Low-temperature carburizing improves hydrogen embrittlement resistance of cold worked 304 austenitic stainless steel

Cold deformation-induced martensitic transformation in 304 austenitic stainless steel (ASS) increases its susceptibility to hydrogen embrittlement (HE). In this study, low-temperature carburizing (LTC) was performed on cold worked 304 ASS. Its effect on the mechanical properties and HE was investiga...

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Main Authors: Xiao Qin, Lars Nyborg, Huiqun Liu, Alexandra Bauer, Yu Cao
Format: Article
Language:English
Published: Elsevier 2025-05-01
Series:Journal of Materials Research and Technology
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Online Access:http://www.sciencedirect.com/science/article/pii/S2238785425012803
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author Xiao Qin
Lars Nyborg
Huiqun Liu
Alexandra Bauer
Yu Cao
author_facet Xiao Qin
Lars Nyborg
Huiqun Liu
Alexandra Bauer
Yu Cao
author_sort Xiao Qin
collection DOAJ
description Cold deformation-induced martensitic transformation in 304 austenitic stainless steel (ASS) increases its susceptibility to hydrogen embrittlement (HE). In this study, low-temperature carburizing (LTC) was performed on cold worked 304 ASS. Its effect on the mechanical properties and HE was investigated by electrochemical cathodic hydrogen charging and slow strain rate tensile test. Microstructure, fractography, and hydrogen uptake were analyzed to examine the hydrogen-induced failure. It has been found that LTC introduced the expanded austenite on the steel surface, which increased strength and surface hardness but reduced the elongation. LTC increased the initial strain hardening rate and suppressed strain-induced martensitic transformation, showing higher strain rate sensitivity. Hydrogen uptake caused loss of ductility and formation of a quasi-cleavage layer with some cracks on the surface of the steel. The HE resistance was significantly improved by LTC treatment. Cold-worked 304 showed a higher HE index due to the martensitic transformation and a higher hydrogen concentration. The remarkably reduced susceptibility to HE by LTC treatment was attributed to the carbon stabilized austenite and consequently inhibited martensite transformation, as well as compressive stress in the expanded austenite. These factors reduce hydrogen diffusion and hydrogen uptake.
format Article
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institution OA Journals
issn 2238-7854
language English
publishDate 2025-05-01
publisher Elsevier
record_format Article
series Journal of Materials Research and Technology
spelling doaj-art-de0c170c07e341aba7cd34adce2728442025-08-20T01:55:31ZengElsevierJournal of Materials Research and Technology2238-78542025-05-01368816882510.1016/j.jmrt.2025.05.125Low-temperature carburizing improves hydrogen embrittlement resistance of cold worked 304 austenitic stainless steelXiao Qin0Lars Nyborg1Huiqun Liu2Alexandra Bauer3Yu Cao4Department of Industrial and Materials Science, Chalmers University of Technology, Gothenburg, 41296, Sweden; School of Materials Science and Engineering, Central South University, Changsha, 410083, PR ChinaDepartment of Industrial and Materials Science, Chalmers University of Technology, Gothenburg, 41296, SwedenSchool of Materials Science and Engineering, Central South University, Changsha, 410083, PR ChinaBodycote Specialist Technologies GmbH, 86899, Landsberg, GermanyDepartment of Industrial and Materials Science, Chalmers University of Technology, Gothenburg, 41296, Sweden; Corresponding author.Cold deformation-induced martensitic transformation in 304 austenitic stainless steel (ASS) increases its susceptibility to hydrogen embrittlement (HE). In this study, low-temperature carburizing (LTC) was performed on cold worked 304 ASS. Its effect on the mechanical properties and HE was investigated by electrochemical cathodic hydrogen charging and slow strain rate tensile test. Microstructure, fractography, and hydrogen uptake were analyzed to examine the hydrogen-induced failure. It has been found that LTC introduced the expanded austenite on the steel surface, which increased strength and surface hardness but reduced the elongation. LTC increased the initial strain hardening rate and suppressed strain-induced martensitic transformation, showing higher strain rate sensitivity. Hydrogen uptake caused loss of ductility and formation of a quasi-cleavage layer with some cracks on the surface of the steel. The HE resistance was significantly improved by LTC treatment. Cold-worked 304 showed a higher HE index due to the martensitic transformation and a higher hydrogen concentration. The remarkably reduced susceptibility to HE by LTC treatment was attributed to the carbon stabilized austenite and consequently inhibited martensite transformation, as well as compressive stress in the expanded austenite. These factors reduce hydrogen diffusion and hydrogen uptake.http://www.sciencedirect.com/science/article/pii/S2238785425012803Low-temperature carburizingAustenitic stainless steelHydrogen embrittlementExpanded austenite
spellingShingle Xiao Qin
Lars Nyborg
Huiqun Liu
Alexandra Bauer
Yu Cao
Low-temperature carburizing improves hydrogen embrittlement resistance of cold worked 304 austenitic stainless steel
Journal of Materials Research and Technology
Low-temperature carburizing
Austenitic stainless steel
Hydrogen embrittlement
Expanded austenite
title Low-temperature carburizing improves hydrogen embrittlement resistance of cold worked 304 austenitic stainless steel
title_full Low-temperature carburizing improves hydrogen embrittlement resistance of cold worked 304 austenitic stainless steel
title_fullStr Low-temperature carburizing improves hydrogen embrittlement resistance of cold worked 304 austenitic stainless steel
title_full_unstemmed Low-temperature carburizing improves hydrogen embrittlement resistance of cold worked 304 austenitic stainless steel
title_short Low-temperature carburizing improves hydrogen embrittlement resistance of cold worked 304 austenitic stainless steel
title_sort low temperature carburizing improves hydrogen embrittlement resistance of cold worked 304 austenitic stainless steel
topic Low-temperature carburizing
Austenitic stainless steel
Hydrogen embrittlement
Expanded austenite
url http://www.sciencedirect.com/science/article/pii/S2238785425012803
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AT larsnyborg lowtemperaturecarburizingimproveshydrogenembrittlementresistanceofcoldworked304austeniticstainlesssteel
AT huiqunliu lowtemperaturecarburizingimproveshydrogenembrittlementresistanceofcoldworked304austeniticstainlesssteel
AT alexandrabauer lowtemperaturecarburizingimproveshydrogenembrittlementresistanceofcoldworked304austeniticstainlesssteel
AT yucao lowtemperaturecarburizingimproveshydrogenembrittlementresistanceofcoldworked304austeniticstainlesssteel