Responsive cellulose nanocrystal‐based liquid crystals: From structural color manipulation to applications

Abstract Cellulose, one of the most versatile and abundant biopolymers in nature, has been employed by humans for thousands of years in diverse applications, such as renewable energy resources, structural materials, and fabric constituents. Cellulose nanocrystals (CNCs), obtained through the acidic...

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Main Authors: Jiao Liu, Ye‐Ming Qing, Jun‐Jie Wu, Jing‐Qi Tian, Chi‐Bo Feng, Xin‐Yu Zhou, Yun Ma, Bing‐Xiang Li, Yan‐Qing Lu, Quan Li
Format: Article
Language:English
Published: Wiley 2025-08-01
Series:Responsive Materials
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Online Access:https://doi.org/10.1002/rpm2.70020
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author Jiao Liu
Ye‐Ming Qing
Jun‐Jie Wu
Jing‐Qi Tian
Chi‐Bo Feng
Xin‐Yu Zhou
Yun Ma
Bing‐Xiang Li
Yan‐Qing Lu
Quan Li
author_facet Jiao Liu
Ye‐Ming Qing
Jun‐Jie Wu
Jing‐Qi Tian
Chi‐Bo Feng
Xin‐Yu Zhou
Yun Ma
Bing‐Xiang Li
Yan‐Qing Lu
Quan Li
author_sort Jiao Liu
collection DOAJ
description Abstract Cellulose, one of the most versatile and abundant biopolymers in nature, has been employed by humans for thousands of years in diverse applications, such as renewable energy resources, structural materials, and fabric constituents. Cellulose nanocrystals (CNCs), obtained through the acidic hydrolysis of cellulose‐based materials including wood, cotton, and additional sources, have attracted significant attention in areas, for example, energy storage, cosmetics, and medical devices. CNCs can spontaneously assemble into a cholesteric liquid crystal phase, which exhibits distinctive properties including biodegradability, high surface area, low cost, excellent mechanical strength, and surface functionality. Modifying the surfaces of CNCs or embedding CNCs with other materials enables novel cellulose‐based composites for advanced technologies and applications. This review systematically outlines the preparation of cellulose‐based liquid crystals (LCs), highlights the structural color regulation, photonic properties manipulation, and potential applications. Specifically, stimuli responsiveness, for example, temperature‐responsiveness, humidity‐responsiveness, pressure‐responsiveness, tension‐responsiveness, electricity‐responsiveness, magnetic force‐responsiveness and the optical properties of cellulose‐based LCs (circularly polarized light modulation and circularly polarized phosphorescence properties) are demonstrated. Furthermore, the applications of cellulose‐based LCs for gas detection, anticounterfeiting, multicolor separation, multifunctional E‐skin, and advanced fabrics are also reviewed. Finally, this review concludes with the remaining challenges and perspectives for unleashing new possibilities in the development of high‐performance multiple‐responsive cellulose‐based LCs.
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spelling doaj-art-e0e359061f6e46c5ba0bf36578a62fc52025-08-20T03:36:19ZengWileyResponsive Materials2834-89662025-08-0133n/an/a10.1002/rpm2.70020Responsive cellulose nanocrystal‐based liquid crystals: From structural color manipulation to applicationsJiao Liu0Ye‐Ming Qing1Jun‐Jie Wu2Jing‐Qi Tian3Chi‐Bo Feng4Xin‐Yu Zhou5Yun Ma6Bing‐Xiang Li7Yan‐Qing Lu8Quan Li9College of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology) Nanjing University of Posts and Telecommunications Nanjing ChinaCollege of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology) Nanjing University of Posts and Telecommunications Nanjing ChinaCollege of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology) Nanjing University of Posts and Telecommunications Nanjing ChinaCollege of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology) Nanjing University of Posts and Telecommunications Nanjing ChinaCollege of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology) Nanjing University of Posts and Telecommunications Nanjing ChinaCollege of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology) Nanjing University of Posts and Telecommunications Nanjing ChinaCollege of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology) Nanjing University of Posts and Telecommunications Nanjing ChinaCollege of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology) Nanjing University of Posts and Telecommunications Nanjing ChinaNational Laboratory of Solid State Microstructures & Collaborative Innovation Center of Advanced Microstructures & College of Engineering and Applied Sciences Nanjing University Nanjing ChinaInstitute of Advanced Materials & School of Chemistry and Chemical Engineering Southeast University Nanjing ChinaAbstract Cellulose, one of the most versatile and abundant biopolymers in nature, has been employed by humans for thousands of years in diverse applications, such as renewable energy resources, structural materials, and fabric constituents. Cellulose nanocrystals (CNCs), obtained through the acidic hydrolysis of cellulose‐based materials including wood, cotton, and additional sources, have attracted significant attention in areas, for example, energy storage, cosmetics, and medical devices. CNCs can spontaneously assemble into a cholesteric liquid crystal phase, which exhibits distinctive properties including biodegradability, high surface area, low cost, excellent mechanical strength, and surface functionality. Modifying the surfaces of CNCs or embedding CNCs with other materials enables novel cellulose‐based composites for advanced technologies and applications. This review systematically outlines the preparation of cellulose‐based liquid crystals (LCs), highlights the structural color regulation, photonic properties manipulation, and potential applications. Specifically, stimuli responsiveness, for example, temperature‐responsiveness, humidity‐responsiveness, pressure‐responsiveness, tension‐responsiveness, electricity‐responsiveness, magnetic force‐responsiveness and the optical properties of cellulose‐based LCs (circularly polarized light modulation and circularly polarized phosphorescence properties) are demonstrated. Furthermore, the applications of cellulose‐based LCs for gas detection, anticounterfeiting, multicolor separation, multifunctional E‐skin, and advanced fabrics are also reviewed. Finally, this review concludes with the remaining challenges and perspectives for unleashing new possibilities in the development of high‐performance multiple‐responsive cellulose‐based LCs.https://doi.org/10.1002/rpm2.70020cellulose nanocrystalcholesteric liquid crystalstimuli responsivestructural color
spellingShingle Jiao Liu
Ye‐Ming Qing
Jun‐Jie Wu
Jing‐Qi Tian
Chi‐Bo Feng
Xin‐Yu Zhou
Yun Ma
Bing‐Xiang Li
Yan‐Qing Lu
Quan Li
Responsive cellulose nanocrystal‐based liquid crystals: From structural color manipulation to applications
Responsive Materials
cellulose nanocrystal
cholesteric liquid crystal
stimuli responsive
structural color
title Responsive cellulose nanocrystal‐based liquid crystals: From structural color manipulation to applications
title_full Responsive cellulose nanocrystal‐based liquid crystals: From structural color manipulation to applications
title_fullStr Responsive cellulose nanocrystal‐based liquid crystals: From structural color manipulation to applications
title_full_unstemmed Responsive cellulose nanocrystal‐based liquid crystals: From structural color manipulation to applications
title_short Responsive cellulose nanocrystal‐based liquid crystals: From structural color manipulation to applications
title_sort responsive cellulose nanocrystal based liquid crystals from structural color manipulation to applications
topic cellulose nanocrystal
cholesteric liquid crystal
stimuli responsive
structural color
url https://doi.org/10.1002/rpm2.70020
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