Synthesis of Silicon-Containing Chitosan Hydrogels in a Glycolic Acid Medium

The present paper considers a “one-pot” green sol-gel synthesis of hybrid inorganic/organic hydrogels based on chitosan glycolate by using organically modified silica Si(OGly)4·2GlyOH as a precursor to form a network of ≡Si–O–Si≡ bonds at 4, 20, and 37°C. The gelation time of the multicomponent chit...

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Main Authors: A. B. Shipovskaya, O. N. Malinkina, Yu. Yu. Zhuravleva, S. M. Rogacheva
Format: Article
Language:English
Published: Wiley 2016-01-01
Series:Advances in Materials Science and Engineering
Online Access:http://dx.doi.org/10.1155/2016/3951703
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author A. B. Shipovskaya
O. N. Malinkina
Yu. Yu. Zhuravleva
S. M. Rogacheva
author_facet A. B. Shipovskaya
O. N. Malinkina
Yu. Yu. Zhuravleva
S. M. Rogacheva
author_sort A. B. Shipovskaya
collection DOAJ
description The present paper considers a “one-pot” green sol-gel synthesis of hybrid inorganic/organic hydrogels based on chitosan glycolate by using organically modified silica Si(OGly)4·2GlyOH as a precursor to form a network of ≡Si–O–Si≡ bonds at 4, 20, and 37°C. The gelation time of the multicomponent chitosan-containing system was estimated as a function of the composition (the polymer template and precursor concentrations, introduction of a low-molecular-weight accelerator NaCl) and gelation conditions (the pH and temperature of the sol-gel process). It has been shown that an increased polymeric salt concentration, the introduction of an accelerator, and increased pH and temperature accelerate the gel-forming process.
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issn 1687-8434
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publishDate 2016-01-01
publisher Wiley
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series Advances in Materials Science and Engineering
spelling doaj-art-e3c522c437a147568eeee5dfd429c22d2025-08-20T02:21:24ZengWileyAdvances in Materials Science and Engineering1687-84341687-84422016-01-01201610.1155/2016/39517033951703Synthesis of Silicon-Containing Chitosan Hydrogels in a Glycolic Acid MediumA. B. Shipovskaya0O. N. Malinkina1Yu. Yu. Zhuravleva2S. M. Rogacheva3Chernyshevsky Saratov State University, 83 Astrakhanskaya St., Saratov 410012, RussiaChernyshevsky Saratov State University, 83 Astrakhanskaya St., Saratov 410012, RussiaChernyshevsky Saratov State University, 83 Astrakhanskaya St., Saratov 410012, RussiaYuri Gagarin State Technical University, 77 Politechnicheskaya St., Saratov 410054, RussiaThe present paper considers a “one-pot” green sol-gel synthesis of hybrid inorganic/organic hydrogels based on chitosan glycolate by using organically modified silica Si(OGly)4·2GlyOH as a precursor to form a network of ≡Si–O–Si≡ bonds at 4, 20, and 37°C. The gelation time of the multicomponent chitosan-containing system was estimated as a function of the composition (the polymer template and precursor concentrations, introduction of a low-molecular-weight accelerator NaCl) and gelation conditions (the pH and temperature of the sol-gel process). It has been shown that an increased polymeric salt concentration, the introduction of an accelerator, and increased pH and temperature accelerate the gel-forming process.http://dx.doi.org/10.1155/2016/3951703
spellingShingle A. B. Shipovskaya
O. N. Malinkina
Yu. Yu. Zhuravleva
S. M. Rogacheva
Synthesis of Silicon-Containing Chitosan Hydrogels in a Glycolic Acid Medium
Advances in Materials Science and Engineering
title Synthesis of Silicon-Containing Chitosan Hydrogels in a Glycolic Acid Medium
title_full Synthesis of Silicon-Containing Chitosan Hydrogels in a Glycolic Acid Medium
title_fullStr Synthesis of Silicon-Containing Chitosan Hydrogels in a Glycolic Acid Medium
title_full_unstemmed Synthesis of Silicon-Containing Chitosan Hydrogels in a Glycolic Acid Medium
title_short Synthesis of Silicon-Containing Chitosan Hydrogels in a Glycolic Acid Medium
title_sort synthesis of silicon containing chitosan hydrogels in a glycolic acid medium
url http://dx.doi.org/10.1155/2016/3951703
work_keys_str_mv AT abshipovskaya synthesisofsiliconcontainingchitosanhydrogelsinaglycolicacidmedium
AT onmalinkina synthesisofsiliconcontainingchitosanhydrogelsinaglycolicacidmedium
AT yuyuzhuravleva synthesisofsiliconcontainingchitosanhydrogelsinaglycolicacidmedium
AT smrogacheva synthesisofsiliconcontainingchitosanhydrogelsinaglycolicacidmedium