Gelsolin-mediated actin filament severing, mechanics, and conformational changes at neutral and acidic pH

Gelsolin is a calcium (Ca2+) dependent, pH sensitive actin-binding protein that regulates actin filament dynamics to remodel the actin cytoskeleton. It is known that gelsolin binding induces conformational changes of actin filaments, leading to filament severing. However, the influence of physiologi...

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Main Authors: Taylor V. Douglas, Claire A. Toland, Sydney A. Paulin, Nicholas Castaneda, Laurene Tetard, Ellen H. Kang
Format: Article
Language:English
Published: Frontiers Media S.A. 2025-03-01
Series:Frontiers in Soft Matter
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Online Access:https://www.frontiersin.org/articles/10.3389/frsfm.2025.1530439/full
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author Taylor V. Douglas
Taylor V. Douglas
Claire A. Toland
Sydney A. Paulin
Nicholas Castaneda
Nicholas Castaneda
Laurene Tetard
Laurene Tetard
Ellen H. Kang
Ellen H. Kang
Ellen H. Kang
author_facet Taylor V. Douglas
Taylor V. Douglas
Claire A. Toland
Sydney A. Paulin
Nicholas Castaneda
Nicholas Castaneda
Laurene Tetard
Laurene Tetard
Ellen H. Kang
Ellen H. Kang
Ellen H. Kang
author_sort Taylor V. Douglas
collection DOAJ
description Gelsolin is a calcium (Ca2+) dependent, pH sensitive actin-binding protein that regulates actin filament dynamics to remodel the actin cytoskeleton. It is known that gelsolin binding induces conformational changes of actin filaments, leading to filament severing. However, the influence of physiological conditions, such as pH variations, on gelsolin-mediated filament severing activities, mechanics and conformations remains unclear despite their role in actin-actin interactions. Using Total Internal Reflection Fluorescence (TIRF) microscopy imaging and pyrene fluorescence assays, we demonstrate that filament severing efficiencies by gelsolin are enhanced in acidic conditions. In addition, analysis of filament thermal fluctuations using TIRF reveals that gelsolin binding stiffens actin filaments. Furthermore, we show that gelsolin binding induces conformational changes in filaments by measuring the filament half-pitch using high resolution Atomic Force Microscopy imaging. Together, our results suggest that pH modulation plays a key role in gelsolin-mediated filament severing activities, bending mechanics, and conformational changes, which have implications in many cellular processes including cell motility and morphogenesis.
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spelling doaj-art-efefeafd0abf43f09f7c9cb73cec33a72025-08-20T03:39:57ZengFrontiers Media S.A.Frontiers in Soft Matter2813-04992025-03-01510.3389/frsfm.2025.15304391530439Gelsolin-mediated actin filament severing, mechanics, and conformational changes at neutral and acidic pHTaylor V. Douglas0Taylor V. Douglas1Claire A. Toland2Sydney A. Paulin3Nicholas Castaneda4Nicholas Castaneda5Laurene Tetard6Laurene Tetard7Ellen H. Kang8Ellen H. Kang9Ellen H. Kang10NanoScience Technology Center, University of Central Florida, Orlando, FL, United StatesDepartment of Physics, College of Sciences, University of Central Florida, Orlando, FL, United StatesNanoScience Technology Center, University of Central Florida, Orlando, FL, United StatesNanoScience Technology Center, University of Central Florida, Orlando, FL, United StatesNanoScience Technology Center, University of Central Florida, Orlando, FL, United StatesBurnett School of Biomedical Sciences, College of Medicine, University of Central Florda, Orlando, FL, United StatesNanoScience Technology Center, University of Central Florida, Orlando, FL, United StatesDepartment of Physics, College of Sciences, University of Central Florida, Orlando, FL, United StatesNanoScience Technology Center, University of Central Florida, Orlando, FL, United StatesDepartment of Physics, College of Sciences, University of Central Florida, Orlando, FL, United StatesDepartmnet of Material Science and Engineering, College of Engineering and Computer Science University of Central Florida, Orlando, FL, United StatesGelsolin is a calcium (Ca2+) dependent, pH sensitive actin-binding protein that regulates actin filament dynamics to remodel the actin cytoskeleton. It is known that gelsolin binding induces conformational changes of actin filaments, leading to filament severing. However, the influence of physiological conditions, such as pH variations, on gelsolin-mediated filament severing activities, mechanics and conformations remains unclear despite their role in actin-actin interactions. Using Total Internal Reflection Fluorescence (TIRF) microscopy imaging and pyrene fluorescence assays, we demonstrate that filament severing efficiencies by gelsolin are enhanced in acidic conditions. In addition, analysis of filament thermal fluctuations using TIRF reveals that gelsolin binding stiffens actin filaments. Furthermore, we show that gelsolin binding induces conformational changes in filaments by measuring the filament half-pitch using high resolution Atomic Force Microscopy imaging. Together, our results suggest that pH modulation plays a key role in gelsolin-mediated filament severing activities, bending mechanics, and conformational changes, which have implications in many cellular processes including cell motility and morphogenesis.https://www.frontiersin.org/articles/10.3389/frsfm.2025.1530439/fullactin cytoskeletongelsolinseveringbending mechanicsfilament conformationintracellular pH
spellingShingle Taylor V. Douglas
Taylor V. Douglas
Claire A. Toland
Sydney A. Paulin
Nicholas Castaneda
Nicholas Castaneda
Laurene Tetard
Laurene Tetard
Ellen H. Kang
Ellen H. Kang
Ellen H. Kang
Gelsolin-mediated actin filament severing, mechanics, and conformational changes at neutral and acidic pH
Frontiers in Soft Matter
actin cytoskeleton
gelsolin
severing
bending mechanics
filament conformation
intracellular pH
title Gelsolin-mediated actin filament severing, mechanics, and conformational changes at neutral and acidic pH
title_full Gelsolin-mediated actin filament severing, mechanics, and conformational changes at neutral and acidic pH
title_fullStr Gelsolin-mediated actin filament severing, mechanics, and conformational changes at neutral and acidic pH
title_full_unstemmed Gelsolin-mediated actin filament severing, mechanics, and conformational changes at neutral and acidic pH
title_short Gelsolin-mediated actin filament severing, mechanics, and conformational changes at neutral and acidic pH
title_sort gelsolin mediated actin filament severing mechanics and conformational changes at neutral and acidic ph
topic actin cytoskeleton
gelsolin
severing
bending mechanics
filament conformation
intracellular pH
url https://www.frontiersin.org/articles/10.3389/frsfm.2025.1530439/full
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