Sb‐Se‐based electrical switching device with fast transition speed and minimized performance degradation due to stable mid‐gap states

Abstract Chalcogenide glass has a unique volatile transition between high‐ and low‐resistance states under an electric field, a phenomenon termed ovonic threshold switching (OTS). This characteristic is extensively utilized in various electronic memory and computational devices, particularly as sele...

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Main Authors: Xianliang Mai, Qundao Xu, Zhe Yang, Huan Wang, Yongpeng Liu, Yinghua Shen, Hengyi Hu, Meng Xu, Zhongrui Wang, Hao Tong, Chengliang Wang, Xiangshui Miao, Ming Xu
Format: Article
Language:English
Published: Wiley 2025-02-01
Series:Electron
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Online Access:https://doi.org/10.1002/elt2.46
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author Xianliang Mai
Qundao Xu
Zhe Yang
Huan Wang
Yongpeng Liu
Yinghua Shen
Hengyi Hu
Meng Xu
Zhongrui Wang
Hao Tong
Chengliang Wang
Xiangshui Miao
Ming Xu
author_facet Xianliang Mai
Qundao Xu
Zhe Yang
Huan Wang
Yongpeng Liu
Yinghua Shen
Hengyi Hu
Meng Xu
Zhongrui Wang
Hao Tong
Chengliang Wang
Xiangshui Miao
Ming Xu
author_sort Xianliang Mai
collection DOAJ
description Abstract Chalcogenide glass has a unique volatile transition between high‐ and low‐resistance states under an electric field, a phenomenon termed ovonic threshold switching (OTS). This characteristic is extensively utilized in various electronic memory and computational devices, particularly as selectors for cross‐point memory architectures. Despite its advantages, the material is susceptible to glass relaxation, which can result in substantial drifts in threshold voltage and a decline in off‐current performance over successive operational cycles or long storage time. In this study, we introduce an OTS device made from stoichiometric Sb2Se3 glass, which retains an octahedral local structure within its amorphous matrix. This innovative material exhibits outstanding OTS capabilities, maintaining minimal degradation despite undergoing over 107 operating cycles. Via comprehensive first‐principles calculations, our findings indicate that the mid‐gap states in amorphous Sb2Se3 predominantly stem from the atomic chains characterized by heteropolar Sb‐Se bonds. These bonds exhibit remarkable stability, showing minimal alteration over time, thereby contributing to the overall durability and consistent performance of the material. Our findings not only shed light on the complex physical origins that govern the OTS behavior but also lay the groundwork for creating or optimizing innovative electrical switching materials.
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institution Kabale University
issn 2751-2606
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publishDate 2025-02-01
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spelling doaj-art-e378addd507d4310bb3a11f2c74cd47f2025-08-20T03:30:56ZengWileyElectron2751-26062751-26142025-02-0131n/an/a10.1002/elt2.46Sb‐Se‐based electrical switching device with fast transition speed and minimized performance degradation due to stable mid‐gap statesXianliang Mai0Qundao Xu1Zhe Yang2Huan Wang3Yongpeng Liu4Yinghua Shen5Hengyi Hu6Meng Xu7Zhongrui Wang8Hao Tong9Chengliang Wang10Xiangshui Miao11Ming Xu12Wuhan National Laboratory for Optoelectronics School of Integrated Circuits Huazhong University of Science and Technology Wuhan ChinaWuhan National Laboratory for Optoelectronics School of Integrated Circuits Huazhong University of Science and Technology Wuhan ChinaWuhan National Laboratory for Optoelectronics School of Integrated Circuits Huazhong University of Science and Technology Wuhan ChinaWuhan National Laboratory for Optoelectronics School of Integrated Circuits Huazhong University of Science and Technology Wuhan ChinaWuhan National Laboratory for Optoelectronics School of Integrated Circuits Huazhong University of Science and Technology Wuhan ChinaWuhan National Laboratory for Optoelectronics School of Integrated Circuits Huazhong University of Science and Technology Wuhan ChinaWuhan National Laboratory for Optoelectronics School of Integrated Circuits Huazhong University of Science and Technology Wuhan ChinaDepartment of Electrical and Electronic Engineering The University of Hong Kong Hong Kong ChinaDepartment of Electrical and Electronic Engineering The University of Hong Kong Hong Kong ChinaWuhan National Laboratory for Optoelectronics School of Integrated Circuits Huazhong University of Science and Technology Wuhan ChinaWuhan National Laboratory for Optoelectronics School of Integrated Circuits Huazhong University of Science and Technology Wuhan ChinaWuhan National Laboratory for Optoelectronics School of Integrated Circuits Huazhong University of Science and Technology Wuhan ChinaWuhan National Laboratory for Optoelectronics School of Integrated Circuits Huazhong University of Science and Technology Wuhan ChinaAbstract Chalcogenide glass has a unique volatile transition between high‐ and low‐resistance states under an electric field, a phenomenon termed ovonic threshold switching (OTS). This characteristic is extensively utilized in various electronic memory and computational devices, particularly as selectors for cross‐point memory architectures. Despite its advantages, the material is susceptible to glass relaxation, which can result in substantial drifts in threshold voltage and a decline in off‐current performance over successive operational cycles or long storage time. In this study, we introduce an OTS device made from stoichiometric Sb2Se3 glass, which retains an octahedral local structure within its amorphous matrix. This innovative material exhibits outstanding OTS capabilities, maintaining minimal degradation despite undergoing over 107 operating cycles. Via comprehensive first‐principles calculations, our findings indicate that the mid‐gap states in amorphous Sb2Se3 predominantly stem from the atomic chains characterized by heteropolar Sb‐Se bonds. These bonds exhibit remarkable stability, showing minimal alteration over time, thereby contributing to the overall durability and consistent performance of the material. Our findings not only shed light on the complex physical origins that govern the OTS behavior but also lay the groundwork for creating or optimizing innovative electrical switching materials.https://doi.org/10.1002/elt2.46chalcogenide glassfirst‐principles calculationovonic threshold switchingphase change memorySb2Se3
spellingShingle Xianliang Mai
Qundao Xu
Zhe Yang
Huan Wang
Yongpeng Liu
Yinghua Shen
Hengyi Hu
Meng Xu
Zhongrui Wang
Hao Tong
Chengliang Wang
Xiangshui Miao
Ming Xu
Sb‐Se‐based electrical switching device with fast transition speed and minimized performance degradation due to stable mid‐gap states
Electron
chalcogenide glass
first‐principles calculation
ovonic threshold switching
phase change memory
Sb2Se3
title Sb‐Se‐based electrical switching device with fast transition speed and minimized performance degradation due to stable mid‐gap states
title_full Sb‐Se‐based electrical switching device with fast transition speed and minimized performance degradation due to stable mid‐gap states
title_fullStr Sb‐Se‐based electrical switching device with fast transition speed and minimized performance degradation due to stable mid‐gap states
title_full_unstemmed Sb‐Se‐based electrical switching device with fast transition speed and minimized performance degradation due to stable mid‐gap states
title_short Sb‐Se‐based electrical switching device with fast transition speed and minimized performance degradation due to stable mid‐gap states
title_sort sb se based electrical switching device with fast transition speed and minimized performance degradation due to stable mid gap states
topic chalcogenide glass
first‐principles calculation
ovonic threshold switching
phase change memory
Sb2Se3
url https://doi.org/10.1002/elt2.46
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