Adsorption and Co-Adsorption of Polyaldehyde Dextran Nanoparticles and Nonionic Surfactant at an Air–Water Interface: Potential Implications for Pulmonary Drug Delivery

Measurements of dynamic surface tension were carried out in aqueous systems (water or 0.1 mM Triton X-100) comprising nanoparticles formed from chemically modified polyaldehyde dextran (PAD). The nanostructures, considered as potential drug carriers in aerosol therapy, were obtained from biocompatib...

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Main Authors: Jabłczyńska Katarzyna, Sosnowski Tomasz R.
Format: Article
Language:English
Published: Polish Academy of Sciences Committee of Chemical and Process Engineering 2017-03-01
Series:Chemical and Process Engineering
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Online Access:http://www.degruyter.com/view/j/cpe.2017.38.issue-1/cpe-2017-0006/cpe-2017-0006.xml?format=INT
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author Jabłczyńska Katarzyna
Sosnowski Tomasz R.
author_facet Jabłczyńska Katarzyna
Sosnowski Tomasz R.
author_sort Jabłczyńska Katarzyna
collection DOAJ
description Measurements of dynamic surface tension were carried out in aqueous systems (water or 0.1 mM Triton X-100) comprising nanoparticles formed from chemically modified polyaldehyde dextran (PAD). The nanostructures, considered as potential drug carriers in aerosol therapy, were obtained from biocompatible polysaccharides by successive oxidation and reactive coiling in an aqueous solution. The dynamic surface tension of the samples was determined by the maximum bubble pressure (MBP) method and by the axisymmetric drop shape analysis (ADSA). Experiments with harmonic area perturbations were also carried out in order to determine surface dilatational viscoelasticity. PAD showed a remarkable surface activity. Ward-Tordai equation was used to determine the equilibrium surface tension and diffusion coefficient of PAD nanoparticles (D = 2.3×10-6 m2/s). In a mixture with Triton X-100, PAD particles showed co-adsorption and synergic effect in surface tension reduction at short times (below 10 s). Tested nanoparticles had impact on surface rheology in a mixed system with nonionic surfactant, suggesting their possible interactions with the lung surfactant system after inhalation. This preliminary investigation sets the methodological approach for further research related to the influence of inhaled PAD nanoparticles on the lung surfactant and mass transfer processes in the respiratory system.
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spelling doaj-art-ef542d25079a403883be2bc255b6dbb72025-08-20T02:13:36ZengPolish Academy of Sciences Committee of Chemical and Process EngineeringChemical and Process Engineering2300-19252017-03-01381677710.1515/cpe-2017-0006cpe-2017-0006Adsorption and Co-Adsorption of Polyaldehyde Dextran Nanoparticles and Nonionic Surfactant at an Air–Water Interface: Potential Implications for Pulmonary Drug DeliveryJabłczyńska Katarzyna0Sosnowski Tomasz R.1Warsaw University of Technology, Faculty of Chemical and Process Engineering, Waryńskiego 1, 00-645 Warsaw, PolandWarsaw University of Technology, Faculty of Chemical and Process Engineering, Waryńskiego 1, 00-645 Warsaw, PolandMeasurements of dynamic surface tension were carried out in aqueous systems (water or 0.1 mM Triton X-100) comprising nanoparticles formed from chemically modified polyaldehyde dextran (PAD). The nanostructures, considered as potential drug carriers in aerosol therapy, were obtained from biocompatible polysaccharides by successive oxidation and reactive coiling in an aqueous solution. The dynamic surface tension of the samples was determined by the maximum bubble pressure (MBP) method and by the axisymmetric drop shape analysis (ADSA). Experiments with harmonic area perturbations were also carried out in order to determine surface dilatational viscoelasticity. PAD showed a remarkable surface activity. Ward-Tordai equation was used to determine the equilibrium surface tension and diffusion coefficient of PAD nanoparticles (D = 2.3×10-6 m2/s). In a mixture with Triton X-100, PAD particles showed co-adsorption and synergic effect in surface tension reduction at short times (below 10 s). Tested nanoparticles had impact on surface rheology in a mixed system with nonionic surfactant, suggesting their possible interactions with the lung surfactant system after inhalation. This preliminary investigation sets the methodological approach for further research related to the influence of inhaled PAD nanoparticles on the lung surfactant and mass transfer processes in the respiratory system.http://www.degruyter.com/view/j/cpe.2017.38.issue-1/cpe-2017-0006/cpe-2017-0006.xml?format=INTpolysaccharide nanoparticleslung surfactantdynamic surface tensionsurface viscoelasticityhysteresis
spellingShingle Jabłczyńska Katarzyna
Sosnowski Tomasz R.
Adsorption and Co-Adsorption of Polyaldehyde Dextran Nanoparticles and Nonionic Surfactant at an Air–Water Interface: Potential Implications for Pulmonary Drug Delivery
Chemical and Process Engineering
polysaccharide nanoparticles
lung surfactant
dynamic surface tension
surface viscoelasticity
hysteresis
title Adsorption and Co-Adsorption of Polyaldehyde Dextran Nanoparticles and Nonionic Surfactant at an Air–Water Interface: Potential Implications for Pulmonary Drug Delivery
title_full Adsorption and Co-Adsorption of Polyaldehyde Dextran Nanoparticles and Nonionic Surfactant at an Air–Water Interface: Potential Implications for Pulmonary Drug Delivery
title_fullStr Adsorption and Co-Adsorption of Polyaldehyde Dextran Nanoparticles and Nonionic Surfactant at an Air–Water Interface: Potential Implications for Pulmonary Drug Delivery
title_full_unstemmed Adsorption and Co-Adsorption of Polyaldehyde Dextran Nanoparticles and Nonionic Surfactant at an Air–Water Interface: Potential Implications for Pulmonary Drug Delivery
title_short Adsorption and Co-Adsorption of Polyaldehyde Dextran Nanoparticles and Nonionic Surfactant at an Air–Water Interface: Potential Implications for Pulmonary Drug Delivery
title_sort adsorption and co adsorption of polyaldehyde dextran nanoparticles and nonionic surfactant at an air water interface potential implications for pulmonary drug delivery
topic polysaccharide nanoparticles
lung surfactant
dynamic surface tension
surface viscoelasticity
hysteresis
url http://www.degruyter.com/view/j/cpe.2017.38.issue-1/cpe-2017-0006/cpe-2017-0006.xml?format=INT
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