Sample preparation method for IR analysis of petroleum-contaminated soil: An innovative technology for ecological remediation using Miscanthus x giganteus

Miscanthus x giganteus phytoremediation of soil contaminated with petroleum was assessed in this study. A method of soil sample preparation for determining the total content of petroleum products by infrared spectrophotometry has been developed. It is a one-stage extraction method with minimal use o...

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Main Authors: Ruslana Huminilovych, Vitalii Stadnik, Martyn Sozanskyi, Pavlo Shapoval, Valentina Pidlisnyuk, Ihor Poliuzhyn, Viktoriia Kochubei, Yurii Hrynchuk, Bohdan Korchak
Format: Article
Language:English
Published: Elsevier 2024-12-01
Series:Heliyon
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Online Access:http://www.sciencedirect.com/science/article/pii/S2405844024167448
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author Ruslana Huminilovych
Vitalii Stadnik
Martyn Sozanskyi
Pavlo Shapoval
Valentina Pidlisnyuk
Ihor Poliuzhyn
Viktoriia Kochubei
Yurii Hrynchuk
Bohdan Korchak
author_facet Ruslana Huminilovych
Vitalii Stadnik
Martyn Sozanskyi
Pavlo Shapoval
Valentina Pidlisnyuk
Ihor Poliuzhyn
Viktoriia Kochubei
Yurii Hrynchuk
Bohdan Korchak
author_sort Ruslana Huminilovych
collection DOAJ
description Miscanthus x giganteus phytoremediation of soil contaminated with petroleum was assessed in this study. A method of soil sample preparation for determining the total content of petroleum products by infrared spectrophotometry has been developed. It is a one-stage extraction method with minimal use of carbon tetrachloride as an extractant. This soil sample preparation method was environmentally friendly and cost-effective, as it required a significantly lower amount of extractant (15–30 ml of tetrachloromethane) compared to the commonly used threefold extraction method, which uses up to 150 ml of extractant. The extraction degree of petroleum products (PP) was determined to be from 81.78 % to 94.22 % after two days of extraction using the additive method of determining PP. It was observed that the presence of different fertilizer additives in the soil samples led to a reduction in the determined PP content in the following series: “without fertilizer” – “Biochar” additive – “Biohumus” additive. These results were compared with reference samples that did not involve the use of Miscanthus x giganteus. Furthermore, the main thermolysis stages of petroleum products sorbed by the soil matrix and the thermal behavior of an artificial soil sample spiked with PP were examined. Detailed interpretation of thermograms of laboratory soil samples was conducted at various phytoremediation stages.
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spelling doaj-art-eebd9be0251f47e8a9a005358f936e462025-08-20T01:59:31ZengElsevierHeliyon2405-84402024-12-011023e4071310.1016/j.heliyon.2024.e40713Sample preparation method for IR analysis of petroleum-contaminated soil: An innovative technology for ecological remediation using Miscanthus x giganteusRuslana Huminilovych0Vitalii Stadnik1Martyn Sozanskyi2Pavlo Shapoval3Valentina Pidlisnyuk4Ihor Poliuzhyn5Viktoriia Kochubei6Yurii Hrynchuk7Bohdan Korchak8Department of Physical, Analytical and General Chemistry, Lviv Polytechnic National University, 12 S. Bandery St., 79013, Lviv, Ukraine; Corresponding author.Department of Physical, Analytical and General Chemistry, Lviv Polytechnic National University, 12 S. Bandery St., 79013, Lviv, UkraineDepartment of Physical, Analytical and General Chemistry, Lviv Polytechnic National University, 12 S. Bandery St., 79013, Lviv, UkraineDepartment of Physical, Analytical and General Chemistry, Lviv Polytechnic National University, 12 S. Bandery St., 79013, Lviv, UkraineDepartment of Environmental Chemistry and Technology, Faculty of Environment, Jan Evangelista Purkyne University in Ústí nad Labem, 400 96, Ústí nad Labem, Czech RepublicDepartment of Physical, Analytical and General Chemistry, Lviv Polytechnic National University, 12 S. Bandery St., 79013, Lviv, UkraineDepartment of Physical, Analytical and General Chemistry, Lviv Polytechnic National University, 12 S. Bandery St., 79013, Lviv, UkraineDepartment of Physical, Analytical and General Chemistry, Lviv Polytechnic National University, 12 S. Bandery St., 79013, Lviv, UkraineDepartment of Civil Safety, Lviv Polytechnic National University, 12 S. Bandery St., 79013, Lviv, UkraineMiscanthus x giganteus phytoremediation of soil contaminated with petroleum was assessed in this study. A method of soil sample preparation for determining the total content of petroleum products by infrared spectrophotometry has been developed. It is a one-stage extraction method with minimal use of carbon tetrachloride as an extractant. This soil sample preparation method was environmentally friendly and cost-effective, as it required a significantly lower amount of extractant (15–30 ml of tetrachloromethane) compared to the commonly used threefold extraction method, which uses up to 150 ml of extractant. The extraction degree of petroleum products (PP) was determined to be from 81.78 % to 94.22 % after two days of extraction using the additive method of determining PP. It was observed that the presence of different fertilizer additives in the soil samples led to a reduction in the determined PP content in the following series: “without fertilizer” – “Biochar” additive – “Biohumus” additive. These results were compared with reference samples that did not involve the use of Miscanthus x giganteus. Furthermore, the main thermolysis stages of petroleum products sorbed by the soil matrix and the thermal behavior of an artificial soil sample spiked with PP were examined. Detailed interpretation of thermograms of laboratory soil samples was conducted at various phytoremediation stages.http://www.sciencedirect.com/science/article/pii/S2405844024167448PhytoremediationPetroleum productsInfrared spectrophotometryThermal analysisExtractionMiscanthus x giganteus
spellingShingle Ruslana Huminilovych
Vitalii Stadnik
Martyn Sozanskyi
Pavlo Shapoval
Valentina Pidlisnyuk
Ihor Poliuzhyn
Viktoriia Kochubei
Yurii Hrynchuk
Bohdan Korchak
Sample preparation method for IR analysis of petroleum-contaminated soil: An innovative technology for ecological remediation using Miscanthus x giganteus
Heliyon
Phytoremediation
Petroleum products
Infrared spectrophotometry
Thermal analysis
Extraction
Miscanthus x giganteus
title Sample preparation method for IR analysis of petroleum-contaminated soil: An innovative technology for ecological remediation using Miscanthus x giganteus
title_full Sample preparation method for IR analysis of petroleum-contaminated soil: An innovative technology for ecological remediation using Miscanthus x giganteus
title_fullStr Sample preparation method for IR analysis of petroleum-contaminated soil: An innovative technology for ecological remediation using Miscanthus x giganteus
title_full_unstemmed Sample preparation method for IR analysis of petroleum-contaminated soil: An innovative technology for ecological remediation using Miscanthus x giganteus
title_short Sample preparation method for IR analysis of petroleum-contaminated soil: An innovative technology for ecological remediation using Miscanthus x giganteus
title_sort sample preparation method for ir analysis of petroleum contaminated soil an innovative technology for ecological remediation using miscanthus x giganteus
topic Phytoremediation
Petroleum products
Infrared spectrophotometry
Thermal analysis
Extraction
Miscanthus x giganteus
url http://www.sciencedirect.com/science/article/pii/S2405844024167448
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