Enhanced performance of hafnia self-rectifying ferroelectric tunnel junctions at cryogenic temperatures

Abstract The advancement in high-performance computing technologies, including quantum and aerospace systems, necessitates components that operate efficiently at cryogenic temperatures. In this study, we demonstrate a hafnia-based ferroelectric tunnel junction (FTJ) that achieves a record-high tunne...

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Main Authors: Junghyeon Hwang, Chaeheon Kim, Jinho Ahn, Sanghun Jeon
Format: Article
Language:English
Published: SpringerOpen 2024-12-01
Series:Nano Convergence
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Online Access:https://doi.org/10.1186/s40580-024-00461-2
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author Junghyeon Hwang
Chaeheon Kim
Jinho Ahn
Sanghun Jeon
author_facet Junghyeon Hwang
Chaeheon Kim
Jinho Ahn
Sanghun Jeon
author_sort Junghyeon Hwang
collection DOAJ
description Abstract The advancement in high-performance computing technologies, including quantum and aerospace systems, necessitates components that operate efficiently at cryogenic temperatures. In this study, we demonstrate a hafnia-based ferroelectric tunnel junction (FTJ) that achieves a record-high tunneling electroresistance (TER) ratio of over 200,000 and decade-long retention characteristics. By introducing asymmetric oxygen vacancies through the strategic use of indium oxide (InOx) layer, we enhance the TER ratio without increasing off-current, addressing the longstanding issue of low on-current in hafnia-based FTJs. Unlike prior approaches that led to leakage currents, our method optimizes tunneling behavior by leveraging the differential oxygen dissociation energy between InOx and hafnium zirconium oxide (HZO). This results in asymmetric modulation of the tunnel barrier, enhancing electron tunneling in one polarization state while maintaining stability in the opposite state. Furthermore, we explore the intrinsic characteristics of the FTJ at cryogenic temperatures, where reduced thermal energy minimizes leakage currents and allows the maximization of device performance. These findings establish a new benchmark for TER in hafnia-based FTJs and provide valuable insights for the integration of these devices into advanced cryogenic memory systems. Graphical Abstract
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spelling doaj-art-e3203fd83ee345e29d4f18ab27c7b7492024-12-22T12:40:56ZengSpringerOpenNano Convergence2196-54042024-12-011111910.1186/s40580-024-00461-2Enhanced performance of hafnia self-rectifying ferroelectric tunnel junctions at cryogenic temperaturesJunghyeon Hwang0Chaeheon Kim1Jinho Ahn2Sanghun Jeon3School of Electrical Engineering, Korea Advanced Institute of Science and Technology (KAIST)School of Electrical Engineering, Korea Advanced Institute of Science and Technology (KAIST)Division of Materials Science and Engineering, Hanyang UniversitySchool of Electrical Engineering, Korea Advanced Institute of Science and Technology (KAIST)Abstract The advancement in high-performance computing technologies, including quantum and aerospace systems, necessitates components that operate efficiently at cryogenic temperatures. In this study, we demonstrate a hafnia-based ferroelectric tunnel junction (FTJ) that achieves a record-high tunneling electroresistance (TER) ratio of over 200,000 and decade-long retention characteristics. By introducing asymmetric oxygen vacancies through the strategic use of indium oxide (InOx) layer, we enhance the TER ratio without increasing off-current, addressing the longstanding issue of low on-current in hafnia-based FTJs. Unlike prior approaches that led to leakage currents, our method optimizes tunneling behavior by leveraging the differential oxygen dissociation energy between InOx and hafnium zirconium oxide (HZO). This results in asymmetric modulation of the tunnel barrier, enhancing electron tunneling in one polarization state while maintaining stability in the opposite state. Furthermore, we explore the intrinsic characteristics of the FTJ at cryogenic temperatures, where reduced thermal energy minimizes leakage currents and allows the maximization of device performance. These findings establish a new benchmark for TER in hafnia-based FTJs and provide valuable insights for the integration of these devices into advanced cryogenic memory systems. Graphical Abstracthttps://doi.org/10.1186/s40580-024-00461-2Ferroelectric tunnel junctionSelf-rectifyingHafnia-based ferroelectricsImprint effectCryogenic
spellingShingle Junghyeon Hwang
Chaeheon Kim
Jinho Ahn
Sanghun Jeon
Enhanced performance of hafnia self-rectifying ferroelectric tunnel junctions at cryogenic temperatures
Nano Convergence
Ferroelectric tunnel junction
Self-rectifying
Hafnia-based ferroelectrics
Imprint effect
Cryogenic
title Enhanced performance of hafnia self-rectifying ferroelectric tunnel junctions at cryogenic temperatures
title_full Enhanced performance of hafnia self-rectifying ferroelectric tunnel junctions at cryogenic temperatures
title_fullStr Enhanced performance of hafnia self-rectifying ferroelectric tunnel junctions at cryogenic temperatures
title_full_unstemmed Enhanced performance of hafnia self-rectifying ferroelectric tunnel junctions at cryogenic temperatures
title_short Enhanced performance of hafnia self-rectifying ferroelectric tunnel junctions at cryogenic temperatures
title_sort enhanced performance of hafnia self rectifying ferroelectric tunnel junctions at cryogenic temperatures
topic Ferroelectric tunnel junction
Self-rectifying
Hafnia-based ferroelectrics
Imprint effect
Cryogenic
url https://doi.org/10.1186/s40580-024-00461-2
work_keys_str_mv AT junghyeonhwang enhancedperformanceofhafniaselfrectifyingferroelectrictunneljunctionsatcryogenictemperatures
AT chaeheonkim enhancedperformanceofhafniaselfrectifyingferroelectrictunneljunctionsatcryogenictemperatures
AT jinhoahn enhancedperformanceofhafniaselfrectifyingferroelectrictunneljunctionsatcryogenictemperatures
AT sanghunjeon enhancedperformanceofhafniaselfrectifyingferroelectrictunneljunctionsatcryogenictemperatures