Riverine photosynthesis influences the carbon sequestration potential of enhanced rock weathering

As climate mitigation efforts lag, dependence on anthropogenic CO2 removal increases. Enhanced rock weathering (ERW) is a rapidly growing CO2 removal approach. In terrestrial ERW, crushed rocks are spread on land where they react with CO2 and water, forming dissolved inorganic carbon (DIC) and alkal...

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Main Authors: Rebecca B. Neumann, Tyler Kukla, Shuang Zhang, David E. Butman
Format: Article
Language:English
Published: Frontiers Media S.A. 2025-04-01
Series:Frontiers in Climate
Subjects:
Online Access:https://www.frontiersin.org/articles/10.3389/fclim.2025.1582786/full
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author Rebecca B. Neumann
Tyler Kukla
Shuang Zhang
David E. Butman
David E. Butman
author_facet Rebecca B. Neumann
Tyler Kukla
Shuang Zhang
David E. Butman
David E. Butman
author_sort Rebecca B. Neumann
collection DOAJ
description As climate mitigation efforts lag, dependence on anthropogenic CO2 removal increases. Enhanced rock weathering (ERW) is a rapidly growing CO2 removal approach. In terrestrial ERW, crushed rocks are spread on land where they react with CO2 and water, forming dissolved inorganic carbon (DIC) and alkalinity. For long-term sequestration, these products must travel through rivers to oceans, where carbon remains stored for over 10,000 years. Carbon and alkalinity can be lost during river transport, reducing ERW efficacy. However, the ability of biological processes, such as aquatic photosynthesis, to affect the fate of DIC and alkalinity within rivers has been overlooked. Our analysis indicates that within a stream-order segment, aquatic photosynthesis uptakes 1%–30% of DIC delivered by flow for most locations. The effect of this uptake on ERW efficacy, however, depends on the cell-membrane transport mechanism and the fate of photosynthetic carbon. Different pathways can decrease just DIC, DIC and alkalinity, or just alkalinity, and the relative importance of each is unknown. Further, data show that expected river chemistry changes from ERW may stimulate photosynthesis, amplifying the importance of these biological processes. We argue that estimating ERW’s carbon sequestration potential requires consideration and better understanding of biological processes in rivers.
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series Frontiers in Climate
spelling doaj-art-e30f1eafe027464491dea2da36567c092025-08-20T01:51:47ZengFrontiers Media S.A.Frontiers in Climate2624-95532025-04-01710.3389/fclim.2025.15827861582786Riverine photosynthesis influences the carbon sequestration potential of enhanced rock weatheringRebecca B. Neumann0Tyler Kukla1Shuang Zhang2David E. Butman3David E. Butman4Department of Civil & Environmental Engineering, University of Washington, Seattle, WA, United StatesCarbonPlan, San Francisco, CA, United StatesDepartment of Oceanography, Texas A&M University, College Station, TX, United StatesDepartment of Civil & Environmental Engineering, University of Washington, Seattle, WA, United StatesSchool of Environmental and Forest Sciences, University of Washington, Seattle, WA, United StatesAs climate mitigation efforts lag, dependence on anthropogenic CO2 removal increases. Enhanced rock weathering (ERW) is a rapidly growing CO2 removal approach. In terrestrial ERW, crushed rocks are spread on land where they react with CO2 and water, forming dissolved inorganic carbon (DIC) and alkalinity. For long-term sequestration, these products must travel through rivers to oceans, where carbon remains stored for over 10,000 years. Carbon and alkalinity can be lost during river transport, reducing ERW efficacy. However, the ability of biological processes, such as aquatic photosynthesis, to affect the fate of DIC and alkalinity within rivers has been overlooked. Our analysis indicates that within a stream-order segment, aquatic photosynthesis uptakes 1%–30% of DIC delivered by flow for most locations. The effect of this uptake on ERW efficacy, however, depends on the cell-membrane transport mechanism and the fate of photosynthetic carbon. Different pathways can decrease just DIC, DIC and alkalinity, or just alkalinity, and the relative importance of each is unknown. Further, data show that expected river chemistry changes from ERW may stimulate photosynthesis, amplifying the importance of these biological processes. We argue that estimating ERW’s carbon sequestration potential requires consideration and better understanding of biological processes in rivers.https://www.frontiersin.org/articles/10.3389/fclim.2025.1582786/fullcarbon dioxide removal (CDR)enhanced rock weatheringaquatic photosynthesisenhanced mineral weatheringcarbonalkalinity
spellingShingle Rebecca B. Neumann
Tyler Kukla
Shuang Zhang
David E. Butman
David E. Butman
Riverine photosynthesis influences the carbon sequestration potential of enhanced rock weathering
Frontiers in Climate
carbon dioxide removal (CDR)
enhanced rock weathering
aquatic photosynthesis
enhanced mineral weathering
carbon
alkalinity
title Riverine photosynthesis influences the carbon sequestration potential of enhanced rock weathering
title_full Riverine photosynthesis influences the carbon sequestration potential of enhanced rock weathering
title_fullStr Riverine photosynthesis influences the carbon sequestration potential of enhanced rock weathering
title_full_unstemmed Riverine photosynthesis influences the carbon sequestration potential of enhanced rock weathering
title_short Riverine photosynthesis influences the carbon sequestration potential of enhanced rock weathering
title_sort riverine photosynthesis influences the carbon sequestration potential of enhanced rock weathering
topic carbon dioxide removal (CDR)
enhanced rock weathering
aquatic photosynthesis
enhanced mineral weathering
carbon
alkalinity
url https://www.frontiersin.org/articles/10.3389/fclim.2025.1582786/full
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AT tylerkukla riverinephotosynthesisinfluencesthecarbonsequestrationpotentialofenhancedrockweathering
AT shuangzhang riverinephotosynthesisinfluencesthecarbonsequestrationpotentialofenhancedrockweathering
AT davidebutman riverinephotosynthesisinfluencesthecarbonsequestrationpotentialofenhancedrockweathering
AT davidebutman riverinephotosynthesisinfluencesthecarbonsequestrationpotentialofenhancedrockweathering