Development of waterborne epoxy-based resin incorporated with modified natural rubber latex for coating application

Abstract Water-based coating has gained much attention globally due to environmental issues. This work aims to develop a waterborne epoxy coating incorporated with modified natural rubber (NR) latex for improved performance. For this purpose, the NR latex was modified into three types of low molecul...

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Main Authors: Wasan Tessanan, Thanchanok Ratvijitvech, Sombat Thanawan, Taweechai Amornsakchai, Pranee Phinyocheep
Format: Article
Language:English
Published: Nature Portfolio 2024-11-01
Series:Scientific Reports
Subjects:
Online Access:https://doi.org/10.1038/s41598-024-77990-7
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author Wasan Tessanan
Thanchanok Ratvijitvech
Sombat Thanawan
Taweechai Amornsakchai
Pranee Phinyocheep
author_facet Wasan Tessanan
Thanchanok Ratvijitvech
Sombat Thanawan
Taweechai Amornsakchai
Pranee Phinyocheep
author_sort Wasan Tessanan
collection DOAJ
description Abstract Water-based coating has gained much attention globally due to environmental issues. This work aims to develop a waterborne epoxy coating incorporated with modified natural rubber (NR) latex for improved performance. For this purpose, the NR latex was modified into three types of low molecular weight epoxidized natural rubber (LENR) latex. The waterborne epoxy resin was prepared by simply mixing the epoxy resin with an amine curing agent in water and various LENR latex contents (10 to 50 wt%). The waterborne epoxy/LENR blend was coated on a tin substrate and the cured coating demonstrated better adhesion and bending properties than the neat epoxy. Phase morphological properties displayed a rough surface with a heterogeneous surface structure of the dispersed rubber and epoxy matrix. Two glass transition temperatures were observed, corresponding to the rubber modifier and the epoxy matrix. The mechanical properties of the thermosetting epoxy/LENR blends were assessed, revealing a maximum increment in elongation ability by approximately 370% for adding 50 wt% LENR, compared to the neat epoxy. These results hold the potential avenue for utilizing NR-based material in the waterborne epoxy-based resin for coating applications. Furthermore, it contributes to the NR, a renewable and eco-friendly material, in the coating technology, embracing a sustainable future.
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spelling doaj-art-ef2b87d47fcd4260909b2a62f970e14f2025-08-20T02:50:00ZengNature PortfolioScientific Reports2045-23222024-11-0114111810.1038/s41598-024-77990-7Development of waterborne epoxy-based resin incorporated with modified natural rubber latex for coating applicationWasan Tessanan0Thanchanok Ratvijitvech1Sombat Thanawan2Taweechai Amornsakchai3Pranee Phinyocheep4Department of Chemistry, Faculty of Science, Mahidol UniversityDepartment of Chemistry, Faculty of Science, Mahidol UniversityRubber Technology Research Center, Faculty of Science, Mahidol UniversityDepartment of Chemistry, Faculty of Science, Mahidol UniversityDepartment of Chemistry, Faculty of Science, Mahidol UniversityAbstract Water-based coating has gained much attention globally due to environmental issues. This work aims to develop a waterborne epoxy coating incorporated with modified natural rubber (NR) latex for improved performance. For this purpose, the NR latex was modified into three types of low molecular weight epoxidized natural rubber (LENR) latex. The waterborne epoxy resin was prepared by simply mixing the epoxy resin with an amine curing agent in water and various LENR latex contents (10 to 50 wt%). The waterborne epoxy/LENR blend was coated on a tin substrate and the cured coating demonstrated better adhesion and bending properties than the neat epoxy. Phase morphological properties displayed a rough surface with a heterogeneous surface structure of the dispersed rubber and epoxy matrix. Two glass transition temperatures were observed, corresponding to the rubber modifier and the epoxy matrix. The mechanical properties of the thermosetting epoxy/LENR blends were assessed, revealing a maximum increment in elongation ability by approximately 370% for adding 50 wt% LENR, compared to the neat epoxy. These results hold the potential avenue for utilizing NR-based material in the waterborne epoxy-based resin for coating applications. Furthermore, it contributes to the NR, a renewable and eco-friendly material, in the coating technology, embracing a sustainable future.https://doi.org/10.1038/s41598-024-77990-7Modified natural rubbersWaterborne epoxyEco-friendly materialsTougheningCoating applications
spellingShingle Wasan Tessanan
Thanchanok Ratvijitvech
Sombat Thanawan
Taweechai Amornsakchai
Pranee Phinyocheep
Development of waterborne epoxy-based resin incorporated with modified natural rubber latex for coating application
Scientific Reports
Modified natural rubbers
Waterborne epoxy
Eco-friendly materials
Toughening
Coating applications
title Development of waterborne epoxy-based resin incorporated with modified natural rubber latex for coating application
title_full Development of waterborne epoxy-based resin incorporated with modified natural rubber latex for coating application
title_fullStr Development of waterborne epoxy-based resin incorporated with modified natural rubber latex for coating application
title_full_unstemmed Development of waterborne epoxy-based resin incorporated with modified natural rubber latex for coating application
title_short Development of waterborne epoxy-based resin incorporated with modified natural rubber latex for coating application
title_sort development of waterborne epoxy based resin incorporated with modified natural rubber latex for coating application
topic Modified natural rubbers
Waterborne epoxy
Eco-friendly materials
Toughening
Coating applications
url https://doi.org/10.1038/s41598-024-77990-7
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AT sombatthanawan developmentofwaterborneepoxybasedresinincorporatedwithmodifiednaturalrubberlatexforcoatingapplication
AT taweechaiamornsakchai developmentofwaterborneepoxybasedresinincorporatedwithmodifiednaturalrubberlatexforcoatingapplication
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