Segregation of Cu-In-S Elements in the Spray-Pyrolysis-Deposited Layer of CIS Solar Cells

We report the fabrication of superstrate-structured solar cells by the deposition of Cu-In-S (CIS) films on 〈glass/FTO/TiO2/In2S3〉 under air by spray pyrolysis. The cells had an open-circuit voltage of 0.551 V, a photocurrent density of 9.5 mA/cm2, a fill factor of 0.45, and a conversion efficiency...

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Main Authors: Seigo Ito, Toshihiro Ryo
Format: Article
Language:English
Published: Wiley 2012-01-01
Series:Advances in Materials Science and Engineering
Online Access:http://dx.doi.org/10.1155/2012/136092
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author Seigo Ito
Toshihiro Ryo
author_facet Seigo Ito
Toshihiro Ryo
author_sort Seigo Ito
collection DOAJ
description We report the fabrication of superstrate-structured solar cells by the deposition of Cu-In-S (CIS) films on 〈glass/FTO/TiO2/In2S3〉 under air by spray pyrolysis. The cells had an open-circuit voltage of 0.551 V, a photocurrent density of 9.5 mA/cm2, a fill factor of 0.45, and a conversion efficiency of 2.14%. However, transmission electron microscopy/energy dispersive X-ray (TEM-EDX) analysis revealed significant differences between the atomic ratio of the setting material in the spray-deposition solution and the elements in the layer. Moreover, TEM-EDX measurements suggested strong segregation of the Cu-In-S elements in the spray-pyrolysis-deposited layer. The degree of segregation depended on the substrate (〈glass〉, 〈glass/TiO2〉, or 〈glass/TiO2/In2S3〉), although Cu3In5S9 nanoparticles were segregated in the sulfur layer.
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institution Kabale University
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spelling doaj-art-e0074d4f8c7d443f9d2e6677e52bf6dc2025-08-20T03:24:36ZengWileyAdvances in Materials Science and Engineering1687-84341687-84422012-01-01201210.1155/2012/136092136092Segregation of Cu-In-S Elements in the Spray-Pyrolysis-Deposited Layer of CIS Solar CellsSeigo Ito0Toshihiro Ryo1Department of Electric Engineering and Computer Sciences and Department of Materials Science and Chemistry, University of Hyogo, 2167 Shosha, Himeji, Hyogo 671-2280, JapanDepartment of Electric Engineering and Computer Sciences and Department of Materials Science and Chemistry, University of Hyogo, 2167 Shosha, Himeji, Hyogo 671-2280, JapanWe report the fabrication of superstrate-structured solar cells by the deposition of Cu-In-S (CIS) films on 〈glass/FTO/TiO2/In2S3〉 under air by spray pyrolysis. The cells had an open-circuit voltage of 0.551 V, a photocurrent density of 9.5 mA/cm2, a fill factor of 0.45, and a conversion efficiency of 2.14%. However, transmission electron microscopy/energy dispersive X-ray (TEM-EDX) analysis revealed significant differences between the atomic ratio of the setting material in the spray-deposition solution and the elements in the layer. Moreover, TEM-EDX measurements suggested strong segregation of the Cu-In-S elements in the spray-pyrolysis-deposited layer. The degree of segregation depended on the substrate (〈glass〉, 〈glass/TiO2〉, or 〈glass/TiO2/In2S3〉), although Cu3In5S9 nanoparticles were segregated in the sulfur layer.http://dx.doi.org/10.1155/2012/136092
spellingShingle Seigo Ito
Toshihiro Ryo
Segregation of Cu-In-S Elements in the Spray-Pyrolysis-Deposited Layer of CIS Solar Cells
Advances in Materials Science and Engineering
title Segregation of Cu-In-S Elements in the Spray-Pyrolysis-Deposited Layer of CIS Solar Cells
title_full Segregation of Cu-In-S Elements in the Spray-Pyrolysis-Deposited Layer of CIS Solar Cells
title_fullStr Segregation of Cu-In-S Elements in the Spray-Pyrolysis-Deposited Layer of CIS Solar Cells
title_full_unstemmed Segregation of Cu-In-S Elements in the Spray-Pyrolysis-Deposited Layer of CIS Solar Cells
title_short Segregation of Cu-In-S Elements in the Spray-Pyrolysis-Deposited Layer of CIS Solar Cells
title_sort segregation of cu in s elements in the spray pyrolysis deposited layer of cis solar cells
url http://dx.doi.org/10.1155/2012/136092
work_keys_str_mv AT seigoito segregationofcuinselementsinthespraypyrolysisdepositedlayerofcissolarcells
AT toshihiroryo segregationofcuinselementsinthespraypyrolysisdepositedlayerofcissolarcells