Enhancing electromechanical performance of extruded piezoresistive strain sensors: Study of TPU shore hardness effects

Flexible strain sensors based on conductive thermoplastic elastomer composites have garnered significant attention for wearable electronics and soft robotics applications. Among the various material combinations, thermoplastic polyurethane (TPU) and multi-walled carbon nanotubes (MWCNTs) have emerge...

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Main Authors: Imen Ayedi, Slim Naifar, Rajarajan Ramalingame, Mario Scholze, Martin Wagner, Olfa Kanoun
Format: Article
Language:English
Published: Elsevier 2025-07-01
Series:Journal of Materials Research and Technology
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Online Access:http://www.sciencedirect.com/science/article/pii/S2238785425015029
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author Imen Ayedi
Slim Naifar
Rajarajan Ramalingame
Mario Scholze
Martin Wagner
Olfa Kanoun
author_facet Imen Ayedi
Slim Naifar
Rajarajan Ramalingame
Mario Scholze
Martin Wagner
Olfa Kanoun
author_sort Imen Ayedi
collection DOAJ
description Flexible strain sensors based on conductive thermoplastic elastomer composites have garnered significant attention for wearable electronics and soft robotics applications. Among the various material combinations, thermoplastic polyurethane (TPU) and multi-walled carbon nanotubes (MWCNTs) have emerged as promising candidates due to their processability and electromechanical properties. However, achieving the desired properties of these strain sensors requires careful selection of materials and meeting specific criteria. In this context, filament strain sensors have been developed by investigating different types of TPU with varying Shore hardnesses from 37 to 71, combined with MWCNTs as a conductive filler through an extrusion process. The fabrication process and characterization techniques are reported, guiding material selection when combining a TPU with a piezoresistive filler to create a soft, stretchable sensor. Characterization of the filament sensors by dynamic tensile testing shows that the sensors have a good piezoresistive response and can detect deformation accurately. Critical parameters such as drift, relaxation behavior, hysteresis and lifetime have extensively evaluated. It has seen that higher Shore hardness decreased the elongation at the point of fracture. In quasi-static cycle testing, Harder TPUs exhibited lower relaxation (4.34) and lower drift (3.72).
format Article
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issn 2238-7854
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publishDate 2025-07-01
publisher Elsevier
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spelling doaj-art-e85a8039feba46038d1a30d1155574be2025-08-20T03:15:22ZengElsevierJournal of Materials Research and Technology2238-78542025-07-01373142315410.1016/j.jmrt.2025.06.080Enhancing electromechanical performance of extruded piezoresistive strain sensors: Study of TPU shore hardness effectsImen Ayedi0Slim Naifar1Rajarajan Ramalingame2Mario Scholze3Martin Wagner4Olfa Kanoun5Professorship Measurement and Sensor Technology, Chemnitz University of Technology, Chemnitz, 09126, Germany; Corresponding author.Laboratory of Electromechanical Systems (LASEM), National School of Engineers of Sfax, Sfax, 3038, Tunisia; Higher Institute of Applied Sciences and Technology of Gabes, University of Gabes, Gabes, 6072, TunisiaProfessorship Measurement and Sensor Technology, Chemnitz University of Technology, Chemnitz, 09126, GermanyInstitute of Materials Science and Engineering, Chemnitz University of Technology, Chemnitz, 09126, GermanyInstitute of Materials Science and Engineering, Chemnitz University of Technology, Chemnitz, 09126, GermanyProfessorship Measurement and Sensor Technology, Chemnitz University of Technology, Chemnitz, 09126, GermanyFlexible strain sensors based on conductive thermoplastic elastomer composites have garnered significant attention for wearable electronics and soft robotics applications. Among the various material combinations, thermoplastic polyurethane (TPU) and multi-walled carbon nanotubes (MWCNTs) have emerged as promising candidates due to their processability and electromechanical properties. However, achieving the desired properties of these strain sensors requires careful selection of materials and meeting specific criteria. In this context, filament strain sensors have been developed by investigating different types of TPU with varying Shore hardnesses from 37 to 71, combined with MWCNTs as a conductive filler through an extrusion process. The fabrication process and characterization techniques are reported, guiding material selection when combining a TPU with a piezoresistive filler to create a soft, stretchable sensor. Characterization of the filament sensors by dynamic tensile testing shows that the sensors have a good piezoresistive response and can detect deformation accurately. Critical parameters such as drift, relaxation behavior, hysteresis and lifetime have extensively evaluated. It has seen that higher Shore hardness decreased the elongation at the point of fracture. In quasi-static cycle testing, Harder TPUs exhibited lower relaxation (4.34) and lower drift (3.72).http://www.sciencedirect.com/science/article/pii/S2238785425015029Thermoplastic polyurethaneCarbon nanotubePolymer nanocompositeExtrusionFilament sensorFlexible strain sensor
spellingShingle Imen Ayedi
Slim Naifar
Rajarajan Ramalingame
Mario Scholze
Martin Wagner
Olfa Kanoun
Enhancing electromechanical performance of extruded piezoresistive strain sensors: Study of TPU shore hardness effects
Journal of Materials Research and Technology
Thermoplastic polyurethane
Carbon nanotube
Polymer nanocomposite
Extrusion
Filament sensor
Flexible strain sensor
title Enhancing electromechanical performance of extruded piezoresistive strain sensors: Study of TPU shore hardness effects
title_full Enhancing electromechanical performance of extruded piezoresistive strain sensors: Study of TPU shore hardness effects
title_fullStr Enhancing electromechanical performance of extruded piezoresistive strain sensors: Study of TPU shore hardness effects
title_full_unstemmed Enhancing electromechanical performance of extruded piezoresistive strain sensors: Study of TPU shore hardness effects
title_short Enhancing electromechanical performance of extruded piezoresistive strain sensors: Study of TPU shore hardness effects
title_sort enhancing electromechanical performance of extruded piezoresistive strain sensors study of tpu shore hardness effects
topic Thermoplastic polyurethane
Carbon nanotube
Polymer nanocomposite
Extrusion
Filament sensor
Flexible strain sensor
url http://www.sciencedirect.com/science/article/pii/S2238785425015029
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