Hydrogel-Based Biointerfaces: Recent Advances, Challenges, and Future Directions in Human–Machine Integration

Human–machine interfacing (HMI) has emerged as a critical technology in healthcare, robotics, and wearable electronics, with hydrogels offering unique advantages as multifunctional materials that seamlessly connect biological systems with electronic devices. This review provides a detailed examinati...

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Main Authors: Aziz Ullah, Do Youn Kim, Sung In Lim, Hyo-Ryoung Lim
Format: Article
Language:English
Published: MDPI AG 2025-03-01
Series:Gels
Subjects:
Online Access:https://www.mdpi.com/2310-2861/11/4/232
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author Aziz Ullah
Do Youn Kim
Sung In Lim
Hyo-Ryoung Lim
author_facet Aziz Ullah
Do Youn Kim
Sung In Lim
Hyo-Ryoung Lim
author_sort Aziz Ullah
collection DOAJ
description Human–machine interfacing (HMI) has emerged as a critical technology in healthcare, robotics, and wearable electronics, with hydrogels offering unique advantages as multifunctional materials that seamlessly connect biological systems with electronic devices. This review provides a detailed examination of recent advancements in hydrogel design, focusing on their properties and potential applications in HMI. We explore the key characteristics such as biocompatibility, mechanical flexibility, and responsiveness, which are essential for effective and long-term integration with biological tissues. Additionally, we highlight innovations in conductive hydrogels, hybrid and composite materials, and fabrication techniques such as 3D/4D printing, which allow for the customization of hydrogel properties to meet the demands of specific HMI applications. Further, we discuss the diverse classes of polymers that contribute to hydrogel conductivity, including conducting, natural, synthetic, and hybrid polymers, emphasizing their role in enhancing electrical performance and mechanical adaptability. In addition to material design, we examine the regulatory landscape governing hydrogel-based biointerfaces for HMI applications, addressing the key considerations for clinical translation and commercialization. An analysis of the patent landscape provides insights into emerging trends and innovations shaping the future of hydrogel technologies in human–machine interactions. The review also covers a range of applications, including wearable electronics, neural interfaces, soft robotics, and haptic systems, where hydrogels play a transformative role in enhancing human–machine interactions. Thereafter, the review addresses the challenges hydrogels face in HMI applications, including issues related to stability, biocompatibility, and scalability, while offering future perspectives on the continued evolution of hydrogel-based systems for HMI technologies.
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spelling doaj-art-e7a19ed22e4a4f1bbd3cf2ae231411a32025-08-20T03:13:47ZengMDPI AGGels2310-28612025-03-0111423210.3390/gels11040232Hydrogel-Based Biointerfaces: Recent Advances, Challenges, and Future Directions in Human–Machine IntegrationAziz Ullah0Do Youn Kim1Sung In Lim2Hyo-Ryoung Lim3Major of Human Bioconvergence, Division of Smart Healthcare, College of Information Technology and Convergence, Pukyong National University, Busan 48513, Republic of KoreaMajor of Human Bioconvergence, Division of Smart Healthcare, College of Information Technology and Convergence, Pukyong National University, Busan 48513, Republic of KoreaDepartment of Chemical Engineering, Pukyong National University, Busan 48513, Republic of KoreaMajor of Human Bioconvergence, Division of Smart Healthcare, College of Information Technology and Convergence, Pukyong National University, Busan 48513, Republic of KoreaHuman–machine interfacing (HMI) has emerged as a critical technology in healthcare, robotics, and wearable electronics, with hydrogels offering unique advantages as multifunctional materials that seamlessly connect biological systems with electronic devices. This review provides a detailed examination of recent advancements in hydrogel design, focusing on their properties and potential applications in HMI. We explore the key characteristics such as biocompatibility, mechanical flexibility, and responsiveness, which are essential for effective and long-term integration with biological tissues. Additionally, we highlight innovations in conductive hydrogels, hybrid and composite materials, and fabrication techniques such as 3D/4D printing, which allow for the customization of hydrogel properties to meet the demands of specific HMI applications. Further, we discuss the diverse classes of polymers that contribute to hydrogel conductivity, including conducting, natural, synthetic, and hybrid polymers, emphasizing their role in enhancing electrical performance and mechanical adaptability. In addition to material design, we examine the regulatory landscape governing hydrogel-based biointerfaces for HMI applications, addressing the key considerations for clinical translation and commercialization. An analysis of the patent landscape provides insights into emerging trends and innovations shaping the future of hydrogel technologies in human–machine interactions. The review also covers a range of applications, including wearable electronics, neural interfaces, soft robotics, and haptic systems, where hydrogels play a transformative role in enhancing human–machine interactions. Thereafter, the review addresses the challenges hydrogels face in HMI applications, including issues related to stability, biocompatibility, and scalability, while offering future perspectives on the continued evolution of hydrogel-based systems for HMI technologies.https://www.mdpi.com/2310-2861/11/4/232human–machine interfacinghydrogelsbiocompatible materialswearable electronicsconductive hydrogelsneural interfaces
spellingShingle Aziz Ullah
Do Youn Kim
Sung In Lim
Hyo-Ryoung Lim
Hydrogel-Based Biointerfaces: Recent Advances, Challenges, and Future Directions in Human–Machine Integration
Gels
human–machine interfacing
hydrogels
biocompatible materials
wearable electronics
conductive hydrogels
neural interfaces
title Hydrogel-Based Biointerfaces: Recent Advances, Challenges, and Future Directions in Human–Machine Integration
title_full Hydrogel-Based Biointerfaces: Recent Advances, Challenges, and Future Directions in Human–Machine Integration
title_fullStr Hydrogel-Based Biointerfaces: Recent Advances, Challenges, and Future Directions in Human–Machine Integration
title_full_unstemmed Hydrogel-Based Biointerfaces: Recent Advances, Challenges, and Future Directions in Human–Machine Integration
title_short Hydrogel-Based Biointerfaces: Recent Advances, Challenges, and Future Directions in Human–Machine Integration
title_sort hydrogel based biointerfaces recent advances challenges and future directions in human machine integration
topic human–machine interfacing
hydrogels
biocompatible materials
wearable electronics
conductive hydrogels
neural interfaces
url https://www.mdpi.com/2310-2861/11/4/232
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AT doyounkim hydrogelbasedbiointerfacesrecentadvanceschallengesandfuturedirectionsinhumanmachineintegration
AT sunginlim hydrogelbasedbiointerfacesrecentadvanceschallengesandfuturedirectionsinhumanmachineintegration
AT hyoryounglim hydrogelbasedbiointerfacesrecentadvanceschallengesandfuturedirectionsinhumanmachineintegration