Hydrogen Production from Wastewater Degradation on a Rotating Hole-Arranged Boron-Doped Diamond Anode

An electrochemical system using a rotating hole-arranged boron-doped diamond (HABDD) film anode was designed for wastewater degradation. Meanwhile, in a reciprocal process, a foam nickel (FNi) cathode was employed for hydrogen evolution using the ions liberated from the HABDD. The HABDD was custom-m...

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Main Authors: Daibing Luo, Yong Luo, Daichuan Ma
Format: Article
Language:English
Published: MDPI AG 2024-12-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/14/23/11284
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author Daibing Luo
Yong Luo
Daichuan Ma
author_facet Daibing Luo
Yong Luo
Daichuan Ma
author_sort Daibing Luo
collection DOAJ
description An electrochemical system using a rotating hole-arranged boron-doped diamond (HABDD) film anode was designed for wastewater degradation. Meanwhile, in a reciprocal process, a foam nickel (FNi) cathode was employed for hydrogen evolution using the ions liberated from the HABDD. The HABDD was custom-made using an MWCVD device and characterized by SEM, Raman and electrochemical measurement. Some wastewater was tested on the HABDD anode to examine its electrochemical performance. The efficiency of the electrochemical system was evaluated by COD removal rate and hydrogen production yields. The influence of the rotating and flowing rates of the electrolyte on electrochemical performance was discussed. The rotating HABDD with dynamic three-dimensional flowing paths provided a high mass transfer, which promoted the overall performance of the wastewater mineralization. Meanwhile, the ions released from the anode to the cathode improved the hydrogen generation performance on the cathode. The hydrogen production efficiency in relation to the electrochemical oxidation process was studied in terms of the COD change and treatment time.
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institution DOAJ
issn 2076-3417
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publishDate 2024-12-01
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record_format Article
series Applied Sciences
spelling doaj-art-db1d42160902431ea302ef5e6e7719792025-08-20T02:50:13ZengMDPI AGApplied Sciences2076-34172024-12-0114231128410.3390/app142311284Hydrogen Production from Wastewater Degradation on a Rotating Hole-Arranged Boron-Doped Diamond AnodeDaibing Luo0Yong Luo1Daichuan Ma2Analytical & Testing Center, Sichuan University, No. 29, Wangjiang Road, Wuhou District, Chengdu 610064, ChinaAnalytical & Testing Center, Sichuan University, No. 29, Wangjiang Road, Wuhou District, Chengdu 610064, ChinaAnalytical & Testing Center, Sichuan University, No. 29, Wangjiang Road, Wuhou District, Chengdu 610064, ChinaAn electrochemical system using a rotating hole-arranged boron-doped diamond (HABDD) film anode was designed for wastewater degradation. Meanwhile, in a reciprocal process, a foam nickel (FNi) cathode was employed for hydrogen evolution using the ions liberated from the HABDD. The HABDD was custom-made using an MWCVD device and characterized by SEM, Raman and electrochemical measurement. Some wastewater was tested on the HABDD anode to examine its electrochemical performance. The efficiency of the electrochemical system was evaluated by COD removal rate and hydrogen production yields. The influence of the rotating and flowing rates of the electrolyte on electrochemical performance was discussed. The rotating HABDD with dynamic three-dimensional flowing paths provided a high mass transfer, which promoted the overall performance of the wastewater mineralization. Meanwhile, the ions released from the anode to the cathode improved the hydrogen generation performance on the cathode. The hydrogen production efficiency in relation to the electrochemical oxidation process was studied in terms of the COD change and treatment time.https://www.mdpi.com/2076-3417/14/23/11284hole-arrayed boron-doped diamondwastewater degradationhydrogen production
spellingShingle Daibing Luo
Yong Luo
Daichuan Ma
Hydrogen Production from Wastewater Degradation on a Rotating Hole-Arranged Boron-Doped Diamond Anode
Applied Sciences
hole-arrayed boron-doped diamond
wastewater degradation
hydrogen production
title Hydrogen Production from Wastewater Degradation on a Rotating Hole-Arranged Boron-Doped Diamond Anode
title_full Hydrogen Production from Wastewater Degradation on a Rotating Hole-Arranged Boron-Doped Diamond Anode
title_fullStr Hydrogen Production from Wastewater Degradation on a Rotating Hole-Arranged Boron-Doped Diamond Anode
title_full_unstemmed Hydrogen Production from Wastewater Degradation on a Rotating Hole-Arranged Boron-Doped Diamond Anode
title_short Hydrogen Production from Wastewater Degradation on a Rotating Hole-Arranged Boron-Doped Diamond Anode
title_sort hydrogen production from wastewater degradation on a rotating hole arranged boron doped diamond anode
topic hole-arrayed boron-doped diamond
wastewater degradation
hydrogen production
url https://www.mdpi.com/2076-3417/14/23/11284
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AT yongluo hydrogenproductionfromwastewaterdegradationonarotatingholearrangedborondopeddiamondanode
AT daichuanma hydrogenproductionfromwastewaterdegradationonarotatingholearrangedborondopeddiamondanode