Zn-Co nanoferrite electrocatalysts for enhanced hydrogen and oxygen generation

This study aims to investigate the role of Zn1-xCoxFe2O4 electrocatalysts in enhancing the efficiency of water splitting reactions for hydrogen and oxygen evolution. A potpourri of hydrothermally synthesized Zn1-xCoxFe2O4 electrocatalysts was prepared to enhance water splitting reaction to evolve va...

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Main Authors: Kiran Shahzadi, Muhammad Sarfraz, Muneerah Alomar, M.A. Mujtaba, Muhammad Nasir Bashir, Muhammad Mahmood Ali, Faisal Ali
Format: Article
Language:English
Published: Elsevier 2025-07-01
Series:Results in Chemistry
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Online Access:http://www.sciencedirect.com/science/article/pii/S2211715625003753
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author Kiran Shahzadi
Muhammad Sarfraz
Muneerah Alomar
M.A. Mujtaba
Muhammad Nasir Bashir
Muhammad Mahmood Ali
Faisal Ali
author_facet Kiran Shahzadi
Muhammad Sarfraz
Muneerah Alomar
M.A. Mujtaba
Muhammad Nasir Bashir
Muhammad Mahmood Ali
Faisal Ali
author_sort Kiran Shahzadi
collection DOAJ
description This study aims to investigate the role of Zn1-xCoxFe2O4 electrocatalysts in enhancing the efficiency of water splitting reactions for hydrogen and oxygen evolution. A potpourri of hydrothermally synthesized Zn1-xCoxFe2O4 electrocatalysts was prepared to enhance water splitting reaction to evolve valuable hydrogen and oxygen gases. Fourier transform infrared spectroscopy and X-ray diffraction techniques respectively corroborated chemical synthesis and cubic spinel structure of Zn1-xCoxFe2O4 alpha-ferrite electrocatalyst nanocrystals. Electrocatalytic behavior of prepared electrocatalysts was measured in terms of Tafel slope, overpotential and onset potential via linear sweep voltammetry and cyclic voltammetry techniques. Electrochemical impedance spectroscopy assessed electrocatalytic capability for solution resistance and charge transfer. Electrocatalyst with higher concentration of cobalt than zinc in concocted ferrites (CoFe2O4), rendered largest electrocatalytic oxygen evolution reaction with lowest charge transfer resistance of 2.1 Ω, onset potential of 1.51 V, overpotential of 280 mV, and a Tafel slope of 65 mV/dec. Synthesized nanoferrite materials find electrocatalytic potential for evolution of hydrogen and oxygen in water splitting reactions according to electrochemical investigations. The findings suggest that Zn₁₋ₓCoₓFe₂O₄ electrocatalysts, particularly those with higher cobalt content, can serve as efficient electrocatalysts for water splitting, providing a pathway for clean hydrogen fuel production.
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spelling doaj-art-e5d917868aa44771b44e2bb01fd1c4892025-08-20T03:23:34ZengElsevierResults in Chemistry2211-71562025-07-011610239210.1016/j.rechem.2025.102392Zn-Co nanoferrite electrocatalysts for enhanced hydrogen and oxygen generationKiran Shahzadi0Muhammad Sarfraz1Muneerah Alomar2M.A. Mujtaba3Muhammad Nasir Bashir4Muhammad Mahmood Ali5Faisal Ali6Department of Polymer and Process Engineering, University of Engineering and Technology, 54890, PakistanDepartment of Polymer and Process Engineering, University of Engineering and Technology, 54890, Pakistan; Corresponding authors.Department of Physics, College of Science, Princess Nourah bint Abdulrahman University, P.O. Box 84428, Riyadh 11671, Saudi ArabiaDepartment of Mechanical Engineering, UET Lahore (New Campus), Lahore 54890, PakistanDepartment of Mechanical Engineering, University of Malaya, Kuala Lumpur 50603, Malaysia; National University of Sciences and Technology, Islamabad, PakistanDepartment of Mechatronic Engineering, Atlantic Technological University Sligo, Ash Lane, F91 YW50 Sligo, Ireland; Centre for Mathematical Modelling and Intelligent Systems for Health and Environment (MISHE), Atlantic Technological University, F91 YW50 Sligo, Ireland; Corresponding authors.Department of Mechanical Engineering, UET Lahore (New Campus), Lahore 54890, PakistanThis study aims to investigate the role of Zn1-xCoxFe2O4 electrocatalysts in enhancing the efficiency of water splitting reactions for hydrogen and oxygen evolution. A potpourri of hydrothermally synthesized Zn1-xCoxFe2O4 electrocatalysts was prepared to enhance water splitting reaction to evolve valuable hydrogen and oxygen gases. Fourier transform infrared spectroscopy and X-ray diffraction techniques respectively corroborated chemical synthesis and cubic spinel structure of Zn1-xCoxFe2O4 alpha-ferrite electrocatalyst nanocrystals. Electrocatalytic behavior of prepared electrocatalysts was measured in terms of Tafel slope, overpotential and onset potential via linear sweep voltammetry and cyclic voltammetry techniques. Electrochemical impedance spectroscopy assessed electrocatalytic capability for solution resistance and charge transfer. Electrocatalyst with higher concentration of cobalt than zinc in concocted ferrites (CoFe2O4), rendered largest electrocatalytic oxygen evolution reaction with lowest charge transfer resistance of 2.1 Ω, onset potential of 1.51 V, overpotential of 280 mV, and a Tafel slope of 65 mV/dec. Synthesized nanoferrite materials find electrocatalytic potential for evolution of hydrogen and oxygen in water splitting reactions according to electrochemical investigations. The findings suggest that Zn₁₋ₓCoₓFe₂O₄ electrocatalysts, particularly those with higher cobalt content, can serve as efficient electrocatalysts for water splitting, providing a pathway for clean hydrogen fuel production.http://www.sciencedirect.com/science/article/pii/S2211715625003753Zn-Co nanoferritesElectrocatalysisOxygen evolution reactionHydrothermal synthesisWater splitting reaction
spellingShingle Kiran Shahzadi
Muhammad Sarfraz
Muneerah Alomar
M.A. Mujtaba
Muhammad Nasir Bashir
Muhammad Mahmood Ali
Faisal Ali
Zn-Co nanoferrite electrocatalysts for enhanced hydrogen and oxygen generation
Results in Chemistry
Zn-Co nanoferrites
Electrocatalysis
Oxygen evolution reaction
Hydrothermal synthesis
Water splitting reaction
title Zn-Co nanoferrite electrocatalysts for enhanced hydrogen and oxygen generation
title_full Zn-Co nanoferrite electrocatalysts for enhanced hydrogen and oxygen generation
title_fullStr Zn-Co nanoferrite electrocatalysts for enhanced hydrogen and oxygen generation
title_full_unstemmed Zn-Co nanoferrite electrocatalysts for enhanced hydrogen and oxygen generation
title_short Zn-Co nanoferrite electrocatalysts for enhanced hydrogen and oxygen generation
title_sort zn co nanoferrite electrocatalysts for enhanced hydrogen and oxygen generation
topic Zn-Co nanoferrites
Electrocatalysis
Oxygen evolution reaction
Hydrothermal synthesis
Water splitting reaction
url http://www.sciencedirect.com/science/article/pii/S2211715625003753
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AT muhammadsarfraz znconanoferriteelectrocatalystsforenhancedhydrogenandoxygengeneration
AT muneerahalomar znconanoferriteelectrocatalystsforenhancedhydrogenandoxygengeneration
AT mamujtaba znconanoferriteelectrocatalystsforenhancedhydrogenandoxygengeneration
AT muhammadnasirbashir znconanoferriteelectrocatalystsforenhancedhydrogenandoxygengeneration
AT muhammadmahmoodali znconanoferriteelectrocatalystsforenhancedhydrogenandoxygengeneration
AT faisalali znconanoferriteelectrocatalystsforenhancedhydrogenandoxygengeneration