Novel PLA-Henna composite for sustainable tertiary enhanced oil recovery

Abstract Enhanced oil recovery (EOR) remains a critical focus for the petroleum industry, aiming to overcome the challenges of residual oil mobilization and maximize hydrocarbon recovery in increasingly complex reservoirs. This study introduces an innovative approach using synthesized Polylactic Aci...

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Main Authors: Tariq Alkhrissat, Ali Raqee Abdulhadi, Muntadar Muhsen, Jasgurpreet Singh Chohan, M. K. Ranganathaswamy, Premananda Pradhan, Parveen Kumar, Gauri Chauhan, Ahmad Abumalek
Format: Article
Language:English
Published: Nature Portfolio 2025-08-01
Series:Scientific Reports
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Online Access:https://doi.org/10.1038/s41598-025-15660-y
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author Tariq Alkhrissat
Ali Raqee Abdulhadi
Muntadar Muhsen
Jasgurpreet Singh Chohan
M. K. Ranganathaswamy
Premananda Pradhan
Parveen Kumar
Gauri Chauhan
Ahmad Abumalek
author_facet Tariq Alkhrissat
Ali Raqee Abdulhadi
Muntadar Muhsen
Jasgurpreet Singh Chohan
M. K. Ranganathaswamy
Premananda Pradhan
Parveen Kumar
Gauri Chauhan
Ahmad Abumalek
author_sort Tariq Alkhrissat
collection DOAJ
description Abstract Enhanced oil recovery (EOR) remains a critical focus for the petroleum industry, aiming to overcome the challenges of residual oil mobilization and maximize hydrocarbon recovery in increasingly complex reservoirs. This study introduces an innovative approach using synthesized Polylactic Acid (PLA)/Henna composites as an environmentally sustainable additive to enhance oil recovery through mechanisms such as interfacial tension (IFT) reduction, wettability alteration, and physical sweeping for improved fluid sweep efficiency. The composite was synthesized using extrusion techniques to ensure a uniform filler dispersion and was extensively characterized through FTIR, SEM, and EDS analyses. Brines, including seawater (SW), formation water (FW), and PLA-Henna-modified SW, were formulated to simulate actual reservoir conditions. Experimental analyses included IFT measurement using the pendant drop method, wettability studies using contact angle measurements, and core flooding experiments to assess EOR performance. Experimental findings revealed that the optimal PLA-Henna concentration was 2 wt%, which achieved significant IFT reductions (to 27 mN/m in SW). The composite also altered rock wettability from oil-wet to water-wet with pronounced effects in SW brine, where contact angles reduced from 142 to 89°. Core flooding experiments highlighted an increase in oil recovery factors, with PLA-Henna-modified SW yielding the highest recovery (85%) compared to FW (49.7%) or SW (61%). These advancements emphasize PLA/Henna composites’ potential for sustainable EOR applications, ensuring improved recovery outcomes while utilizing biodegradable, eco-friendly materials.
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spelling doaj-art-e0698991fbff4e468adb0f7c3ef784922025-08-24T11:26:54ZengNature PortfolioScientific Reports2045-23222025-08-0115111610.1038/s41598-025-15660-yNovel PLA-Henna composite for sustainable tertiary enhanced oil recoveryTariq Alkhrissat0Ali Raqee Abdulhadi1Muntadar Muhsen2Jasgurpreet Singh Chohan3M. K. Ranganathaswamy4Premananda Pradhan5Parveen Kumar6Gauri Chauhan7Ahmad Abumalek8Faculty of Engineering, Hourani Center for Applied Scientific Research, Al-Ahliyya Amman UniversityMechanical Engineering Department, Al-Turath UniversityDepartment of Structurals Techniques Engineering, College of Technical Engineering, The Islamic UniversityUniversity School of Mechanical Engineering, Rayat Bahra UniversityDepartment of Mechanical Engineering, School of Engineering and Technology, JAIN (Deemed to be University)Department of Mechanical Engineering, Siksha ‘O’ Anusandhan (Deemed to be University)Department of Mechanical Engineering, Chandigarh Engineering College, Chandigarh Group of Colleges-JhanjeriCentre for Research Impact & Outcome, Chitkara University Institute of Engineering and Technology, Chitkara UniversityFaculty of Engineering, Balkh UniversityAbstract Enhanced oil recovery (EOR) remains a critical focus for the petroleum industry, aiming to overcome the challenges of residual oil mobilization and maximize hydrocarbon recovery in increasingly complex reservoirs. This study introduces an innovative approach using synthesized Polylactic Acid (PLA)/Henna composites as an environmentally sustainable additive to enhance oil recovery through mechanisms such as interfacial tension (IFT) reduction, wettability alteration, and physical sweeping for improved fluid sweep efficiency. The composite was synthesized using extrusion techniques to ensure a uniform filler dispersion and was extensively characterized through FTIR, SEM, and EDS analyses. Brines, including seawater (SW), formation water (FW), and PLA-Henna-modified SW, were formulated to simulate actual reservoir conditions. Experimental analyses included IFT measurement using the pendant drop method, wettability studies using contact angle measurements, and core flooding experiments to assess EOR performance. Experimental findings revealed that the optimal PLA-Henna concentration was 2 wt%, which achieved significant IFT reductions (to 27 mN/m in SW). The composite also altered rock wettability from oil-wet to water-wet with pronounced effects in SW brine, where contact angles reduced from 142 to 89°. Core flooding experiments highlighted an increase in oil recovery factors, with PLA-Henna-modified SW yielding the highest recovery (85%) compared to FW (49.7%) or SW (61%). These advancements emphasize PLA/Henna composites’ potential for sustainable EOR applications, ensuring improved recovery outcomes while utilizing biodegradable, eco-friendly materials.https://doi.org/10.1038/s41598-025-15660-yEnhanced oil recoveryPLA/HennaInterfacial tensionWettability alterationCore flooding
spellingShingle Tariq Alkhrissat
Ali Raqee Abdulhadi
Muntadar Muhsen
Jasgurpreet Singh Chohan
M. K. Ranganathaswamy
Premananda Pradhan
Parveen Kumar
Gauri Chauhan
Ahmad Abumalek
Novel PLA-Henna composite for sustainable tertiary enhanced oil recovery
Scientific Reports
Enhanced oil recovery
PLA/Henna
Interfacial tension
Wettability alteration
Core flooding
title Novel PLA-Henna composite for sustainable tertiary enhanced oil recovery
title_full Novel PLA-Henna composite for sustainable tertiary enhanced oil recovery
title_fullStr Novel PLA-Henna composite for sustainable tertiary enhanced oil recovery
title_full_unstemmed Novel PLA-Henna composite for sustainable tertiary enhanced oil recovery
title_short Novel PLA-Henna composite for sustainable tertiary enhanced oil recovery
title_sort novel pla henna composite for sustainable tertiary enhanced oil recovery
topic Enhanced oil recovery
PLA/Henna
Interfacial tension
Wettability alteration
Core flooding
url https://doi.org/10.1038/s41598-025-15660-y
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