WS<sub>2</sub>/Si<sub>3</sub>N<sub>4</sub>-Based Biosensor for Low-Concentration Coronavirus Detection

This study presents the optimization of two SPR biosensors, Sys<sub>3</sub> and Sys<sub>5</sub>, for SARS-CoV-2 detection at concentrations of 0.01–100 nM. Sys<sub>3</sub>, with a 55 nm silver layer, a 13 nm silicon nitride layer, and a 10 nm ssDNA layer, achieved...

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Main Authors: Talia Tene, Fabian Arias Arias, Karina I. Paredes-Páliz, Ana M. Cunachi Pillajo, Ana Gabriela Flores Huilcapi, Luis Santiago Carrera Almendariz, Stefano Bellucci
Format: Article
Language:English
Published: MDPI AG 2025-01-01
Series:Micromachines
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Online Access:https://www.mdpi.com/2072-666X/16/2/128
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author Talia Tene
Fabian Arias Arias
Karina I. Paredes-Páliz
Ana M. Cunachi Pillajo
Ana Gabriela Flores Huilcapi
Luis Santiago Carrera Almendariz
Stefano Bellucci
author_facet Talia Tene
Fabian Arias Arias
Karina I. Paredes-Páliz
Ana M. Cunachi Pillajo
Ana Gabriela Flores Huilcapi
Luis Santiago Carrera Almendariz
Stefano Bellucci
author_sort Talia Tene
collection DOAJ
description This study presents the optimization of two SPR biosensors, Sys<sub>3</sub> and Sys<sub>5</sub>, for SARS-CoV-2 detection at concentrations of 0.01–100 nM. Sys<sub>3</sub>, with a 55 nm silver layer, a 13 nm silicon nitride layer, and a 10 nm ssDNA layer, achieved a figure of merit (FoM) of 571.24 RIU<sup>−1</sup>, a signal-to-noise ratio (SNR) of 0.12, and a detection accuracy (DA) of 48.93 × 10<sup>−2</sup>. Sys<sub>5</sub>, incorporating a 50 nm silver layer, a 10 nm silicon nitride layer, a 10 nm ssDNA layer, and a 1.6 nm tungsten disulfide layer (L = 2), demonstrated a higher sensitivity of 305.33 °/RIU and a lower limit of detection (LoD) of 1.65 × 10<sup>−5</sup>. Sys<sub>3</sub> outshined in precision with low attenuation (<1%), while Sys<sub>5</sub> provided enhanced sensitivity and lower detection limits, crucial for early-stage viral detection. These configurations align with the refractive index ranges of clinical SARS-CoV-2 samples, showcasing their diagnostic potential. Future work will focus on experimental validation and integration into point-of-care platforms.
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spelling doaj-art-e1a5341b47534e08b62bf04de72be9e02025-08-20T02:04:02ZengMDPI AGMicromachines2072-666X2025-01-0116212810.3390/mi16020128WS<sub>2</sub>/Si<sub>3</sub>N<sub>4</sub>-Based Biosensor for Low-Concentration Coronavirus DetectionTalia Tene0Fabian Arias Arias1Karina I. Paredes-Páliz2Ana M. Cunachi Pillajo3Ana Gabriela Flores Huilcapi4Luis Santiago Carrera Almendariz5Stefano Bellucci6Department of Chemistry, Universidad Técnica Particular de Loja, Loja 110160, EcuadorDipartimento di Chimica e Tecnologie Chimiche, University of Calabria, Via P. Bucci, Cubo 15D, 87036 Rende, ItalyGrupo de Investigación en Salud Pública, Facultad de Ciencias de la Salud, Universidad Nacional de Chimborazo, Riobamba 060108, EcuadorLaboratorio Ciencias Biológicas, Facultad Recursos Naturales, Escuela Superior Politécnica de Chimborazo (ESPOCH), Riobamba 060155, EcuadorDipartimento di Chimica e Tecnologie Chimiche, University of Calabria, Via P. Bucci, Cubo 15D, 87036 Rende, ItalyFacultad de Ciencias, Escuela Superior Politécnica de Chimborazo (ESPOCH), Riobamba 060155, EcuadorINFN-Laboratori Nazionali di Frascati, Via E. Fermi 54, 00044 Frascati, ItalyThis study presents the optimization of two SPR biosensors, Sys<sub>3</sub> and Sys<sub>5</sub>, for SARS-CoV-2 detection at concentrations of 0.01–100 nM. Sys<sub>3</sub>, with a 55 nm silver layer, a 13 nm silicon nitride layer, and a 10 nm ssDNA layer, achieved a figure of merit (FoM) of 571.24 RIU<sup>−1</sup>, a signal-to-noise ratio (SNR) of 0.12, and a detection accuracy (DA) of 48.93 × 10<sup>−2</sup>. Sys<sub>5</sub>, incorporating a 50 nm silver layer, a 10 nm silicon nitride layer, a 10 nm ssDNA layer, and a 1.6 nm tungsten disulfide layer (L = 2), demonstrated a higher sensitivity of 305.33 °/RIU and a lower limit of detection (LoD) of 1.65 × 10<sup>−5</sup>. Sys<sub>3</sub> outshined in precision with low attenuation (<1%), while Sys<sub>5</sub> provided enhanced sensitivity and lower detection limits, crucial for early-stage viral detection. These configurations align with the refractive index ranges of clinical SARS-CoV-2 samples, showcasing their diagnostic potential. Future work will focus on experimental validation and integration into point-of-care platforms.https://www.mdpi.com/2072-666X/16/2/128surface plasmon resonancetungsten disulfidesilicon nitridessDNASARS-CoV-2biosensor
spellingShingle Talia Tene
Fabian Arias Arias
Karina I. Paredes-Páliz
Ana M. Cunachi Pillajo
Ana Gabriela Flores Huilcapi
Luis Santiago Carrera Almendariz
Stefano Bellucci
WS<sub>2</sub>/Si<sub>3</sub>N<sub>4</sub>-Based Biosensor for Low-Concentration Coronavirus Detection
Micromachines
surface plasmon resonance
tungsten disulfide
silicon nitride
ssDNA
SARS-CoV-2
biosensor
title WS<sub>2</sub>/Si<sub>3</sub>N<sub>4</sub>-Based Biosensor for Low-Concentration Coronavirus Detection
title_full WS<sub>2</sub>/Si<sub>3</sub>N<sub>4</sub>-Based Biosensor for Low-Concentration Coronavirus Detection
title_fullStr WS<sub>2</sub>/Si<sub>3</sub>N<sub>4</sub>-Based Biosensor for Low-Concentration Coronavirus Detection
title_full_unstemmed WS<sub>2</sub>/Si<sub>3</sub>N<sub>4</sub>-Based Biosensor for Low-Concentration Coronavirus Detection
title_short WS<sub>2</sub>/Si<sub>3</sub>N<sub>4</sub>-Based Biosensor for Low-Concentration Coronavirus Detection
title_sort ws sub 2 sub si sub 3 sub n sub 4 sub based biosensor for low concentration coronavirus detection
topic surface plasmon resonance
tungsten disulfide
silicon nitride
ssDNA
SARS-CoV-2
biosensor
url https://www.mdpi.com/2072-666X/16/2/128
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