Immobilization of peroxidase from fresh horseradish extract for anthraquinone dye decolorization

Synthetic dyes are used in all sectors of industry and represent a serious ecological problem. By the presence, anthraquinone dyes are right after the azo dyes. Unlike azo, anthraquinone dyes are considerably harder to degrade due to the presence of coupled aromatic rings in their structure. Horsera...

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Main Authors: Nataša Ž. Šekuljica, Nevena Ž. Prlainović, Nevena M. Lukić, Aleksandra M. Jakovljević, Sanja Ž. Grbavčić, Dušan Ž. Mijin, Jugović Zorica D. Knežević
Format: Article
Language:English
Published: Engineering Society for Corrosion, Belgrade 2015-09-01
Series:Zaštita Materijala
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Online Access:https://www.zastita-materijala.org/index.php/home/article/view/812
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author Nataša Ž. Šekuljica
Nevena Ž. Prlainović
Nevena M. Lukić
Aleksandra M. Jakovljević
Sanja Ž. Grbavčić
Dušan Ž. Mijin
Jugović Zorica D. Knežević
author_facet Nataša Ž. Šekuljica
Nevena Ž. Prlainović
Nevena M. Lukić
Aleksandra M. Jakovljević
Sanja Ž. Grbavčić
Dušan Ž. Mijin
Jugović Zorica D. Knežević
author_sort Nataša Ž. Šekuljica
collection DOAJ
description Synthetic dyes are used in all sectors of industry and represent a serious ecological problem. By the presence, anthraquinone dyes are right after the azo dyes. Unlike azo, anthraquinone dyes are considerably harder to degrade due to the presence of coupled aromatic rings in their structure. Horseradish peroxidase (HRP) proved to be an efficient and ecologically acceptable solution for synthetic dyes decolonization. For that reason, feasibility of peroxidase from fresh horseradish extract application in anthraquinone dye decolonization was the object of this research. Unpurified peroxidase (1.5 mg mL-1), was immobilized onto fumed silica by adsorption. In order to optimize the decolonization of anthraquinone dye Acid Violet 109 (AV 109) 0.1 IU of obtained immobilized HRP was applied in a batch reactor. Under the optimal conditions (pH 4.0, dye concentration 30 mg L-1, hydrogen peroxide concentration 0.1 mM) 55.1 % of initial dye concentration was decolorized, within 30 min. In addition, compared to free enzyme, immobilized HRP showed higher resistance towards inhibitory influence of the dye and hydrogen peroxide.
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record_format Article
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spelling doaj-art-ddaf2145a5ee46439fcd382b4fb0e20c2025-08-20T02:21:30ZengEngineering Society for Corrosion, BelgradeZaštita Materijala0351-94652466-25852015-09-0156333533910.5937/ZasMat1503335S811Immobilization of peroxidase from fresh horseradish extract for anthraquinone dye decolorizationNataša Ž. Šekuljica0Nevena Ž. Prlainović1Nevena M. Lukić2Aleksandra M. Jakovljević3Sanja Ž. Grbavčić4Dušan Ž. Mijin5Jugović Zorica D. Knežević6University of Belgrade, Faculty of Technology and Metallurgy, SerbiaUniversity of Belgrade, Faculty of Technology and Metallurgy, SerbiaUniversity of Belgrade, Faculty of Technology and Metallurgy, SerbiaUniversity of Belgrade, Faculty of Technology and Metallurgy, SerbiaUniversity of Belgrade, Faculty of Technology and Metallurgy, SerbiaUniversity of Belgrade, Faculty of Technology and Metallurgy, SerbiaUniversity of Belgrade, Faculty of Technology and Metallurgy, SerbiaSynthetic dyes are used in all sectors of industry and represent a serious ecological problem. By the presence, anthraquinone dyes are right after the azo dyes. Unlike azo, anthraquinone dyes are considerably harder to degrade due to the presence of coupled aromatic rings in their structure. Horseradish peroxidase (HRP) proved to be an efficient and ecologically acceptable solution for synthetic dyes decolonization. For that reason, feasibility of peroxidase from fresh horseradish extract application in anthraquinone dye decolonization was the object of this research. Unpurified peroxidase (1.5 mg mL-1), was immobilized onto fumed silica by adsorption. In order to optimize the decolonization of anthraquinone dye Acid Violet 109 (AV 109) 0.1 IU of obtained immobilized HRP was applied in a batch reactor. Under the optimal conditions (pH 4.0, dye concentration 30 mg L-1, hydrogen peroxide concentration 0.1 mM) 55.1 % of initial dye concentration was decolorized, within 30 min. In addition, compared to free enzyme, immobilized HRP showed higher resistance towards inhibitory influence of the dye and hydrogen peroxide.https://www.zastita-materijala.org/index.php/home/article/view/812horseradish peroxidaseimmobilizationdyewastewater
spellingShingle Nataša Ž. Šekuljica
Nevena Ž. Prlainović
Nevena M. Lukić
Aleksandra M. Jakovljević
Sanja Ž. Grbavčić
Dušan Ž. Mijin
Jugović Zorica D. Knežević
Immobilization of peroxidase from fresh horseradish extract for anthraquinone dye decolorization
Zaštita Materijala
horseradish peroxidase
immobilization
dye
wastewater
title Immobilization of peroxidase from fresh horseradish extract for anthraquinone dye decolorization
title_full Immobilization of peroxidase from fresh horseradish extract for anthraquinone dye decolorization
title_fullStr Immobilization of peroxidase from fresh horseradish extract for anthraquinone dye decolorization
title_full_unstemmed Immobilization of peroxidase from fresh horseradish extract for anthraquinone dye decolorization
title_short Immobilization of peroxidase from fresh horseradish extract for anthraquinone dye decolorization
title_sort immobilization of peroxidase from fresh horseradish extract for anthraquinone dye decolorization
topic horseradish peroxidase
immobilization
dye
wastewater
url https://www.zastita-materijala.org/index.php/home/article/view/812
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AT nevenazprlainovic immobilizationofperoxidasefromfreshhorseradishextractforanthraquinonedyedecolorization
AT nevenamlukic immobilizationofperoxidasefromfreshhorseradishextractforanthraquinonedyedecolorization
AT aleksandramjakovljevic immobilizationofperoxidasefromfreshhorseradishextractforanthraquinonedyedecolorization
AT sanjazgrbavcic immobilizationofperoxidasefromfreshhorseradishextractforanthraquinonedyedecolorization
AT dusanzmijin immobilizationofperoxidasefromfreshhorseradishextractforanthraquinonedyedecolorization
AT jugoviczoricadknezevic immobilizationofperoxidasefromfreshhorseradishextractforanthraquinonedyedecolorization