Forest Fire Smoke Layers Observed in the Free Troposphere over Portugal with a Multiwavelength Raman Lidar: Optical and Microphysical Properties

Vertically resolved optical and microphysical properties of biomass burning aerosols, measured in 2011 with a multiwavelength Raman lidar, are presented. The transportation time, within 1-2 days (or less), pointed towards the presence of relatively fresh smoke particles over the site. Some strong la...

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Main Authors: Sérgio Nepomuceno Pereira, Jana Preißler, Juan Luis Guerrero-Rascado, Ana Maria Silva, Frank Wagner
Format: Article
Language:English
Published: Wiley 2014-01-01
Series:The Scientific World Journal
Online Access:http://dx.doi.org/10.1155/2014/421838
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author Sérgio Nepomuceno Pereira
Jana Preißler
Juan Luis Guerrero-Rascado
Ana Maria Silva
Frank Wagner
author_facet Sérgio Nepomuceno Pereira
Jana Preißler
Juan Luis Guerrero-Rascado
Ana Maria Silva
Frank Wagner
author_sort Sérgio Nepomuceno Pereira
collection DOAJ
description Vertically resolved optical and microphysical properties of biomass burning aerosols, measured in 2011 with a multiwavelength Raman lidar, are presented. The transportation time, within 1-2 days (or less), pointed towards the presence of relatively fresh smoke particles over the site. Some strong layers aloft were observed with particle backscatter and extinction coefficients (at 355 nm) greater than 5 Mm−1 sr−1 and close to 300 Mm−1, respectively. The particle intensive optical properties showed features different from the ones reported for aged smoke, but rather consistent with fresh smoke. The Ångström exponents were generally high, mainly above 1.4, indicating a dominating accumulation mode. Weak depolarization values, as shown by the small depolarization ratio of 5% or lower, were measured. Furthermore, the lidar ratio presented no clear wavelength dependency. The inversion of the lidar signals provided a set of microphysical properties including particle effective radius below 0.2 μm, which is less than values previously observed for aged smoke particles. Real and imaginary parts of refractive index of about 1.5-1.6 and 0.02i, respectively, were derived. The single scattering albedo was in the range between 0.85 and 0.93; these last two quantities indicate the nonnegligible absorbing characteristics of the observed particles.
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language English
publishDate 2014-01-01
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series The Scientific World Journal
spelling doaj-art-f97bd70198634edb8f0b74bd119a29e52025-02-03T01:32:49ZengWileyThe Scientific World Journal2356-61401537-744X2014-01-01201410.1155/2014/421838421838Forest Fire Smoke Layers Observed in the Free Troposphere over Portugal with a Multiwavelength Raman Lidar: Optical and Microphysical PropertiesSérgio Nepomuceno Pereira0Jana Preißler1Juan Luis Guerrero-Rascado2Ana Maria Silva3Frank Wagner4Évora Geophysics Center, Rua Romão Ramalho 59, 7000 Évora, PortugalÉvora Geophysics Center, Rua Romão Ramalho 59, 7000 Évora, PortugalÉvora Geophysics Center, Rua Romão Ramalho 59, 7000 Évora, PortugalÉvora Geophysics Center, Rua Romão Ramalho 59, 7000 Évora, PortugalÉvora Geophysics Center, Rua Romão Ramalho 59, 7000 Évora, PortugalVertically resolved optical and microphysical properties of biomass burning aerosols, measured in 2011 with a multiwavelength Raman lidar, are presented. The transportation time, within 1-2 days (or less), pointed towards the presence of relatively fresh smoke particles over the site. Some strong layers aloft were observed with particle backscatter and extinction coefficients (at 355 nm) greater than 5 Mm−1 sr−1 and close to 300 Mm−1, respectively. The particle intensive optical properties showed features different from the ones reported for aged smoke, but rather consistent with fresh smoke. The Ångström exponents were generally high, mainly above 1.4, indicating a dominating accumulation mode. Weak depolarization values, as shown by the small depolarization ratio of 5% or lower, were measured. Furthermore, the lidar ratio presented no clear wavelength dependency. The inversion of the lidar signals provided a set of microphysical properties including particle effective radius below 0.2 μm, which is less than values previously observed for aged smoke particles. Real and imaginary parts of refractive index of about 1.5-1.6 and 0.02i, respectively, were derived. The single scattering albedo was in the range between 0.85 and 0.93; these last two quantities indicate the nonnegligible absorbing characteristics of the observed particles.http://dx.doi.org/10.1155/2014/421838
spellingShingle Sérgio Nepomuceno Pereira
Jana Preißler
Juan Luis Guerrero-Rascado
Ana Maria Silva
Frank Wagner
Forest Fire Smoke Layers Observed in the Free Troposphere over Portugal with a Multiwavelength Raman Lidar: Optical and Microphysical Properties
The Scientific World Journal
title Forest Fire Smoke Layers Observed in the Free Troposphere over Portugal with a Multiwavelength Raman Lidar: Optical and Microphysical Properties
title_full Forest Fire Smoke Layers Observed in the Free Troposphere over Portugal with a Multiwavelength Raman Lidar: Optical and Microphysical Properties
title_fullStr Forest Fire Smoke Layers Observed in the Free Troposphere over Portugal with a Multiwavelength Raman Lidar: Optical and Microphysical Properties
title_full_unstemmed Forest Fire Smoke Layers Observed in the Free Troposphere over Portugal with a Multiwavelength Raman Lidar: Optical and Microphysical Properties
title_short Forest Fire Smoke Layers Observed in the Free Troposphere over Portugal with a Multiwavelength Raman Lidar: Optical and Microphysical Properties
title_sort forest fire smoke layers observed in the free troposphere over portugal with a multiwavelength raman lidar optical and microphysical properties
url http://dx.doi.org/10.1155/2014/421838
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