Phase hardening during cyclic quasi-martensitic transformations in ferroroactive solid solutions of the multicomponent system (Na, K)NbO3-PZT

Solid solutions (SS) with a quasi-binary cross-section of a four-component system of the composition [Formula: see text](Na[Formula: see text]K[Formula: see text])NbO3–xPb(Ti[Formula: see text]Zr[Formula: see text])O3, based on compositions with fundamentally different physical responses (Na, K)NbO3...

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Main Authors: Inna Andryushina, Konstantin Andryushin, Ekaterina Glazunova, Sidek Khasbulatov, Larisa Reznichenko
Format: Article
Language:English
Published: World Scientific Publishing 2025-06-01
Series:Journal of Advanced Dielectrics
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Online Access:https://www.worldscientific.com/doi/10.1142/S2010135X24500334
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author Inna Andryushina
Konstantin Andryushin
Ekaterina Glazunova
Sidek Khasbulatov
Larisa Reznichenko
author_facet Inna Andryushina
Konstantin Andryushin
Ekaterina Glazunova
Sidek Khasbulatov
Larisa Reznichenko
author_sort Inna Andryushina
collection DOAJ
description Solid solutions (SS) with a quasi-binary cross-section of a four-component system of the composition [Formula: see text](Na[Formula: see text]K[Formula: see text])NbO3–xPb(Ti[Formula: see text]Zr[Formula: see text])O3, based on compositions with fundamentally different physical responses (Na, K)NbO3 (KNN), Pb(Ti, Zr)O3 (PZT), have been prepared by a two-stage solid-phase synthesis followed by sintering using conventional ceramic technology. The influence of thermal cycling on the dielectric properties of ceramic SS with [Formula: see text] has been studied. It has been shown that thermally induced fatigue does not have a significant effect on the Curie temperature and the diffusing of the phase transition (PT) of SS containing only extreme components. It has been found that when the concentration of PZT in the studied system is varied, the [Formula: see text]/[Formula: see text] dependencies take on a form characteristic of ferroelectrics with a diffuse PT. When the repolarisation cycles are varied, the diffusing parameter and the Curie and Burns temperatures show a wave-like behavior. The observed effects are explained by the interaction of different defect types. A conclusion is drawn on the possible practical applications of the studied SS.
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publishDate 2025-06-01
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spelling doaj-art-ee5d782a4f084a13851342baf89afc112025-08-20T02:41:42ZengWorld Scientific PublishingJournal of Advanced Dielectrics2010-135X2010-13682025-06-01150310.1142/S2010135X24500334Phase hardening during cyclic quasi-martensitic transformations in ferroroactive solid solutions of the multicomponent system (Na, K)NbO3-PZTInna Andryushina0Konstantin Andryushin1Ekaterina Glazunova2Sidek Khasbulatov3Larisa Reznichenko4Research Institute of Physics, Southern Federal University, Stachki Str. 194, Rostov-on-Don, 344090, RussiaResearch Institute of Physics, Southern Federal University, Stachki Str. 194, Rostov-on-Don, 344090, RussiaResearch Institute of Physics, Southern Federal University, Stachki Str. 194, Rostov-on-Don, 344090, RussiaKh. Ibragimov Complex Institute of the Russian Academy of Sciences (CI RAS), V. Alieva 21a, Grozny, 364906, RussiaResearch Institute of Physics, Southern Federal University, Stachki Str. 194, Rostov-on-Don, 344090, RussiaSolid solutions (SS) with a quasi-binary cross-section of a four-component system of the composition [Formula: see text](Na[Formula: see text]K[Formula: see text])NbO3–xPb(Ti[Formula: see text]Zr[Formula: see text])O3, based on compositions with fundamentally different physical responses (Na, K)NbO3 (KNN), Pb(Ti, Zr)O3 (PZT), have been prepared by a two-stage solid-phase synthesis followed by sintering using conventional ceramic technology. The influence of thermal cycling on the dielectric properties of ceramic SS with [Formula: see text] has been studied. It has been shown that thermally induced fatigue does not have a significant effect on the Curie temperature and the diffusing of the phase transition (PT) of SS containing only extreme components. It has been found that when the concentration of PZT in the studied system is varied, the [Formula: see text]/[Formula: see text] dependencies take on a form characteristic of ferroelectrics with a diffuse PT. When the repolarisation cycles are varied, the diffusing parameter and the Curie and Burns temperatures show a wave-like behavior. The observed effects are explained by the interaction of different defect types. A conclusion is drawn on the possible practical applications of the studied SS.https://www.worldscientific.com/doi/10.1142/S2010135X24500334Solid solutionsPZTKNNthermal cyclingCurie–Weiss temperatureburns temperature
spellingShingle Inna Andryushina
Konstantin Andryushin
Ekaterina Glazunova
Sidek Khasbulatov
Larisa Reznichenko
Phase hardening during cyclic quasi-martensitic transformations in ferroroactive solid solutions of the multicomponent system (Na, K)NbO3-PZT
Journal of Advanced Dielectrics
Solid solutions
PZT
KNN
thermal cycling
Curie–Weiss temperature
burns temperature
title Phase hardening during cyclic quasi-martensitic transformations in ferroroactive solid solutions of the multicomponent system (Na, K)NbO3-PZT
title_full Phase hardening during cyclic quasi-martensitic transformations in ferroroactive solid solutions of the multicomponent system (Na, K)NbO3-PZT
title_fullStr Phase hardening during cyclic quasi-martensitic transformations in ferroroactive solid solutions of the multicomponent system (Na, K)NbO3-PZT
title_full_unstemmed Phase hardening during cyclic quasi-martensitic transformations in ferroroactive solid solutions of the multicomponent system (Na, K)NbO3-PZT
title_short Phase hardening during cyclic quasi-martensitic transformations in ferroroactive solid solutions of the multicomponent system (Na, K)NbO3-PZT
title_sort phase hardening during cyclic quasi martensitic transformations in ferroroactive solid solutions of the multicomponent system na k nbo3 pzt
topic Solid solutions
PZT
KNN
thermal cycling
Curie–Weiss temperature
burns temperature
url https://www.worldscientific.com/doi/10.1142/S2010135X24500334
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