Enhanced methane generation using zeolitic imidazolate framework (ZIF-8) during biogas production

Abstract Metal–organic frameworks (MOFs) are increasingly being utilized in catalysis, fuel cells, and related fields due to their unique characteristics. This study explores the use of Zeolitic Imidazolate Framework-8 (ZIF-8) MOF during co-digestion of tuber and fruit waste to enhance biogas produc...

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Main Authors: Gracious Makuba, Idah Jim Calvin, Mercy Kiende, Martha N. Chollomo, Register Mrosso, Achisa C. Mecha
Format: Article
Language:English
Published: Springer 2025-04-01
Series:Discover Sustainability
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Online Access:https://doi.org/10.1007/s43621-025-00984-6
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author Gracious Makuba
Idah Jim Calvin
Mercy Kiende
Martha N. Chollomo
Register Mrosso
Achisa C. Mecha
author_facet Gracious Makuba
Idah Jim Calvin
Mercy Kiende
Martha N. Chollomo
Register Mrosso
Achisa C. Mecha
author_sort Gracious Makuba
collection DOAJ
description Abstract Metal–organic frameworks (MOFs) are increasingly being utilized in catalysis, fuel cells, and related fields due to their unique characteristics. This study explores the use of Zeolitic Imidazolate Framework-8 (ZIF-8) MOF during co-digestion of tuber and fruit waste to enhance biogas production and methane content. The ZIF-8 was synthesized and characterized using Fourier Transform Infra-Red spectroscopy, to confirm the presence of functional groups. The following properties of the feedstock and inoculum were evaluated: moisture content, volatile solids, total volatile solids, biodegradability index, total dissolved solids, pH, and electrical conductivity. The effect of solution pH and MOF mass was assessed. FTIR spectra were obtained with an FTIR spectrometer over a wavenumber range of 4500–500 cm⁻1. The pH values were near neutral, i.e., 6.9 (fruit waste), 6.7 (tuber waste), and 7.4 (inoculum). The biogas yield increased with ZIF-8 catalyst dosage, the highest biogas production of 1851 mL at ZIF-8 dosage of 0.5 g was attained which is twice as much as the control experiment (without ZIF-8) attained 914 mL. The use of ZIF-8 resulted in a 103% increase in biogas yield and showed that the application of ZIF-8 catalyzed the methanogenesis step resulting in increased yield and efficiency of the process.
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spelling doaj-art-eb8d51444eb847fa82bacf933bdc6b4a2025-08-20T02:17:53ZengSpringerDiscover Sustainability2662-99842025-04-016111010.1007/s43621-025-00984-6Enhanced methane generation using zeolitic imidazolate framework (ZIF-8) during biogas productionGracious Makuba0Idah Jim Calvin1Mercy Kiende2Martha N. Chollomo3Register Mrosso4Achisa C. Mecha5Renewable Energy, Environment, Nanomaterials, and Water Research Group, Department of Chemical and Process Engineering, Moi UniversityRenewable Energy, Environment, Nanomaterials, and Water Research Group, Department of Chemical and Process Engineering, Moi UniversityRenewable Energy, Environment, Nanomaterials, and Water Research Group, Department of Chemical and Process Engineering, Moi UniversityEnvironmental Pollution and Remediation Research Group, Department of Chemical Engineering, Mangosuthu University of TechnologyClean Energy Technologies Research Group, School of Materials, Energy, Water and Environmental Sciences (MEWES), Nelson Mandela African Institution of Science and Technology (NM-AIST)Renewable Energy, Environment, Nanomaterials, and Water Research Group, Department of Chemical and Process Engineering, Moi UniversityAbstract Metal–organic frameworks (MOFs) are increasingly being utilized in catalysis, fuel cells, and related fields due to their unique characteristics. This study explores the use of Zeolitic Imidazolate Framework-8 (ZIF-8) MOF during co-digestion of tuber and fruit waste to enhance biogas production and methane content. The ZIF-8 was synthesized and characterized using Fourier Transform Infra-Red spectroscopy, to confirm the presence of functional groups. The following properties of the feedstock and inoculum were evaluated: moisture content, volatile solids, total volatile solids, biodegradability index, total dissolved solids, pH, and electrical conductivity. The effect of solution pH and MOF mass was assessed. FTIR spectra were obtained with an FTIR spectrometer over a wavenumber range of 4500–500 cm⁻1. The pH values were near neutral, i.e., 6.9 (fruit waste), 6.7 (tuber waste), and 7.4 (inoculum). The biogas yield increased with ZIF-8 catalyst dosage, the highest biogas production of 1851 mL at ZIF-8 dosage of 0.5 g was attained which is twice as much as the control experiment (without ZIF-8) attained 914 mL. The use of ZIF-8 resulted in a 103% increase in biogas yield and showed that the application of ZIF-8 catalyzed the methanogenesis step resulting in increased yield and efficiency of the process.https://doi.org/10.1007/s43621-025-00984-6Metal–organic frameworkBiogasZIF-8Tuber wasteFruit waste
spellingShingle Gracious Makuba
Idah Jim Calvin
Mercy Kiende
Martha N. Chollomo
Register Mrosso
Achisa C. Mecha
Enhanced methane generation using zeolitic imidazolate framework (ZIF-8) during biogas production
Discover Sustainability
Metal–organic framework
Biogas
ZIF-8
Tuber waste
Fruit waste
title Enhanced methane generation using zeolitic imidazolate framework (ZIF-8) during biogas production
title_full Enhanced methane generation using zeolitic imidazolate framework (ZIF-8) during biogas production
title_fullStr Enhanced methane generation using zeolitic imidazolate framework (ZIF-8) during biogas production
title_full_unstemmed Enhanced methane generation using zeolitic imidazolate framework (ZIF-8) during biogas production
title_short Enhanced methane generation using zeolitic imidazolate framework (ZIF-8) during biogas production
title_sort enhanced methane generation using zeolitic imidazolate framework zif 8 during biogas production
topic Metal–organic framework
Biogas
ZIF-8
Tuber waste
Fruit waste
url https://doi.org/10.1007/s43621-025-00984-6
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