Opportunities for gas-phase science at short-wavelength free-electron lasers with undulator-based polarization control
Free-electron lasers (FELs) are the world's most brilliant light sources with rapidly evolving technological capabilities in terms of ultrabright and ultrashort pulses over a large range of photon energies. Their revolutionary and innovative developments have opened new fields of science regard...
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American Physical Society
2025-01-01
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| Series: | Physical Review Research |
| Online Access: | http://doi.org/10.1103/PhysRevResearch.7.011001 |
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| author | Markus Ilchen Enrico Allaria Primož Rebernik Ribič Heinz-Dieter Nuhn Alberto Lutman Evgeny Schneidmiller Markus Tischer Mikail Yurkov Marco Calvi Eduard Prat Sven Reiche Thomas Schmidt Gianluca Aldo Geloni Suren Karabekyan Jiawei Yan Svitozar Serkez Zhangfeng Gao Bangjie Deng Chao Feng Haixiao Deng Wolfram Helml Lars Funke Mats Larsson Vitali Zhaunerchyk Michael Meyer Tommaso Mazza Till Jahnke Reinhard Dörner Francesca Calegari Olga Smirnova Caterina Vozzi Giovanni De Ninno Jonas Wätzel Jamal Berakdar Sadia Bari Lucas Schwob Jérémy R. Rouxel Shaul Mukamel Klaus Bartschat Kathryn Hamilton Luca Argenti Nicolas Douguet Nikolay M. Novikovskiy Philipp V. Demekhin Peter Walter |
| author_facet | Markus Ilchen Enrico Allaria Primož Rebernik Ribič Heinz-Dieter Nuhn Alberto Lutman Evgeny Schneidmiller Markus Tischer Mikail Yurkov Marco Calvi Eduard Prat Sven Reiche Thomas Schmidt Gianluca Aldo Geloni Suren Karabekyan Jiawei Yan Svitozar Serkez Zhangfeng Gao Bangjie Deng Chao Feng Haixiao Deng Wolfram Helml Lars Funke Mats Larsson Vitali Zhaunerchyk Michael Meyer Tommaso Mazza Till Jahnke Reinhard Dörner Francesca Calegari Olga Smirnova Caterina Vozzi Giovanni De Ninno Jonas Wätzel Jamal Berakdar Sadia Bari Lucas Schwob Jérémy R. Rouxel Shaul Mukamel Klaus Bartschat Kathryn Hamilton Luca Argenti Nicolas Douguet Nikolay M. Novikovskiy Philipp V. Demekhin Peter Walter |
| author_sort | Markus Ilchen |
| collection | DOAJ |
| description | Free-electron lasers (FELs) are the world's most brilliant light sources with rapidly evolving technological capabilities in terms of ultrabright and ultrashort pulses over a large range of photon energies. Their revolutionary and innovative developments have opened new fields of science regarding nonlinear light-matter interaction, the investigation of ultrafast processes from specific observer sites, and approaches to imaging matter with atomic resolution. A core aspect of FEL science is the study of isolated and prototypical systems in the gas phase with the possibility of addressing well-defined electronic transitions or particular atomic sites in molecules. Notably for polarization-controlled short-wavelength FELs, the gas phase offers new avenues for investigations of nonlinear and ultrafast phenomena in spin-orientated systems, for decoding the function of the chiral building blocks of life as well as steering reactions and particle emission dynamics in otherwise inaccessible ways. This roadmap comprises descriptions of technological capabilities of facilities worldwide, innovative diagnostics and instrumentation, as well as recent scientific highlights, novel methodology, and mathematical modeling. The experimental and theoretical landscape of using polarization controllable FELs for dichroic light-matter interaction in the gas phase will be discussed and comprehensively outlined to stimulate and strengthen global collaborative efforts of all disciplines. |
| format | Article |
| id | doaj-art-f1cc761226394699b0cd1e046080198c |
| institution | Kabale University |
| issn | 2643-1564 |
| language | English |
| publishDate | 2025-01-01 |
| publisher | American Physical Society |
| record_format | Article |
| series | Physical Review Research |
| spelling | doaj-art-f1cc761226394699b0cd1e046080198c2025-01-27T17:57:09ZengAmerican Physical SocietyPhysical Review Research2643-15642025-01-017101100110.1103/PhysRevResearch.7.011001Opportunities for gas-phase science at short-wavelength free-electron lasers with undulator-based polarization controlMarkus IlchenEnrico AllariaPrimož Rebernik RibičHeinz-Dieter NuhnAlberto LutmanEvgeny SchneidmillerMarkus TischerMikail YurkovMarco CalviEduard PratSven ReicheThomas SchmidtGianluca Aldo GeloniSuren KarabekyanJiawei YanSvitozar SerkezZhangfeng GaoBangjie DengChao FengHaixiao DengWolfram HelmlLars FunkeMats LarssonVitali ZhaunerchykMichael MeyerTommaso MazzaTill JahnkeReinhard DörnerFrancesca CalegariOlga SmirnovaCaterina VozziGiovanni De NinnoJonas WätzelJamal BerakdarSadia BariLucas SchwobJérémy R. RouxelShaul MukamelKlaus BartschatKathryn HamiltonLuca ArgentiNicolas DouguetNikolay M. NovikovskiyPhilipp V. DemekhinPeter WalterFree-electron lasers (FELs) are the world's most brilliant light sources with rapidly evolving technological capabilities in terms of ultrabright and ultrashort pulses over a large range of photon energies. Their revolutionary and innovative developments have opened new fields of science regarding nonlinear light-matter interaction, the investigation of ultrafast processes from specific observer sites, and approaches to imaging matter with atomic resolution. A core aspect of FEL science is the study of isolated and prototypical systems in the gas phase with the possibility of addressing well-defined electronic transitions or particular atomic sites in molecules. Notably for polarization-controlled short-wavelength FELs, the gas phase offers new avenues for investigations of nonlinear and ultrafast phenomena in spin-orientated systems, for decoding the function of the chiral building blocks of life as well as steering reactions and particle emission dynamics in otherwise inaccessible ways. This roadmap comprises descriptions of technological capabilities of facilities worldwide, innovative diagnostics and instrumentation, as well as recent scientific highlights, novel methodology, and mathematical modeling. The experimental and theoretical landscape of using polarization controllable FELs for dichroic light-matter interaction in the gas phase will be discussed and comprehensively outlined to stimulate and strengthen global collaborative efforts of all disciplines.http://doi.org/10.1103/PhysRevResearch.7.011001 |
| spellingShingle | Markus Ilchen Enrico Allaria Primož Rebernik Ribič Heinz-Dieter Nuhn Alberto Lutman Evgeny Schneidmiller Markus Tischer Mikail Yurkov Marco Calvi Eduard Prat Sven Reiche Thomas Schmidt Gianluca Aldo Geloni Suren Karabekyan Jiawei Yan Svitozar Serkez Zhangfeng Gao Bangjie Deng Chao Feng Haixiao Deng Wolfram Helml Lars Funke Mats Larsson Vitali Zhaunerchyk Michael Meyer Tommaso Mazza Till Jahnke Reinhard Dörner Francesca Calegari Olga Smirnova Caterina Vozzi Giovanni De Ninno Jonas Wätzel Jamal Berakdar Sadia Bari Lucas Schwob Jérémy R. Rouxel Shaul Mukamel Klaus Bartschat Kathryn Hamilton Luca Argenti Nicolas Douguet Nikolay M. Novikovskiy Philipp V. Demekhin Peter Walter Opportunities for gas-phase science at short-wavelength free-electron lasers with undulator-based polarization control Physical Review Research |
| title | Opportunities for gas-phase science at short-wavelength free-electron lasers with undulator-based polarization control |
| title_full | Opportunities for gas-phase science at short-wavelength free-electron lasers with undulator-based polarization control |
| title_fullStr | Opportunities for gas-phase science at short-wavelength free-electron lasers with undulator-based polarization control |
| title_full_unstemmed | Opportunities for gas-phase science at short-wavelength free-electron lasers with undulator-based polarization control |
| title_short | Opportunities for gas-phase science at short-wavelength free-electron lasers with undulator-based polarization control |
| title_sort | opportunities for gas phase science at short wavelength free electron lasers with undulator based polarization control |
| url | http://doi.org/10.1103/PhysRevResearch.7.011001 |
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