudiptaseal radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit
AT arvindagarwal radiationresistanttibncoatingsinsightsfrom171daysexposuretospaceradiationandatomicoxygeninloworbit