Computational study on a puzzle in the biosynthetic pathway of anthocyanin: Why is an enzymatic oxidation/ reduction process required for a simple tautomerization?

In the late stage of anthocyanin biosynthesis, dihydroflavonol reductase (DFR) and anthocyanidin synthase (ANS) mediate a formal tautomerization. However, such oxidation/reduction process requires high energy and appears to be unnecessary, as the oxidation state does not change during the transforma...

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Bibliographic Details
Main Authors:	Hajime Sato, Chao Wang, Mami Yamazaki, Kazuki Saito, Masanobu Uchiyama
Format:	Article
Language:	English
Published:	Public Library of Science (PLoS) 2018-01-01
Series:	PLoS ONE
Online Access:	https://storage.googleapis.com/plos-corpus-prod/10.1371/journal.pone.0198944/1/pone.0198944.pdf?X-Goog-Algorithm=GOOG4-RSA-SHA256&X-Goog-Credential=wombat-sa%40plos-prod.iam.gserviceaccount.com%2F20210216%2Fauto%2Fstorage%2Fgoog4_request&X-Goog-Date=20210216T131449Z&X-Goog-Expires=3600&X-Goog-SignedHeaders=host&X-Goog-Signature=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Computational study on a puzzle in the biosynthetic pathway of anthocyanin: Why is an enzymatic oxidation/ reduction process required for a simple tautomerization?

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