The effect of different carbon materials’ addition on the biomethane production from food waste

Abstract Anaerobic digestion (AD) is a useful process that could be utilized for food waste (FW) management. Previous studies have shown that carbon materials (CMs) could be an important additive for increasing biomethane yield. However, why CMs improve AD is still uncertain. A significant body of r...

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Main Authors: Michał Kozłowski, Bernard Papaj, Karolina Sobieraj, Kacper Świechowski, Katarzyna Kosiorowska, Andrzej Białowiec
Format: Article
Language:English
Published: Nature Portfolio 2025-05-01
Series:Scientific Reports
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Online Access:https://doi.org/10.1038/s41598-025-02564-0
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author Michał Kozłowski
Bernard Papaj
Karolina Sobieraj
Kacper Świechowski
Katarzyna Kosiorowska
Andrzej Białowiec
author_facet Michał Kozłowski
Bernard Papaj
Karolina Sobieraj
Kacper Świechowski
Katarzyna Kosiorowska
Andrzej Białowiec
author_sort Michał Kozłowski
collection DOAJ
description Abstract Anaerobic digestion (AD) is a useful process that could be utilized for food waste (FW) management. Previous studies have shown that carbon materials (CMs) could be an important additive for increasing biomethane yield. However, why CMs improve AD is still uncertain. A significant body of research has been dedicated to investigating the impact of CMs supplementation on biogas production. However, this article specifically emphasizes examining this effect concerning the specific surface area and the functional groups (e.g. hydroxyl groups, carbonyl groups, or unsaturated carbon structures) present on the surface of CMs, produced by torrefaction—TP (240 °C/60 min), pyrolysis—BC (600 °C/60 min), and hydrothermal carbonization—HC (240 °C/60 min/6–10 Bar) processes. The analyses showed that the size of the specific surface area of the CMs (TP—7.72 m2 g−1, BC- 115.00 m2 g−1, HC—5.46 m2 g−1), does not correspond to the production of biomethane. The highest biomethane potential was found for CMs with the lowest SSA, precisely TP and HC, equal to 407 and 394 mL gVS−1, which was about 13 and 9% higher than production from FW as a sole source of carbon, respectively. The FTIR analysis confirmed the abundance of different organic functional groups on the surface of TP and HC, which could contribute to improved AD performance. These organic residuals, as thermal degradation products, could be an additional source of carbon for microorganisms. The addition of BC, with the highest SSA, decreased the first-order biomethane rate constant k by 16.4% in comparison to food waste without CMs, which could be related to the presence of harmful, more complex organic compounds on the surface of biochar.
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spelling doaj-art-e5bec6c535e24517a3918c67021f83a82025-08-20T03:16:50ZengNature PortfolioScientific Reports2045-23222025-05-0115111110.1038/s41598-025-02564-0The effect of different carbon materials’ addition on the biomethane production from food wasteMichał Kozłowski0Bernard Papaj1Karolina Sobieraj2Kacper Świechowski3Katarzyna Kosiorowska4Andrzej Białowiec5Department of Applied Bioeconomy, Wroclaw University of Environmental and Life SciencesDepartment of Applied Bioeconomy, Wroclaw University of Environmental and Life SciencesDepartment of Applied Bioeconomy, Wroclaw University of Environmental and Life SciencesDepartment of Applied Bioeconomy, Wroclaw University of Environmental and Life SciencesDepartment of Applied Bioeconomy, Wroclaw University of Environmental and Life SciencesDepartment of Applied Bioeconomy, Wroclaw University of Environmental and Life SciencesAbstract Anaerobic digestion (AD) is a useful process that could be utilized for food waste (FW) management. Previous studies have shown that carbon materials (CMs) could be an important additive for increasing biomethane yield. However, why CMs improve AD is still uncertain. A significant body of research has been dedicated to investigating the impact of CMs supplementation on biogas production. However, this article specifically emphasizes examining this effect concerning the specific surface area and the functional groups (e.g. hydroxyl groups, carbonyl groups, or unsaturated carbon structures) present on the surface of CMs, produced by torrefaction—TP (240 °C/60 min), pyrolysis—BC (600 °C/60 min), and hydrothermal carbonization—HC (240 °C/60 min/6–10 Bar) processes. The analyses showed that the size of the specific surface area of the CMs (TP—7.72 m2 g−1, BC- 115.00 m2 g−1, HC—5.46 m2 g−1), does not correspond to the production of biomethane. The highest biomethane potential was found for CMs with the lowest SSA, precisely TP and HC, equal to 407 and 394 mL gVS−1, which was about 13 and 9% higher than production from FW as a sole source of carbon, respectively. The FTIR analysis confirmed the abundance of different organic functional groups on the surface of TP and HC, which could contribute to improved AD performance. These organic residuals, as thermal degradation products, could be an additional source of carbon for microorganisms. The addition of BC, with the highest SSA, decreased the first-order biomethane rate constant k by 16.4% in comparison to food waste without CMs, which could be related to the presence of harmful, more complex organic compounds on the surface of biochar.https://doi.org/10.1038/s41598-025-02564-0Anaerobic digestionTorrefaction productBiocharHydrocharSpecific surface area
spellingShingle Michał Kozłowski
Bernard Papaj
Karolina Sobieraj
Kacper Świechowski
Katarzyna Kosiorowska
Andrzej Białowiec
The effect of different carbon materials’ addition on the biomethane production from food waste
Scientific Reports
Anaerobic digestion
Torrefaction product
Biochar
Hydrochar
Specific surface area
title The effect of different carbon materials’ addition on the biomethane production from food waste
title_full The effect of different carbon materials’ addition on the biomethane production from food waste
title_fullStr The effect of different carbon materials’ addition on the biomethane production from food waste
title_full_unstemmed The effect of different carbon materials’ addition on the biomethane production from food waste
title_short The effect of different carbon materials’ addition on the biomethane production from food waste
title_sort effect of different carbon materials addition on the biomethane production from food waste
topic Anaerobic digestion
Torrefaction product
Biochar
Hydrochar
Specific surface area
url https://doi.org/10.1038/s41598-025-02564-0
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