Green synthesized zinc oxide nanoparticles with lemongrass essential oil for the development of an effective herbal mouthwash

Abstract Oral pathogens contribute to dental caries and other infections affecting oral health. To address concerns related to the adverse effects of chemical mouthwashes like chlorhexidine (CHX), this study introduces a novel herbal mouthwash formulated with green-synthesized zinc oxide nanoparticl...

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Main Authors: Preeti Pallavi, Pragnya Paramita Sahoo, Adyasha Anapurba Sahoo, Sudip kumar Sen, Sangeeta Raut
Format: Article
Language:English
Published: Nature Portfolio 2025-08-01
Series:Scientific Reports
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Online Access:https://doi.org/10.1038/s41598-025-16877-7
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author Preeti Pallavi
Pragnya Paramita Sahoo
Adyasha Anapurba Sahoo
Sudip kumar Sen
Sangeeta Raut
author_facet Preeti Pallavi
Pragnya Paramita Sahoo
Adyasha Anapurba Sahoo
Sudip kumar Sen
Sangeeta Raut
author_sort Preeti Pallavi
collection DOAJ
description Abstract Oral pathogens contribute to dental caries and other infections affecting oral health. To address concerns related to the adverse effects of chemical mouthwashes like chlorhexidine (CHX), this study introduces a novel herbal mouthwash formulated with green-synthesized zinc oxide nanoparticles (ZnONPs) infused with Cymbopogon citratus essential oil (CEO). Unlike traditional formulations, this herbal mouthwash aims to offer a safer, eco-friendly alternative. Four formulations (F1-F4) with varying concentrations of CEOZnONPs were evaluated for in vitro antibacterial and anti-biofilm activities against Streptococcus mutans, Staphylococcus aureus, and Escherichia coli. The F4 formulation demonstrated superior antibacterial efficacy, with inhibition zones of 64.2 ± 2.6 mm for S. mutans, 43.6 ± 1.0 mm for S. aureus, and 31.8 ± 1.5 mm for E. coli, and achieved 97.12% biofilm inhibition of S. mutans. Additionally, in vivo toxicity was assessed using embryonic zebrafish, showing a high survival rate of 93% for F1 and 82% for F4 after 24 hours, compared to 65% for CHX, indicating lower toxicity. This preclinical study shows that the F4 formulation exhibited promising antibacterial and safety profiles, highlighting its potential as a safe, natural oral care product targeting diverse oral pathogens with reduced toxicity. Further research, including in vivo and clinical trials, is needed to validate its effectiveness and safety for regular dental care use. The herbal mouthwash formulated with CEOZnONPs demonstrates strong antibacterial and anti-biofilm effects with lower toxicity, making it a promising natural alternative for oral hygiene. Its safer profile compared to CHX may reduce side effects in patients, potentially enhancing compliance in oral care regimens.
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spelling doaj-art-ec1bb15eb4a44547a7bf555f18db9dff2025-08-24T11:29:54ZengNature PortfolioScientific Reports2045-23222025-08-0115111010.1038/s41598-025-16877-7Green synthesized zinc oxide nanoparticles with lemongrass essential oil for the development of an effective herbal mouthwashPreeti Pallavi0Pragnya Paramita Sahoo1Adyasha Anapurba Sahoo2Sudip kumar Sen3Sangeeta Raut4School of Pharmaceutical Sciences, Centre for Biotechnology, Siksha ‘O’ Anusandhan (Deemed to be University)School of Pharmaceutical Sciences, Centre for Biotechnology, Siksha ‘O’ Anusandhan (Deemed to be University)School of Pharmaceutical Sciences, Centre for Biotechnology, Siksha ‘O’ Anusandhan (Deemed to be University)Coastal Aquaculture Research Institute Private LimitedSchool of Pharmaceutical Sciences, Centre for Biotechnology, Siksha ‘O’ Anusandhan (Deemed to be University)Abstract Oral pathogens contribute to dental caries and other infections affecting oral health. To address concerns related to the adverse effects of chemical mouthwashes like chlorhexidine (CHX), this study introduces a novel herbal mouthwash formulated with green-synthesized zinc oxide nanoparticles (ZnONPs) infused with Cymbopogon citratus essential oil (CEO). Unlike traditional formulations, this herbal mouthwash aims to offer a safer, eco-friendly alternative. Four formulations (F1-F4) with varying concentrations of CEOZnONPs were evaluated for in vitro antibacterial and anti-biofilm activities against Streptococcus mutans, Staphylococcus aureus, and Escherichia coli. The F4 formulation demonstrated superior antibacterial efficacy, with inhibition zones of 64.2 ± 2.6 mm for S. mutans, 43.6 ± 1.0 mm for S. aureus, and 31.8 ± 1.5 mm for E. coli, and achieved 97.12% biofilm inhibition of S. mutans. Additionally, in vivo toxicity was assessed using embryonic zebrafish, showing a high survival rate of 93% for F1 and 82% for F4 after 24 hours, compared to 65% for CHX, indicating lower toxicity. This preclinical study shows that the F4 formulation exhibited promising antibacterial and safety profiles, highlighting its potential as a safe, natural oral care product targeting diverse oral pathogens with reduced toxicity. Further research, including in vivo and clinical trials, is needed to validate its effectiveness and safety for regular dental care use. The herbal mouthwash formulated with CEOZnONPs demonstrates strong antibacterial and anti-biofilm effects with lower toxicity, making it a promising natural alternative for oral hygiene. Its safer profile compared to CHX may reduce side effects in patients, potentially enhancing compliance in oral care regimens.https://doi.org/10.1038/s41598-025-16877-7BiofilmCymbopogon citratusCytotoxicityDental cariesMouthwashZinc oxide
spellingShingle Preeti Pallavi
Pragnya Paramita Sahoo
Adyasha Anapurba Sahoo
Sudip kumar Sen
Sangeeta Raut
Green synthesized zinc oxide nanoparticles with lemongrass essential oil for the development of an effective herbal mouthwash
Scientific Reports
Biofilm
Cymbopogon citratus
Cytotoxicity
Dental caries
Mouthwash
Zinc oxide
title Green synthesized zinc oxide nanoparticles with lemongrass essential oil for the development of an effective herbal mouthwash
title_full Green synthesized zinc oxide nanoparticles with lemongrass essential oil for the development of an effective herbal mouthwash
title_fullStr Green synthesized zinc oxide nanoparticles with lemongrass essential oil for the development of an effective herbal mouthwash
title_full_unstemmed Green synthesized zinc oxide nanoparticles with lemongrass essential oil for the development of an effective herbal mouthwash
title_short Green synthesized zinc oxide nanoparticles with lemongrass essential oil for the development of an effective herbal mouthwash
title_sort green synthesized zinc oxide nanoparticles with lemongrass essential oil for the development of an effective herbal mouthwash
topic Biofilm
Cymbopogon citratus
Cytotoxicity
Dental caries
Mouthwash
Zinc oxide
url https://doi.org/10.1038/s41598-025-16877-7
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