Conductivity and Dielectric Studies of Lithium Trifluoromethanesulfonate Doped Polyethylene Oxide-Graphene Oxide Blend Based Electrolytes

Series of polymer blend consisting of polyethylene oxide (PEO) and graphene oxide (GO) as co-host polymer were prepared using solution cast method. The most amorphous PEO-GO blend was obtained using 90 wt.% of PEO and 10 wt.% of GO as recorded by X-ray diffraction (XRD). Fourier transform infrared s...

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Main Authors: A. A. Azli, N. S. A. Manan, M. F. Z. Kadir
Format: Article
Language:English
Published: Wiley 2015-01-01
Series:Advances in Materials Science and Engineering
Online Access:http://dx.doi.org/10.1155/2015/145735
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author A. A. Azli
N. S. A. Manan
M. F. Z. Kadir
author_facet A. A. Azli
N. S. A. Manan
M. F. Z. Kadir
author_sort A. A. Azli
collection DOAJ
description Series of polymer blend consisting of polyethylene oxide (PEO) and graphene oxide (GO) as co-host polymer were prepared using solution cast method. The most amorphous PEO-GO blend was obtained using 90 wt.% of PEO and 10 wt.% of GO as recorded by X-ray diffraction (XRD). Fourier transform infrared spectroscopy (FTIR) analysis proved the interaction between PEO, GO, lithium trifluoromethanesulfonate (LiCF3SO3), and ethylene sulfite (ES). Incorporation of 25 wt.% LiCF3SO3 into the PEO-GO blend increases the conductivity to 3.84±0.83×10-6 S cm−1. The conductivity starts to decrease when more than 25 wt.% salt is doped into the polymer blend. The addition of 1 wt.% ES into the polymer electrolyte has increased the conductivity to 1.73±0.05×10-5 S cm−1. Dielectric studies show that all the electrolytes obey non-Debye behavior.
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spelling doaj-art-e018cfd0b55b48e8bc0bc3286dd06bab2025-08-20T02:21:07ZengWileyAdvances in Materials Science and Engineering1687-84341687-84422015-01-01201510.1155/2015/145735145735Conductivity and Dielectric Studies of Lithium Trifluoromethanesulfonate Doped Polyethylene Oxide-Graphene Oxide Blend Based ElectrolytesA. A. Azli0N. S. A. Manan1M. F. Z. Kadir2Institute of Graduate Studies, University of Malaya, 50603 Kuala Lumpur, MalaysiaChemistry Department, Faculty of Science, University of Malaya, 50603 Kuala Lumpur, MalaysiaCentre for Foundation Studies in Science, University of Malaya, 50603 Kuala Lumpur, MalaysiaSeries of polymer blend consisting of polyethylene oxide (PEO) and graphene oxide (GO) as co-host polymer were prepared using solution cast method. The most amorphous PEO-GO blend was obtained using 90 wt.% of PEO and 10 wt.% of GO as recorded by X-ray diffraction (XRD). Fourier transform infrared spectroscopy (FTIR) analysis proved the interaction between PEO, GO, lithium trifluoromethanesulfonate (LiCF3SO3), and ethylene sulfite (ES). Incorporation of 25 wt.% LiCF3SO3 into the PEO-GO blend increases the conductivity to 3.84±0.83×10-6 S cm−1. The conductivity starts to decrease when more than 25 wt.% salt is doped into the polymer blend. The addition of 1 wt.% ES into the polymer electrolyte has increased the conductivity to 1.73±0.05×10-5 S cm−1. Dielectric studies show that all the electrolytes obey non-Debye behavior.http://dx.doi.org/10.1155/2015/145735
spellingShingle A. A. Azli
N. S. A. Manan
M. F. Z. Kadir
Conductivity and Dielectric Studies of Lithium Trifluoromethanesulfonate Doped Polyethylene Oxide-Graphene Oxide Blend Based Electrolytes
Advances in Materials Science and Engineering
title Conductivity and Dielectric Studies of Lithium Trifluoromethanesulfonate Doped Polyethylene Oxide-Graphene Oxide Blend Based Electrolytes
title_full Conductivity and Dielectric Studies of Lithium Trifluoromethanesulfonate Doped Polyethylene Oxide-Graphene Oxide Blend Based Electrolytes
title_fullStr Conductivity and Dielectric Studies of Lithium Trifluoromethanesulfonate Doped Polyethylene Oxide-Graphene Oxide Blend Based Electrolytes
title_full_unstemmed Conductivity and Dielectric Studies of Lithium Trifluoromethanesulfonate Doped Polyethylene Oxide-Graphene Oxide Blend Based Electrolytes
title_short Conductivity and Dielectric Studies of Lithium Trifluoromethanesulfonate Doped Polyethylene Oxide-Graphene Oxide Blend Based Electrolytes
title_sort conductivity and dielectric studies of lithium trifluoromethanesulfonate doped polyethylene oxide graphene oxide blend based electrolytes
url http://dx.doi.org/10.1155/2015/145735
work_keys_str_mv AT aaazli conductivityanddielectricstudiesoflithiumtrifluoromethanesulfonatedopedpolyethyleneoxidegrapheneoxideblendbasedelectrolytes
AT nsamanan conductivityanddielectricstudiesoflithiumtrifluoromethanesulfonatedopedpolyethyleneoxidegrapheneoxideblendbasedelectrolytes
AT mfzkadir conductivityanddielectricstudiesoflithiumtrifluoromethanesulfonatedopedpolyethyleneoxidegrapheneoxideblendbasedelectrolytes