A Reconfigurable Polarimetric Photodetector Based on the MoS<sub>2</sub>/PdSe<sub>2</sub> Heterostructure with a Charge-Trap Gate Stack

Besides the intensity and wavelength, the ability to analyze the optical polarization of detected light can provide a new degree of freedom for numerous applications, such as object recognition, biomedical applications, environmental monitoring, and remote sensing imaging. However, conventional filt...

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Bibliographic Details
Main Authors: Xin Huang, Qinghu Bai, Yang Guo, Qijie Liang, Tengzhang Liu, Wugang Liao, Aizi Jin, Baogang Quan, Haifang Yang, Baoli Liu, Changzhi Gu
Format: Article
Language:English
Published: MDPI AG 2024-12-01
Series:Nanomaterials
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Online Access:https://www.mdpi.com/2079-4991/14/23/1936
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Summary:Besides the intensity and wavelength, the ability to analyze the optical polarization of detected light can provide a new degree of freedom for numerous applications, such as object recognition, biomedical applications, environmental monitoring, and remote sensing imaging. However, conventional filter-integrated polarimetric sensing systems require complex optical components and a complicated fabrication process, severely limiting their on-chip miniaturization and functionalities. Herein, the reconfigurable polarimetric photodetection with photovoltaic mode is developed based on a few-layer MoS<sub>2</sub>/PdSe<sub>2</sub> heterostructure channel and a charge-trap structure composed of Al<sub>2</sub>O<sub>3</sub>/HfO<sub>2</sub>/Al<sub>2</sub>O<sub>3</sub> (AHA)-stacked dielectrics. Because of the remarkable charge-trapping ability of carriers in the AHA stack, the MoS<sub>2</sub>/PdSe<sub>2</sub> channel exhibits a high program/erase current ratio of 10<sup>5</sup> and a memory window exceeding 20 V. Moreover, the photovoltaic mode of the MoS<sub>2</sub>/PdSe<sub>2</sub> Schottky diode can be operated and manipulable, resulting in high and distinct responsivities in the visible broadband. Interestingly, the linear polarization of the device can be modulated under program/erase states, enabling the reconfigurable capability of linearly polarized photodetection. This study demonstrates a new prototype heterostructure-based photodetector with the capability of both tunable responsivity and linear polarization, demonstrating great potential application toward reconfigurable photosensing and polarization-resolved imaging applications.
ISSN:2079-4991