Desorption of Cadmium from Cocoa Waste Using Organic Acids

This study evaluated the desorption of cadmium (Cd) from cocoa waste-derived flour using organic acids. Cocoa pods were collected from Antioquia and Casanare, Colombia, to analyze the geographical Cd content and its distribution within the pod tissues. Acid selection was performed using a multi-crit...

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Main Authors: Sebastián Piedrahíta-Pérez, Juliana Rodríguez-Estrada, Margarita Ramírez-Carmona, Leidy Rendón-Castrillón, Carlos Ocampo-López
Format: Article
Language:English
Published: MDPI AG 2024-12-01
Series:Foods
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Online Access:https://www.mdpi.com/2304-8158/13/24/4048
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author Sebastián Piedrahíta-Pérez
Juliana Rodríguez-Estrada
Margarita Ramírez-Carmona
Leidy Rendón-Castrillón
Carlos Ocampo-López
author_facet Sebastián Piedrahíta-Pérez
Juliana Rodríguez-Estrada
Margarita Ramírez-Carmona
Leidy Rendón-Castrillón
Carlos Ocampo-López
author_sort Sebastián Piedrahíta-Pérez
collection DOAJ
description This study evaluated the desorption of cadmium (Cd) from cocoa waste-derived flour using organic acids. Cocoa pods were collected from Antioquia and Casanare, Colombia, to analyze the geographical Cd content and its distribution within the pod tissues. Acid selection was performed using a multi-criteria decision-making (MCDM) matrix, and Cd desorption was assessed through a full factorial 2<sup>3</sup> experimental design, considering acid concentration, pulp density, and agitation speed. Additionally, the oxidation–reduction potential (ORP) was monitored as an indicator of the electrochemical dynamics of the process. The results indicated that pods from Casanare exhibited higher Cd concentrations (1.63 ± 0.20 ppm) compared with those from Antioquia (0.87 ± 0.22 ppm), with 49.31% of the metal being accumulated in the pod. Parameters of citric acid at 0.5 M, 5 g/L pulp density, and 120 rpm were found to be optimal for the Cd desorption process, achieving over 95% efficiency. Based on ORP monitoring, a heuristic was proposed to determine the contact time during leaching. This work outlines a scalable process for Cd desorption, adding value to cocoa industry waste for potential applications.
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publishDate 2024-12-01
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spelling doaj-art-e7197eeb15e445cba253989fa53c406f2025-08-20T02:00:46ZengMDPI AGFoods2304-81582024-12-011324404810.3390/foods13244048Desorption of Cadmium from Cocoa Waste Using Organic AcidsSebastián Piedrahíta-Pérez0Juliana Rodríguez-Estrada1Margarita Ramírez-Carmona2Leidy Rendón-Castrillón3Carlos Ocampo-López4Chemical Engineering Faculty, Centro de Estudios y de Investigación en Biotecnología (CIBIOT), Universidad Pontificia Bolivariana, Medellín 050031, ColombiaChemical Engineering Faculty, Centro de Estudios y de Investigación en Biotecnología (CIBIOT), Universidad Pontificia Bolivariana, Medellín 050031, ColombiaChemical Engineering Faculty, Centro de Estudios y de Investigación en Biotecnología (CIBIOT), Universidad Pontificia Bolivariana, Medellín 050031, ColombiaChemical Engineering Faculty, Centro de Estudios y de Investigación en Biotecnología (CIBIOT), Universidad Pontificia Bolivariana, Medellín 050031, ColombiaChemical Engineering Faculty, Centro de Estudios y de Investigación en Biotecnología (CIBIOT), Universidad Pontificia Bolivariana, Medellín 050031, ColombiaThis study evaluated the desorption of cadmium (Cd) from cocoa waste-derived flour using organic acids. Cocoa pods were collected from Antioquia and Casanare, Colombia, to analyze the geographical Cd content and its distribution within the pod tissues. Acid selection was performed using a multi-criteria decision-making (MCDM) matrix, and Cd desorption was assessed through a full factorial 2<sup>3</sup> experimental design, considering acid concentration, pulp density, and agitation speed. Additionally, the oxidation–reduction potential (ORP) was monitored as an indicator of the electrochemical dynamics of the process. The results indicated that pods from Casanare exhibited higher Cd concentrations (1.63 ± 0.20 ppm) compared with those from Antioquia (0.87 ± 0.22 ppm), with 49.31% of the metal being accumulated in the pod. Parameters of citric acid at 0.5 M, 5 g/L pulp density, and 120 rpm were found to be optimal for the Cd desorption process, achieving over 95% efficiency. Based on ORP monitoring, a heuristic was proposed to determine the contact time during leaching. This work outlines a scalable process for Cd desorption, adding value to cocoa industry waste for potential applications.https://www.mdpi.com/2304-8158/13/24/4048cadmiumcocoa wastecocoa pod husk flourdesorptionleachingorganic acids
spellingShingle Sebastián Piedrahíta-Pérez
Juliana Rodríguez-Estrada
Margarita Ramírez-Carmona
Leidy Rendón-Castrillón
Carlos Ocampo-López
Desorption of Cadmium from Cocoa Waste Using Organic Acids
Foods
cadmium
cocoa waste
cocoa pod husk flour
desorption
leaching
organic acids
title Desorption of Cadmium from Cocoa Waste Using Organic Acids
title_full Desorption of Cadmium from Cocoa Waste Using Organic Acids
title_fullStr Desorption of Cadmium from Cocoa Waste Using Organic Acids
title_full_unstemmed Desorption of Cadmium from Cocoa Waste Using Organic Acids
title_short Desorption of Cadmium from Cocoa Waste Using Organic Acids
title_sort desorption of cadmium from cocoa waste using organic acids
topic cadmium
cocoa waste
cocoa pod husk flour
desorption
leaching
organic acids
url https://www.mdpi.com/2304-8158/13/24/4048
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AT margaritaramirezcarmona desorptionofcadmiumfromcocoawasteusingorganicacids
AT leidyrendoncastrillon desorptionofcadmiumfromcocoawasteusingorganicacids
AT carlosocampolopez desorptionofcadmiumfromcocoawasteusingorganicacids