Signature of magnetoelectric coupling driven finite momentum pairing in 3D ising superconductor

Abstract The finite momentum superconducting paring states (FMPs) represent a forefront of condensed matter physics. Here we report experimental evidence of FMP in a locally noncentrosymmetric bulk superconductor 4H b -TaS2. Using hard X-ray diffraction and angle-resolved photoemission spectroscopy,...

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Main Authors: F. Z. Yang, H. D. Zhang, Saswata Mandal, F. Y. Meng, G. Fabbris, A. H. Said, P. Mercado Lozano, A. Rajapitamahuni, E. Vescovo, C. Nelson, S. Lin, Y. Park, E. M. Clements, T. Z. Ward, H.-N. Lee, H. C. Lei, C. X. Liu, H. Miao
Format: Article
Language:English
Published: Nature Portfolio 2025-07-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-61882-z
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Summary:Abstract The finite momentum superconducting paring states (FMPs) represent a forefront of condensed matter physics. Here we report experimental evidence of FMP in a locally noncentrosymmetric bulk superconductor 4H b -TaS2. Using hard X-ray diffraction and angle-resolved photoemission spectroscopy, we reveal unusual 2D ferro-rotational charge density wave (CDW) and weak interlayer hopping in 4H b -TaS2. The superconducting upper critical field, H c2, linearly increases via decreasing temperature, and well exceeds the Pauli limit, suggesting the dominant orbital pair-breaking mechanism. Remarkably, we observed evidence of field-induced superconductivity-to-superconductivity transition that breaks continuous rotational symmetry of the s-wave uniform pairing in the Bardeen-Cooper-Schrieffer theory down to the six-fold rotation symmetry. Ginzburg-Landau free energy analysis shows that magnetoelectric coupling, induced by 2D ferro-rotational CDW, stabilizes FMP that provides an explanation of the lowering rotation symmetry. Our results provide a new understanding of unconventional superconducting behaviors of the bulk quantum heterostructure 4H b -TaS2.
ISSN:2041-1723