Homogeneous Esterification of Cellulose in the Mixture N-Butylpyridinium Chloride/Dimethylsulfoxide

The present study deals with the homogeneous acylation of cellulose with p-nitrobenzoyl chloride in a reaction medium composed of a mixture of 1-butylpyridinium chloride and dimethylsulfoxide (BPyCl/DMSO), in the presence of different bases and under mild conditions. The preparation of cellulose p-n...

Full description

Saved in:
Bibliographic Details
Main Authors: Lahcen El Hamdaoui, Mohammed El Moussaouiti, Said Gmouh
Format: Article
Language:English
Published: Wiley 2016-01-01
Series:International Journal of Polymer Science
Online Access:http://dx.doi.org/10.1155/2016/1756971
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849467390303141888
author Lahcen El Hamdaoui
Mohammed El Moussaouiti
Said Gmouh
author_facet Lahcen El Hamdaoui
Mohammed El Moussaouiti
Said Gmouh
author_sort Lahcen El Hamdaoui
collection DOAJ
description The present study deals with the homogeneous acylation of cellulose with p-nitrobenzoyl chloride in a reaction medium composed of a mixture of 1-butylpyridinium chloride and dimethylsulfoxide (BPyCl/DMSO), in the presence of different bases and under mild conditions. The preparation of cellulose p-nitrobenzoate depending on the reaction conditions, the influences of reaction parameters such as the base type, and the types of cellulose (kraft and microcrystalline) on the products were investigated. Cellulose p-nitrobenzoate with a degree of substitution (DS) in the range from 0.12 to 1.5 was accessible, with a low excess of reagent and for a short reaction time. The cellulose esters were characterized by 1H-NMR, 13C NMR, and FT-IR spectroscopy, thermogravimetric analysis (TGA), scanning electron microscopy (SEM), and solubility tests.
format Article
id doaj-art-debde96832a540d6a1cb4abd22aa0377
institution Kabale University
issn 1687-9422
1687-9430
language English
publishDate 2016-01-01
publisher Wiley
record_format Article
series International Journal of Polymer Science
spelling doaj-art-debde96832a540d6a1cb4abd22aa03772025-08-20T03:26:15ZengWileyInternational Journal of Polymer Science1687-94221687-94302016-01-01201610.1155/2016/17569711756971Homogeneous Esterification of Cellulose in the Mixture N-Butylpyridinium Chloride/DimethylsulfoxideLahcen El Hamdaoui0Mohammed El Moussaouiti1Said Gmouh2Laboratory of Materials Nanomaterials and Environment, Faculty of Sciences, University Mohammed V, Rabat, MoroccoLaboratory of Materials Nanomaterials and Environment, Faculty of Sciences, University Mohammed V, Rabat, MoroccoNational Center for Scientific Research and Technique, Rabat, MoroccoThe present study deals with the homogeneous acylation of cellulose with p-nitrobenzoyl chloride in a reaction medium composed of a mixture of 1-butylpyridinium chloride and dimethylsulfoxide (BPyCl/DMSO), in the presence of different bases and under mild conditions. The preparation of cellulose p-nitrobenzoate depending on the reaction conditions, the influences of reaction parameters such as the base type, and the types of cellulose (kraft and microcrystalline) on the products were investigated. Cellulose p-nitrobenzoate with a degree of substitution (DS) in the range from 0.12 to 1.5 was accessible, with a low excess of reagent and for a short reaction time. The cellulose esters were characterized by 1H-NMR, 13C NMR, and FT-IR spectroscopy, thermogravimetric analysis (TGA), scanning electron microscopy (SEM), and solubility tests.http://dx.doi.org/10.1155/2016/1756971
spellingShingle Lahcen El Hamdaoui
Mohammed El Moussaouiti
Said Gmouh
Homogeneous Esterification of Cellulose in the Mixture N-Butylpyridinium Chloride/Dimethylsulfoxide
International Journal of Polymer Science
title Homogeneous Esterification of Cellulose in the Mixture N-Butylpyridinium Chloride/Dimethylsulfoxide
title_full Homogeneous Esterification of Cellulose in the Mixture N-Butylpyridinium Chloride/Dimethylsulfoxide
title_fullStr Homogeneous Esterification of Cellulose in the Mixture N-Butylpyridinium Chloride/Dimethylsulfoxide
title_full_unstemmed Homogeneous Esterification of Cellulose in the Mixture N-Butylpyridinium Chloride/Dimethylsulfoxide
title_short Homogeneous Esterification of Cellulose in the Mixture N-Butylpyridinium Chloride/Dimethylsulfoxide
title_sort homogeneous esterification of cellulose in the mixture n butylpyridinium chloride dimethylsulfoxide
url http://dx.doi.org/10.1155/2016/1756971
work_keys_str_mv AT lahcenelhamdaoui homogeneousesterificationofcelluloseinthemixturenbutylpyridiniumchloridedimethylsulfoxide
AT mohammedelmoussaouiti homogeneousesterificationofcelluloseinthemixturenbutylpyridiniumchloridedimethylsulfoxide
AT saidgmouh homogeneousesterificationofcelluloseinthemixturenbutylpyridiniumchloridedimethylsulfoxide