In Situ Generated Sulfate-Facilitated Efficient Nitrate Electrosynthesis on 2D PdS2 with Unique Imitating Growth Feature
Highlights Unique imitating growth feature for PdS2 on different 2D substrates has been firstly discovered for constructing 2D/2D heterostructures by interface engineering. The thin and small PdS2 nanoplates with active defects can be inducted by poly(1-vinyl-3-ethylimidazolium bromide (PVEIB), resu...
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| Main Authors: | , , , , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
SpringerOpen
2025-06-01
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| Series: | Nano-Micro Letters |
| Subjects: | |
| Online Access: | https://doi.org/10.1007/s40820-025-01803-3 |
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| Summary: | Highlights Unique imitating growth feature for PdS2 on different 2D substrates has been firstly discovered for constructing 2D/2D heterostructures by interface engineering. The thin and small PdS2 nanoplates with active defects can be inducted by poly(1-vinyl-3-ethylimidazolium bromide (PVEIB), resulting in the obtained PdS2@PVEIB/PPy/GO exhibited the excellent nitrogen oxidation reaction (NOR) electroactivity with the outstanding stability and selectivity. The in situ generation of SO4 2−, caused by the oxidation during the preparation process or exposed in air, as well as at high NOR potential, plays a crucial role in reducing the activation energy of the NOR process, leading to improved efficiency for nitrate production. |
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| ISSN: | 2311-6706 2150-5551 |