Pseudo bismuth vanadate anchored EDLC-MWCNTs: Supercapacitive electrode to a symmetric solid-state device

Sponge analogous nano pebbles of bismuth vanadate (BiVO4) decorated over multi-walled carbon nanotubes (MWCNTs) synthesized by the successive ionic layer adsorption and reaction (SILAR) method have been explored towards supercapacitor application through enhanced (8 times) surface roughness (Sa) com...

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Main Authors: Lakshmana Kumar Bommineedi, Tushar B. Deshmukh, Avinash C. Mendhe, Sachin R. Rondiya, Babasaheb R. Sankapal
Format: Article
Language:English
Published: Elsevier 2025-04-01
Series:Carbon Trends
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Online Access:http://www.sciencedirect.com/science/article/pii/S2667056925000252
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author Lakshmana Kumar Bommineedi
Tushar B. Deshmukh
Avinash C. Mendhe
Sachin R. Rondiya
Babasaheb R. Sankapal
author_facet Lakshmana Kumar Bommineedi
Tushar B. Deshmukh
Avinash C. Mendhe
Sachin R. Rondiya
Babasaheb R. Sankapal
author_sort Lakshmana Kumar Bommineedi
collection DOAJ
description Sponge analogous nano pebbles of bismuth vanadate (BiVO4) decorated over multi-walled carbon nanotubes (MWCNTs) synthesized by the successive ionic layer adsorption and reaction (SILAR) method have been explored towards supercapacitor application through enhanced (8 times) surface roughness (Sa) compared to bare MWCNTs; well supported by wettability studies. Electrochemical studies through CV, GCD, EIS, and electrochemical stability performances of the electrode have been performed in 1 M KCl electrolyte where MWCNTs/BiVO4 showed the highest capacitance (1334.66 F/g) at 3 mV/s with good electrochemical stability of 103 % even after 3500 CV cycles. Interestingly, symmetric solid-state supercapacitor assembled using PVA embedded LiClO4 gel exhibited a remarkable potential window of 1.83 V with corresponding energy and power densities of 18.38 Wh/kg and 2.13 kW/kg, respectively at 1 mA/cm2. The novelty of this work lies in the introduction of a symmetric device using MWCNTs/BiVO4 electrodes for the first time along with its potential for real-world use by illuminating ‘VNIT ‘acronym consisting of 21 red LEDs.
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publishDate 2025-04-01
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spelling doaj-art-eb0b7d34354c4c3486382d6ccb8da8c32025-08-20T02:12:07ZengElsevierCarbon Trends2667-05692025-04-011910047510.1016/j.cartre.2025.100475Pseudo bismuth vanadate anchored EDLC-MWCNTs: Supercapacitive electrode to a symmetric solid-state deviceLakshmana Kumar Bommineedi0Tushar B. Deshmukh1Avinash C. Mendhe2Sachin R. Rondiya3Babasaheb R. Sankapal4Nano Materials and Device Laboratory, Department of Physics, Visvesvaraya National Institute of Technology, South Ambazari Road, Nagpur 440010, Maharashtra, India; Malla Reddy Engineering College, Campus 1, Maisammaguda, post via Kompally, Rangareddy District, Secunderabad-500100, Telangana, IndiaNano Materials and Device Laboratory, Department of Physics, Visvesvaraya National Institute of Technology, South Ambazari Road, Nagpur 440010, Maharashtra, India; Entity 2 Energy Storage Private Limited, Tenneer Kuppam, Chennai, Tamil Nadu 600056, IndiaDepartment of Electronic Engineering, Institute for Wearable Convergence Electronics, Kyung Hee University, 1732 Deogyeong-daero, Giheung-gu, Yongin 17104, Republic of KoreaDepartment of Materials Engineering, Indian Institute of Science (IISc), Bengaluru, IndiaNano Materials and Device Laboratory, Department of Physics, Visvesvaraya National Institute of Technology, South Ambazari Road, Nagpur 440010, Maharashtra, India; Corresponding author.Sponge analogous nano pebbles of bismuth vanadate (BiVO4) decorated over multi-walled carbon nanotubes (MWCNTs) synthesized by the successive ionic layer adsorption and reaction (SILAR) method have been explored towards supercapacitor application through enhanced (8 times) surface roughness (Sa) compared to bare MWCNTs; well supported by wettability studies. Electrochemical studies through CV, GCD, EIS, and electrochemical stability performances of the electrode have been performed in 1 M KCl electrolyte where MWCNTs/BiVO4 showed the highest capacitance (1334.66 F/g) at 3 mV/s with good electrochemical stability of 103 % even after 3500 CV cycles. Interestingly, symmetric solid-state supercapacitor assembled using PVA embedded LiClO4 gel exhibited a remarkable potential window of 1.83 V with corresponding energy and power densities of 18.38 Wh/kg and 2.13 kW/kg, respectively at 1 mA/cm2. The novelty of this work lies in the introduction of a symmetric device using MWCNTs/BiVO4 electrodes for the first time along with its potential for real-world use by illuminating ‘VNIT ‘acronym consisting of 21 red LEDs.http://www.sciencedirect.com/science/article/pii/S2667056925000252SupercapacitorBiVO4NanopebblesSILARMWCNTs
spellingShingle Lakshmana Kumar Bommineedi
Tushar B. Deshmukh
Avinash C. Mendhe
Sachin R. Rondiya
Babasaheb R. Sankapal
Pseudo bismuth vanadate anchored EDLC-MWCNTs: Supercapacitive electrode to a symmetric solid-state device
Carbon Trends
Supercapacitor
BiVO4
Nanopebbles
SILAR
MWCNTs
title Pseudo bismuth vanadate anchored EDLC-MWCNTs: Supercapacitive electrode to a symmetric solid-state device
title_full Pseudo bismuth vanadate anchored EDLC-MWCNTs: Supercapacitive electrode to a symmetric solid-state device
title_fullStr Pseudo bismuth vanadate anchored EDLC-MWCNTs: Supercapacitive electrode to a symmetric solid-state device
title_full_unstemmed Pseudo bismuth vanadate anchored EDLC-MWCNTs: Supercapacitive electrode to a symmetric solid-state device
title_short Pseudo bismuth vanadate anchored EDLC-MWCNTs: Supercapacitive electrode to a symmetric solid-state device
title_sort pseudo bismuth vanadate anchored edlc mwcnts supercapacitive electrode to a symmetric solid state device
topic Supercapacitor
BiVO4
Nanopebbles
SILAR
MWCNTs
url http://www.sciencedirect.com/science/article/pii/S2667056925000252
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