Collagen fibers as biomass templates constructed multifunctional polyvinyl alcohol composite films for biocompatible wearable e-skins

Multifunctional characteristics are of significance for development of bionic skin materials. Herein, we report the collagen fibers (CFs) as biomass templates constructed multifunctional polyvinyl alcohol composite films (PCBPP) that integrate the diverse properties including the good thermal stabil...

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Main Authors: Wang Ya-nan, Niku Guge, Chen Hao, Wang Yujia
Format: Article
Language:English
Published: De Gruyter 2025-07-01
Series:Science and Engineering of Composite Materials
Subjects:
Online Access:https://doi.org/10.1515/secm-2025-0058
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author Wang Ya-nan
Niku Guge
Chen Hao
Wang Yujia
author_facet Wang Ya-nan
Niku Guge
Chen Hao
Wang Yujia
author_sort Wang Ya-nan
collection DOAJ
description Multifunctional characteristics are of significance for development of bionic skin materials. Herein, we report the collagen fibers (CFs) as biomass templates constructed multifunctional polyvinyl alcohol composite films (PCBPP) that integrate the diverse properties including the good thermal stability, water resistance, self-healing ability, adhesiveness, benign biocompatibility, and sensitive electrical signal response within a single structure, realize much more favorable functionalities in mimicking natural skin. The CFs as biomass template well immobilize and stabilize the polypyrrole (PPy) nanoparticles, which simultaneously improves the dispersity of PPy and enhances its conductivity. More importantly, due to the CFs constructed conductive paths and micro- and nano-sensing structure, the PCBPP prepared e-skin exhibits the GF value of 0.366 in the strain range of 10–40% and is able to distinguish different strain intensities and monitor the movements of the human body, including wrist bending, elbow bending, and swallowing. The self-healed PCBPP prepared e-skin exhibited the recoverable sensitivity. Our investigation provided a new prospect for designing CFs as conductive network packed multifunctional composite film and the as-prepared PCBPP exhibits great potential for versatile applications in various wearable devices and in the field of artificial intelligence.
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institution Kabale University
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series Science and Engineering of Composite Materials
spelling doaj-art-e33eedeefa28420bab380a69f7aa1ecd2025-08-20T03:27:21ZengDe GruyterScience and Engineering of Composite Materials2191-03592025-07-0132198673782010.1515/secm-2025-0058Collagen fibers as biomass templates constructed multifunctional polyvinyl alcohol composite films for biocompatible wearable e-skinsWang Ya-nan0Niku Guge1Chen Hao2Wang Yujia3College of Chemistry and Engineering, Sichuan University of Science and Engineering, Zigong, 643000, P.R. ChinaCollege of Chemistry and Engineering, Sichuan University of Science and Engineering, Zigong, 643000, P.R. ChinaCollege of Chemistry and Engineering, Sichuan University of Science and Engineering, Zigong, 643000, P.R. ChinaDepartment of Biomass Chemistry and Engineering, Sichuan University, Chengdu, 610065, P.R. ChinaMultifunctional characteristics are of significance for development of bionic skin materials. Herein, we report the collagen fibers (CFs) as biomass templates constructed multifunctional polyvinyl alcohol composite films (PCBPP) that integrate the diverse properties including the good thermal stability, water resistance, self-healing ability, adhesiveness, benign biocompatibility, and sensitive electrical signal response within a single structure, realize much more favorable functionalities in mimicking natural skin. The CFs as biomass template well immobilize and stabilize the polypyrrole (PPy) nanoparticles, which simultaneously improves the dispersity of PPy and enhances its conductivity. More importantly, due to the CFs constructed conductive paths and micro- and nano-sensing structure, the PCBPP prepared e-skin exhibits the GF value of 0.366 in the strain range of 10–40% and is able to distinguish different strain intensities and monitor the movements of the human body, including wrist bending, elbow bending, and swallowing. The self-healed PCBPP prepared e-skin exhibited the recoverable sensitivity. Our investigation provided a new prospect for designing CFs as conductive network packed multifunctional composite film and the as-prepared PCBPP exhibits great potential for versatile applications in various wearable devices and in the field of artificial intelligence.https://doi.org/10.1515/secm-2025-0058collagen fibersbiomass templatemultifunctionalitypva composite filmbiocompatibilitywearabilitye-skin
spellingShingle Wang Ya-nan
Niku Guge
Chen Hao
Wang Yujia
Collagen fibers as biomass templates constructed multifunctional polyvinyl alcohol composite films for biocompatible wearable e-skins
Science and Engineering of Composite Materials
collagen fibers
biomass template
multifunctionality
pva composite film
biocompatibility
wearability
e-skin
title Collagen fibers as biomass templates constructed multifunctional polyvinyl alcohol composite films for biocompatible wearable e-skins
title_full Collagen fibers as biomass templates constructed multifunctional polyvinyl alcohol composite films for biocompatible wearable e-skins
title_fullStr Collagen fibers as biomass templates constructed multifunctional polyvinyl alcohol composite films for biocompatible wearable e-skins
title_full_unstemmed Collagen fibers as biomass templates constructed multifunctional polyvinyl alcohol composite films for biocompatible wearable e-skins
title_short Collagen fibers as biomass templates constructed multifunctional polyvinyl alcohol composite films for biocompatible wearable e-skins
title_sort collagen fibers as biomass templates constructed multifunctional polyvinyl alcohol composite films for biocompatible wearable e skins
topic collagen fibers
biomass template
multifunctionality
pva composite film
biocompatibility
wearability
e-skin
url https://doi.org/10.1515/secm-2025-0058
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AT nikuguge collagenfibersasbiomasstemplatesconstructedmultifunctionalpolyvinylalcoholcompositefilmsforbiocompatiblewearableeskins
AT chenhao collagenfibersasbiomasstemplatesconstructedmultifunctionalpolyvinylalcoholcompositefilmsforbiocompatiblewearableeskins
AT wangyujia collagenfibersasbiomasstemplatesconstructedmultifunctionalpolyvinylalcoholcompositefilmsforbiocompatiblewearableeskins