Tensile mechanical response of polyethylene – clay nanocomposites.

In this work we report on the microstructural and the mechanical characteristics of high density polyethylene (HDPE)-clay nanocomposites, with particular attention to the creep behaviour. The samples were prepared through melt compounding, using two high-density polyethylenes with different melt flo...

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Format: Article
Language:English
Published: Budapest University of Technology and Economics 2007-03-01
Series:eXPRESS Polymer Letters
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Online Access:http://www.expresspolymlett.com/letolt.php?file=EPL-0000102&mi=cd
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collection DOAJ
description In this work we report on the microstructural and the mechanical characteristics of high density polyethylene (HDPE)-clay nanocomposites, with particular attention to the creep behaviour. The samples were prepared through melt compounding, using two high-density polyethylenes with different melt flow rate (MFR), two different organo-modified clays, and changing the relative amount of a polyethylene grafted with maleic anhydride (PEgMA) compatibilizer. The intercalation process is more effective as the matrix melt viscosity decreases (higher MFR), while the clay interlamellar spacing increases as the compatibilizer amount increases. The relative stiffness of the nanocomposites increases with the addition of clay, with a limited enhancement of the relative yield stress. The better intercalation obtained by the addition of the compatibilizer is not accompanied by a concurrent improvement of the tensile mechanical properties. The creep resistance is enhanced by the introduction of clay, with an appreciable dependence on both the polyethylene and the clay type.
format Article
id doaj-art-e8ddcbe9082f4df0978685636ca245a8
institution Kabale University
issn 1788-618X
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publishDate 2007-03-01
publisher Budapest University of Technology and Economics
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series eXPRESS Polymer Letters
spelling doaj-art-e8ddcbe9082f4df0978685636ca245a82025-08-20T03:39:18ZengBudapest University of Technology and EconomicseXPRESS Polymer Letters1788-618X2007-03-011312313110.3144/expresspolymlett.2007.21Tensile mechanical response of polyethylene – clay nanocomposites.In this work we report on the microstructural and the mechanical characteristics of high density polyethylene (HDPE)-clay nanocomposites, with particular attention to the creep behaviour. The samples were prepared through melt compounding, using two high-density polyethylenes with different melt flow rate (MFR), two different organo-modified clays, and changing the relative amount of a polyethylene grafted with maleic anhydride (PEgMA) compatibilizer. The intercalation process is more effective as the matrix melt viscosity decreases (higher MFR), while the clay interlamellar spacing increases as the compatibilizer amount increases. The relative stiffness of the nanocomposites increases with the addition of clay, with a limited enhancement of the relative yield stress. The better intercalation obtained by the addition of the compatibilizer is not accompanied by a concurrent improvement of the tensile mechanical properties. The creep resistance is enhanced by the introduction of clay, with an appreciable dependence on both the polyethylene and the clay type.http://www.expresspolymlett.com/letolt.php?file=EPL-0000102&mi=cdNanomaterialspolyethyleneclaypolymer nanocompositescreep
spellingShingle Tensile mechanical response of polyethylene – clay nanocomposites.
eXPRESS Polymer Letters
Nanomaterials
polyethylene
clay
polymer nanocomposites
creep
title Tensile mechanical response of polyethylene – clay nanocomposites.
title_full Tensile mechanical response of polyethylene – clay nanocomposites.
title_fullStr Tensile mechanical response of polyethylene – clay nanocomposites.
title_full_unstemmed Tensile mechanical response of polyethylene – clay nanocomposites.
title_short Tensile mechanical response of polyethylene – clay nanocomposites.
title_sort tensile mechanical response of polyethylene clay nanocomposites
topic Nanomaterials
polyethylene
clay
polymer nanocomposites
creep
url http://www.expresspolymlett.com/letolt.php?file=EPL-0000102&mi=cd