Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian Arctic
<p>The aerosol particles serving as cloud condensation and ice nuclei contribute to key cloud processes associated with cold-air outbreak (CAO) events but are poorly constrained in climate models due to sparse observations. Here we retrieve aerosol number size distribution modes from measureme...
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Copernicus Publications
2024-10-01
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| Series: | Atmospheric Chemistry and Physics |
| Online Access: | https://acp.copernicus.org/articles/24/11791/2024/acp-24-11791-2024.pdf |
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| author | A. S. Williams J. L. Dedrick L. M. Russell F. Tornow F. Tornow I. Silber I. Silber A. M. Fridlind B. Swanson P. J. DeMott P. Zieger P. Zieger R. Krejci R. Krejci |
| author_facet | A. S. Williams J. L. Dedrick L. M. Russell F. Tornow F. Tornow I. Silber I. Silber A. M. Fridlind B. Swanson P. J. DeMott P. Zieger P. Zieger R. Krejci R. Krejci |
| author_sort | A. S. Williams |
| collection | DOAJ |
| description | <p>The aerosol particles serving as cloud condensation and ice nuclei contribute to key cloud processes associated with cold-air outbreak (CAO) events but are poorly constrained in climate models due to sparse observations. Here we retrieve aerosol number size distribution modes from measurements at Andenes, Norway, during the Cold-Air Outbreaks in the Marine Boundary Layer Experiment (COMBLE) and at Zeppelin Observatory, approximately 1000 km upwind from Andenes at Svalbard. During CAO events at Andenes, the sea-spray-mode number concentration is correlated with strong over-ocean winds with a mean of <span class="inline-formula">8±4</span> cm<span class="inline-formula"><sup>−3</sup></span> that is 71 % higher than during non-CAO conditions. Additionally, during CAO events at Andenes, the mean Hoppel minimum diameter is 6 nm smaller than during non-CAO conditions, though the estimated supersaturation is lower, and the mean number concentration of particles that likely activated in-cloud is <span class="inline-formula">109±61</span> cm<span class="inline-formula"><sup>−3</sup></span> with no statistically significant difference from the non-CAO mean of <span class="inline-formula">99±66</span> cm<span class="inline-formula"><sup>−3</sup></span>. For CAO trajectories between Zeppelin Observatory and Andenes, the upwind-to-downwind change in number concentration is the largest for the accumulation mode with a mean decrease of <span class="inline-formula">93±95</span> cm<span class="inline-formula"><sup>−3</sup></span>, likely attributable primarily to precipitation scavenging. These characteristic properties of aerosol number size distributions during CAO events provide guidance for evaluating CAO aerosol–cloud interaction processes in models.</p> |
| format | Article |
| id | doaj-art-e9b6cc6bad26455fbf897945972c8e53 |
| institution | OA Journals |
| issn | 1680-7316 1680-7324 |
| language | English |
| publishDate | 2024-10-01 |
| publisher | Copernicus Publications |
| record_format | Article |
| series | Atmospheric Chemistry and Physics |
| spelling | doaj-art-e9b6cc6bad26455fbf897945972c8e532025-08-20T02:10:20ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242024-10-0124117911180510.5194/acp-24-11791-2024Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian ArcticA. S. Williams0J. L. Dedrick1L. M. Russell2F. Tornow3F. Tornow4I. Silber5I. Silber6A. M. Fridlind7B. Swanson8P. J. DeMott9P. Zieger10P. Zieger11R. Krejci12R. Krejci13Scripps Institution of Oceanography, University of California San Diego, La Jolla, CA, USAScripps Institution of Oceanography, University of California San Diego, La Jolla, CA, USAScripps Institution of Oceanography, University of California San Diego, La Jolla, CA, USACenter for Climate Systems Research, Columbia University, New York, NY, USANASA Goddard Institute for Space Studies, New York, NY, USADepartment of Meteorology and Atmospheric Science, Pennsylvania State University, University Park, PA, USAnow at: Atmospheric, Climate, and Earth Sciences Division, Pacific Northwest National Laboratory, Richland, WA, USANASA Goddard Institute for Space Studies, New York, NY, USADepartment of Atmospheric Science, Colorado State University, Fort Collins, CO, USADepartment of Atmospheric Science, Colorado State University, Fort Collins, CO, USADepartment of Environmental Science, Stockholm University, Stockholm, SwedenBolin Centre for Climate Research, Stockholm University, Stockholm, SwedenDepartment of Environmental Science, Stockholm University, Stockholm, SwedenBolin Centre for Climate Research, Stockholm University, Stockholm, Sweden<p>The aerosol particles serving as cloud condensation and ice nuclei contribute to key cloud processes associated with cold-air outbreak (CAO) events but are poorly constrained in climate models due to sparse observations. Here we retrieve aerosol number size distribution modes from measurements at Andenes, Norway, during the Cold-Air Outbreaks in the Marine Boundary Layer Experiment (COMBLE) and at Zeppelin Observatory, approximately 1000 km upwind from Andenes at Svalbard. During CAO events at Andenes, the sea-spray-mode number concentration is correlated with strong over-ocean winds with a mean of <span class="inline-formula">8±4</span> cm<span class="inline-formula"><sup>−3</sup></span> that is 71 % higher than during non-CAO conditions. Additionally, during CAO events at Andenes, the mean Hoppel minimum diameter is 6 nm smaller than during non-CAO conditions, though the estimated supersaturation is lower, and the mean number concentration of particles that likely activated in-cloud is <span class="inline-formula">109±61</span> cm<span class="inline-formula"><sup>−3</sup></span> with no statistically significant difference from the non-CAO mean of <span class="inline-formula">99±66</span> cm<span class="inline-formula"><sup>−3</sup></span>. For CAO trajectories between Zeppelin Observatory and Andenes, the upwind-to-downwind change in number concentration is the largest for the accumulation mode with a mean decrease of <span class="inline-formula">93±95</span> cm<span class="inline-formula"><sup>−3</sup></span>, likely attributable primarily to precipitation scavenging. These characteristic properties of aerosol number size distributions during CAO events provide guidance for evaluating CAO aerosol–cloud interaction processes in models.</p>https://acp.copernicus.org/articles/24/11791/2024/acp-24-11791-2024.pdf |
| spellingShingle | A. S. Williams J. L. Dedrick L. M. Russell F. Tornow F. Tornow I. Silber I. Silber A. M. Fridlind B. Swanson P. J. DeMott P. Zieger P. Zieger R. Krejci R. Krejci Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian Arctic Atmospheric Chemistry and Physics |
| title | Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian Arctic |
| title_full | Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian Arctic |
| title_fullStr | Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian Arctic |
| title_full_unstemmed | Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian Arctic |
| title_short | Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian Arctic |
| title_sort | aerosol size distribution properties associated with cold air outbreaks in the norwegian arctic |
| url | https://acp.copernicus.org/articles/24/11791/2024/acp-24-11791-2024.pdf |
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