Removal of tetracycline antibiotic from aqueous solution using bimetallic CuCo-ZIFs as an efficient catalyst in the presence of hydrogen peroxide
Antibiotics play an important role in disease treatment; however, they are also a threat to public health and the ecosystem. Therefore, a bimetallic CuCo-ZIFs catalyst was manufactured through the ultrasonic-assisted solvothermal method to activate H2O2 towards the removal of tetracycline (TC) in a...
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| Format: | Article |
| Language: | English |
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Can Tho University Publisher
2024-11-01
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| Series: | CTU Journal of Innovation and Sustainable Development |
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| Online Access: | http://web2010.thanhtoan/index.php/ctujs/article/view/881 |
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| author | Thu Le Bao Tran Ngoc Tri Tan Ho Luu Ngoc Hanh Cao Truong Ngoc Mai Ngo Huynh Vu Thanh Luong Huynh Giao Dang |
| author_facet | Thu Le Bao Tran Ngoc Tri Tan Ho Luu Ngoc Hanh Cao Truong Ngoc Mai Ngo Huynh Vu Thanh Luong Huynh Giao Dang |
| author_sort | Thu Le |
| collection | DOAJ |
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Antibiotics play an important role in disease treatment; however, they are also a threat to public health and the ecosystem. Therefore, a bimetallic CuCo-ZIFs catalyst was manufactured through the ultrasonic-assisted solvothermal method to activate H2O2 towards the removal of tetracycline (TC) in an aqueous environment, a polluting broad-spectrum antibiotic model. PXRD, SEM, TEM, EDX, TGA, FT-IR, and BET analyses indicated that CuCo-ZIFs cubic crystals were successfully synthesized with high crystallinity, large specific surface area, and ideal thermal stability. Factors affecting the TC removal were investigated, including CuCo-ZIFs dosage, H2O2 concentration, treatment time, initial TC concentration, and reaction temperature. The results showed that the CuCo-ZIFs/H2O2 catalytic system was capable of effectively handling TC, with about 93.9% of TC removed in the presence of 0.3 g.L-1 CuCo-ZIFs, 0.01 mol.L-1 H2O2 at room temperature within 30 min. Conclusively, this study contributes to expanding the application potential of bimetallic CuCo-ZIFs materials to eliminate antibiotic residues in an aqueous environment and inspire research on environmental improvement.
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| format | Article |
| id | doaj-art-f227e400b2a74a04859dfb8ea018bb0b |
| institution | OA Journals |
| issn | 2588-1418 2815-6412 |
| language | English |
| publishDate | 2024-11-01 |
| publisher | Can Tho University Publisher |
| record_format | Article |
| series | CTU Journal of Innovation and Sustainable Development |
| spelling | doaj-art-f227e400b2a74a04859dfb8ea018bb0b2025-08-20T02:02:26ZengCan Tho University PublisherCTU Journal of Innovation and Sustainable Development2588-14182815-64122024-11-01163Removal of tetracycline antibiotic from aqueous solution using bimetallic CuCo-ZIFs as an efficient catalyst in the presence of hydrogen peroxideThu Le Bao TranNgoc Tri Tan HoLuu Ngoc Hanh CaoTruong Ngoc Mai NgoHuynh Vu Thanh LuongHuynh Giao Dang0BM.Cong nghe Hoa hoc, Khoa Công nghệ Antibiotics play an important role in disease treatment; however, they are also a threat to public health and the ecosystem. Therefore, a bimetallic CuCo-ZIFs catalyst was manufactured through the ultrasonic-assisted solvothermal method to activate H2O2 towards the removal of tetracycline (TC) in an aqueous environment, a polluting broad-spectrum antibiotic model. PXRD, SEM, TEM, EDX, TGA, FT-IR, and BET analyses indicated that CuCo-ZIFs cubic crystals were successfully synthesized with high crystallinity, large specific surface area, and ideal thermal stability. Factors affecting the TC removal were investigated, including CuCo-ZIFs dosage, H2O2 concentration, treatment time, initial TC concentration, and reaction temperature. The results showed that the CuCo-ZIFs/H2O2 catalytic system was capable of effectively handling TC, with about 93.9% of TC removed in the presence of 0.3 g.L-1 CuCo-ZIFs, 0.01 mol.L-1 H2O2 at room temperature within 30 min. Conclusively, this study contributes to expanding the application potential of bimetallic CuCo-ZIFs materials to eliminate antibiotic residues in an aqueous environment and inspire research on environmental improvement. http://web2010.thanhtoan/index.php/ctujs/article/view/881Advanced oxidation processbimetallic ZIF-67hydrogen peroxidetetracycline removalzeolitic-imidazole frameworks |
| spellingShingle | Thu Le Bao Tran Ngoc Tri Tan Ho Luu Ngoc Hanh Cao Truong Ngoc Mai Ngo Huynh Vu Thanh Luong Huynh Giao Dang Removal of tetracycline antibiotic from aqueous solution using bimetallic CuCo-ZIFs as an efficient catalyst in the presence of hydrogen peroxide CTU Journal of Innovation and Sustainable Development Advanced oxidation process bimetallic ZIF-67 hydrogen peroxide tetracycline removal zeolitic-imidazole frameworks |
| title | Removal of tetracycline antibiotic from aqueous solution using bimetallic CuCo-ZIFs as an efficient catalyst in the presence of hydrogen peroxide |
| title_full | Removal of tetracycline antibiotic from aqueous solution using bimetallic CuCo-ZIFs as an efficient catalyst in the presence of hydrogen peroxide |
| title_fullStr | Removal of tetracycline antibiotic from aqueous solution using bimetallic CuCo-ZIFs as an efficient catalyst in the presence of hydrogen peroxide |
| title_full_unstemmed | Removal of tetracycline antibiotic from aqueous solution using bimetallic CuCo-ZIFs as an efficient catalyst in the presence of hydrogen peroxide |
| title_short | Removal of tetracycline antibiotic from aqueous solution using bimetallic CuCo-ZIFs as an efficient catalyst in the presence of hydrogen peroxide |
| title_sort | removal of tetracycline antibiotic from aqueous solution using bimetallic cuco zifs as an efficient catalyst in the presence of hydrogen peroxide |
| topic | Advanced oxidation process bimetallic ZIF-67 hydrogen peroxide tetracycline removal zeolitic-imidazole frameworks |
| url | http://web2010.thanhtoan/index.php/ctujs/article/view/881 |
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