Study of Purified Cellulosic Pulp and Lignin Produced by Wheat Straw Biorefinery

With the world population rising, wheat straw production is expected to reach 687–740 million tons per year by 2050. Its frequent application as a fuel source leads to air, water, and soil pollution. Limited literature exists on methods for separating components of residual wheat straw. Optimal cond...

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Main Authors: Kalvin Durand, Rodrigue Daassi, Denis Rodrigue, Tatjana Stevanovic
Format: Article
Language:English
Published: MDPI AG 2024-09-01
Series:Macromol
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Online Access:https://www.mdpi.com/2673-6209/4/3/39
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author Kalvin Durand
Rodrigue Daassi
Denis Rodrigue
Tatjana Stevanovic
author_facet Kalvin Durand
Rodrigue Daassi
Denis Rodrigue
Tatjana Stevanovic
author_sort Kalvin Durand
collection DOAJ
description With the world population rising, wheat straw production is expected to reach 687–740 million tons per year by 2050. Its frequent application as a fuel source leads to air, water, and soil pollution. Limited literature exists on methods for separating components of residual wheat straw. Optimal conditions for organosolv pulping of hydrolyzed wheat straw include 3% FeCl<sub>3</sub>·6H<sub>2</sub>O as a catalyst, a biomass-to-solvent ratio of 1:15 (<i>m</i>/<i>v</i>), and 50% ethanol:water as cooking liquor at 200 °C for 30 min. Desilication conditions involve extraction with 7.5% Na<sub>2</sub>CO<sub>3</sub> at a biomass-to-solvent ratio of 1:20 (<i>m</i>/<i>v</i>) treated at 115 °C for 60 min. Lignin from hydrolyzed wheat straw showed similar properties to organosolv lignin from untreated straw, with minimal lignin alteration during hydrolysis. Hydrolysis significantly degraded cellulose. A 41% lignin recovery rate with 95% purity was achieved from pre-extracted hydrolyzed straw. Recovered cellulose after silica removal had 2% ash and 87% purity. The innovation of this process lies in the development of a comprehensive, sustainable, efficient, and economically viable biorefinery process that efficiently separates key components of wheat straw, i.e., xylose, lignin, cellulose, and silica, while addressing environmental pollution associated with its traditional use as fuel.
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spelling doaj-art-eab6d59c40f042feaa7bf3396439a2152025-08-20T01:55:38ZengMDPI AGMacromol2673-62092024-09-014365067910.3390/macromol4030039Study of Purified Cellulosic Pulp and Lignin Produced by Wheat Straw BiorefineryKalvin Durand0Rodrigue Daassi1Denis Rodrigue2Tatjana Stevanovic3Wood and Forest Science Department, Laval University, Quebec, QC G1V 0A6, CanadaBioproducts Development Center, Biopterre, La Pocatière, QC G0R 1Z0, CanadaChemical Engineering Department, Laval University, Quebec, QC G1V 0A6, CanadaWood and Forest Science Department, Laval University, Quebec, QC G1V 0A6, CanadaWith the world population rising, wheat straw production is expected to reach 687–740 million tons per year by 2050. Its frequent application as a fuel source leads to air, water, and soil pollution. Limited literature exists on methods for separating components of residual wheat straw. Optimal conditions for organosolv pulping of hydrolyzed wheat straw include 3% FeCl<sub>3</sub>·6H<sub>2</sub>O as a catalyst, a biomass-to-solvent ratio of 1:15 (<i>m</i>/<i>v</i>), and 50% ethanol:water as cooking liquor at 200 °C for 30 min. Desilication conditions involve extraction with 7.5% Na<sub>2</sub>CO<sub>3</sub> at a biomass-to-solvent ratio of 1:20 (<i>m</i>/<i>v</i>) treated at 115 °C for 60 min. Lignin from hydrolyzed wheat straw showed similar properties to organosolv lignin from untreated straw, with minimal lignin alteration during hydrolysis. Hydrolysis significantly degraded cellulose. A 41% lignin recovery rate with 95% purity was achieved from pre-extracted hydrolyzed straw. Recovered cellulose after silica removal had 2% ash and 87% purity. The innovation of this process lies in the development of a comprehensive, sustainable, efficient, and economically viable biorefinery process that efficiently separates key components of wheat straw, i.e., xylose, lignin, cellulose, and silica, while addressing environmental pollution associated with its traditional use as fuel.https://www.mdpi.com/2673-6209/4/3/39wheat strawlignincellulosesilicahydrolysisorganosolv pulping
spellingShingle Kalvin Durand
Rodrigue Daassi
Denis Rodrigue
Tatjana Stevanovic
Study of Purified Cellulosic Pulp and Lignin Produced by Wheat Straw Biorefinery
Macromol
wheat straw
lignin
cellulose
silica
hydrolysis
organosolv pulping
title Study of Purified Cellulosic Pulp and Lignin Produced by Wheat Straw Biorefinery
title_full Study of Purified Cellulosic Pulp and Lignin Produced by Wheat Straw Biorefinery
title_fullStr Study of Purified Cellulosic Pulp and Lignin Produced by Wheat Straw Biorefinery
title_full_unstemmed Study of Purified Cellulosic Pulp and Lignin Produced by Wheat Straw Biorefinery
title_short Study of Purified Cellulosic Pulp and Lignin Produced by Wheat Straw Biorefinery
title_sort study of purified cellulosic pulp and lignin produced by wheat straw biorefinery
topic wheat straw
lignin
cellulose
silica
hydrolysis
organosolv pulping
url https://www.mdpi.com/2673-6209/4/3/39
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AT denisrodrigue studyofpurifiedcellulosicpulpandligninproducedbywheatstrawbiorefinery
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