Anisotropic spin stripe domains in bilayer La3Ni2O7

Abstract The discovery of superconductivity in La3Ni2O7 under pressure has motivated the investigation of a parent spin density wave (SDW) state, which could provide the underlying pairing interaction. Here, we employ resonant soft x-ray scattering and polarimetry on thin films of bilayer La3Ni2O7 t...

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Bibliographic Details
Main Authors: Naman K. Gupta, Rantong Gong, Yi Wu, Mingu Kang, Christopher T. Parzyck, Benjamin Z. Gregory, Noah Costa, Ronny Sutarto, Suchismita Sarker, Andrej Singer, Darrell G. Schlom, Kyle M. Shen, David G. Hawthorn
Format: Article
Language:English
Published: Nature Portfolio 2025-07-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-61653-w
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Summary:Abstract The discovery of superconductivity in La3Ni2O7 under pressure has motivated the investigation of a parent spin density wave (SDW) state, which could provide the underlying pairing interaction. Here, we employ resonant soft x-ray scattering and polarimetry on thin films of bilayer La3Ni2O7 to determine that the magnetic structure of the SDW forms unidirectional diagonal spin stripes with moments lying within the NiO2 plane and perpendicular to Q SDW, but without evidence of the strong charge disproportionation typically associated with other nickelates. These stripes form anisotropic domains with shorter correlation lengths perpendicular versus parallel to Q SDW, revealing nanoscale rotational and translational symmetry breaking analogous to the cuprate and Fe-based superconductors, with possible Bloch-like antiferromagnetic domain walls separating orthogonal domains.
ISSN:2041-1723