Nano-chitosan-coated, green-synthesized selenium nanoparticles as a novel antifungal agent against Sclerotinia sclerotiorum: in vitro study

Abstract Chemical fungicides have been used to control fungal diseases like Sclerotinia sclerotiorum. These fungicides must be restricted because of their toxicity and the development of resistance strains. Therefore, utilizing natural nanoscale materials in agricultural production is a potential al...

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Main Authors: Mohamed M. Desouky, Radwa H. Abou-Saleh, Tarek A. A. Moussa, Heba M. Fahmy
Format: Article
Language:English
Published: Nature Portfolio 2025-01-01
Series:Scientific Reports
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Online Access:https://doi.org/10.1038/s41598-024-79574-x
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author Mohamed M. Desouky
Radwa H. Abou-Saleh
Tarek A. A. Moussa
Heba M. Fahmy
author_facet Mohamed M. Desouky
Radwa H. Abou-Saleh
Tarek A. A. Moussa
Heba M. Fahmy
author_sort Mohamed M. Desouky
collection DOAJ
description Abstract Chemical fungicides have been used to control fungal diseases like Sclerotinia sclerotiorum. These fungicides must be restricted because of their toxicity and the development of resistance strains. Therefore, utilizing natural nanoscale materials in agricultural production is a potential alternative. This work aimed to investigate the antifungal properties of a nanocomposite (nano-chitosan-coated, green-synthesized selenium nanoparticles) against the plant pathogenic fungus S. sclerotiorum. Chemical reduction was used to produce selenium nanoparticles from citrus peel extracts, and ionotropic gelation was used to produce chitosan nanoparticles. The nanocomposite has been produced using selenium nanoparticles stabilized by chitosan and cross-linked with sodium tripolyphosphate. Transmission electron microscopy, dynamic light scattering, X-ray diffraction, UV-VIS spectroscopy, and Fourier transform infrared spectroscopy were used to characterize all produced nanostructures. The in vitro antifungal activity and minimum inhibitory concentration of all bulk and nanostructures are investigated at (0.5, 1, 5, 10, 50, 100) ppm concentrations. Scanning electron microscopy was used to detect structural deformations in the fungal mycelium. The findings support the successful synthesis and characterization of all nanoparticles. Lemon peel extract produced smaller, more stable, and distributed selenium nanoparticles (42.28 ± 18.5 nm) than orange peel extract (85.7 ± 140.22 nm). Nanostructures, particularly nanocomposite, have shown a considerable increase in antifungal efficacy compared to bulk structures. At a minimum inhibitory concentration of 0.5 ppm, the nanocomposite exhibited 100% inhibitory activity. The nanocomposite with a concentration of 0.5 ppm exhibited the lowest average fungal biomass (0.32 ± 0.05 g) among all tested nanostructures. Fungal hyphae treated with 0.5 ppm of nanocomposite within 18 h of treatment revealed substantial damage and deformation. These results provide new insights into the nanocomposite as an eco-friendly and promising antifungal agent against other plant pathogenic fungi.
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spelling doaj-art-e335d5482dd14ccd9cbb35d92d7e11602025-08-20T02:40:27ZengNature PortfolioScientific Reports2045-23222025-01-0115111710.1038/s41598-024-79574-xNano-chitosan-coated, green-synthesized selenium nanoparticles as a novel antifungal agent against Sclerotinia sclerotiorum: in vitro studyMohamed M. Desouky0Radwa H. Abou-Saleh1Tarek A. A. Moussa2Heba M. Fahmy3Biophysics Department, Faculty of Science, Cairo UniversityNanoscience and Technology Program, Faculty of Science, Galala UniversityBotany and Microbiology Department, Faculty of Science, Cairo UniversityBiophysics Department, Faculty of Science, Cairo UniversityAbstract Chemical fungicides have been used to control fungal diseases like Sclerotinia sclerotiorum. These fungicides must be restricted because of their toxicity and the development of resistance strains. Therefore, utilizing natural nanoscale materials in agricultural production is a potential alternative. This work aimed to investigate the antifungal properties of a nanocomposite (nano-chitosan-coated, green-synthesized selenium nanoparticles) against the plant pathogenic fungus S. sclerotiorum. Chemical reduction was used to produce selenium nanoparticles from citrus peel extracts, and ionotropic gelation was used to produce chitosan nanoparticles. The nanocomposite has been produced using selenium nanoparticles stabilized by chitosan and cross-linked with sodium tripolyphosphate. Transmission electron microscopy, dynamic light scattering, X-ray diffraction, UV-VIS spectroscopy, and Fourier transform infrared spectroscopy were used to characterize all produced nanostructures. The in vitro antifungal activity and minimum inhibitory concentration of all bulk and nanostructures are investigated at (0.5, 1, 5, 10, 50, 100) ppm concentrations. Scanning electron microscopy was used to detect structural deformations in the fungal mycelium. The findings support the successful synthesis and characterization of all nanoparticles. Lemon peel extract produced smaller, more stable, and distributed selenium nanoparticles (42.28 ± 18.5 nm) than orange peel extract (85.7 ± 140.22 nm). Nanostructures, particularly nanocomposite, have shown a considerable increase in antifungal efficacy compared to bulk structures. At a minimum inhibitory concentration of 0.5 ppm, the nanocomposite exhibited 100% inhibitory activity. The nanocomposite with a concentration of 0.5 ppm exhibited the lowest average fungal biomass (0.32 ± 0.05 g) among all tested nanostructures. Fungal hyphae treated with 0.5 ppm of nanocomposite within 18 h of treatment revealed substantial damage and deformation. These results provide new insights into the nanocomposite as an eco-friendly and promising antifungal agent against other plant pathogenic fungi.https://doi.org/10.1038/s41598-024-79574-xGreen SynthesisChitosanSeleniumNanocompositeSclerotinia Sclerotiorum
spellingShingle Mohamed M. Desouky
Radwa H. Abou-Saleh
Tarek A. A. Moussa
Heba M. Fahmy
Nano-chitosan-coated, green-synthesized selenium nanoparticles as a novel antifungal agent against Sclerotinia sclerotiorum: in vitro study
Scientific Reports
Green Synthesis
Chitosan
Selenium
Nanocomposite
Sclerotinia Sclerotiorum
title Nano-chitosan-coated, green-synthesized selenium nanoparticles as a novel antifungal agent against Sclerotinia sclerotiorum: in vitro study
title_full Nano-chitosan-coated, green-synthesized selenium nanoparticles as a novel antifungal agent against Sclerotinia sclerotiorum: in vitro study
title_fullStr Nano-chitosan-coated, green-synthesized selenium nanoparticles as a novel antifungal agent against Sclerotinia sclerotiorum: in vitro study
title_full_unstemmed Nano-chitosan-coated, green-synthesized selenium nanoparticles as a novel antifungal agent against Sclerotinia sclerotiorum: in vitro study
title_short Nano-chitosan-coated, green-synthesized selenium nanoparticles as a novel antifungal agent against Sclerotinia sclerotiorum: in vitro study
title_sort nano chitosan coated green synthesized selenium nanoparticles as a novel antifungal agent against sclerotinia sclerotiorum in vitro study
topic Green Synthesis
Chitosan
Selenium
Nanocomposite
Sclerotinia Sclerotiorum
url https://doi.org/10.1038/s41598-024-79574-x
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