Synthesis and evaluation of some amine compounds having surface active properties as H2S scavenger

In this work three H2S scavengers were prepared by reacting monoethanolamine with formaldehyde in different ratios (1:1, 2:1 and 2:3) to give MF1, MF2 and MF3, respectively. The chemical structures of the prepared scavengers were confirmed by FT-IR spectroscopy. The effect of reaction time (the time...

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Main Authors: Nadia G. Kandile, Taha M.A. Razek, Ahmed M. Al-Sabagh, Maamoun M.T. Khattab
Format: Article
Language:English
Published: Egyptian Petroleum Research Institute 2014-09-01
Series:Egyptian Journal of Petroleum
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Online Access:http://www.sciencedirect.com/science/article/pii/S1110062114000579
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author Nadia G. Kandile
Taha M.A. Razek
Ahmed M. Al-Sabagh
Maamoun M.T. Khattab
author_facet Nadia G. Kandile
Taha M.A. Razek
Ahmed M. Al-Sabagh
Maamoun M.T. Khattab
author_sort Nadia G. Kandile
collection DOAJ
description In this work three H2S scavengers were prepared by reacting monoethanolamine with formaldehyde in different ratios (1:1, 2:1 and 2:3) to give MF1, MF2 and MF3, respectively. The chemical structures of the prepared scavengers were confirmed by FT-IR spectroscopy. The effect of reaction time (the time required for completing the reaction between the scavenger and the H2S gas) has been studied for the three prepared scavengers. The effects of concentration and temperature have been studied on the scavenging efficiency of H2S using three prepared products and two commercial products EPRI-710 and EPRI-730. The surface and thermodynamic parameters of the prepared scavengers were determined at 25 °C including, surface tension (γ), and effectiveness, maximum surface excess (Γmax) and minimum surface area (Amin). Also, the standard free energy of micellization and adsorption was recorded. The results show that the efficiency of scavengers increased with increasing reaction time up to 50 min. Also, as concentration of scavengers and temperature increased, the removal efficiency of the scavengers increased. By comparing the efficiency of the prepared products with the commercial products EPRI-710 and EPRI 730, it was found that, MF3 exhibited a similar efficiency comparing with the commercial scavenger EPRI 730 (currently used in the field) at different concentrations and temperatures.
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spelling doaj-art-db04235e2dc94e48a7f40584faca8e2e2025-08-20T02:03:42ZengEgyptian Petroleum Research InstituteEgyptian Journal of Petroleum1110-06212014-09-0123332332910.1016/j.ejpe.2014.08.008Synthesis and evaluation of some amine compounds having surface active properties as H2S scavengerNadia G. Kandile0Taha M.A. Razek1Ahmed M. Al-Sabagh2Maamoun M.T. Khattab3Faculty of Women, Ain Shams, EgyptInstitute of Environmental Studies and Research, Ain Shams University, EgyptEgyptian Petroleum Research Institute, Nasr City 11727, Cairo, EgyptQarun Petroleum Company, EgyptIn this work three H2S scavengers were prepared by reacting monoethanolamine with formaldehyde in different ratios (1:1, 2:1 and 2:3) to give MF1, MF2 and MF3, respectively. The chemical structures of the prepared scavengers were confirmed by FT-IR spectroscopy. The effect of reaction time (the time required for completing the reaction between the scavenger and the H2S gas) has been studied for the three prepared scavengers. The effects of concentration and temperature have been studied on the scavenging efficiency of H2S using three prepared products and two commercial products EPRI-710 and EPRI-730. The surface and thermodynamic parameters of the prepared scavengers were determined at 25 °C including, surface tension (γ), and effectiveness, maximum surface excess (Γmax) and minimum surface area (Amin). Also, the standard free energy of micellization and adsorption was recorded. The results show that the efficiency of scavengers increased with increasing reaction time up to 50 min. Also, as concentration of scavengers and temperature increased, the removal efficiency of the scavengers increased. By comparing the efficiency of the prepared products with the commercial products EPRI-710 and EPRI 730, it was found that, MF3 exhibited a similar efficiency comparing with the commercial scavenger EPRI 730 (currently used in the field) at different concentrations and temperatures.http://www.sciencedirect.com/science/article/pii/S1110062114000579Hydrogen sulfide scavengerMicellizationThermodynamic parametersMinimum surface area
spellingShingle Nadia G. Kandile
Taha M.A. Razek
Ahmed M. Al-Sabagh
Maamoun M.T. Khattab
Synthesis and evaluation of some amine compounds having surface active properties as H2S scavenger
Egyptian Journal of Petroleum
Hydrogen sulfide scavenger
Micellization
Thermodynamic parameters
Minimum surface area
title Synthesis and evaluation of some amine compounds having surface active properties as H2S scavenger
title_full Synthesis and evaluation of some amine compounds having surface active properties as H2S scavenger
title_fullStr Synthesis and evaluation of some amine compounds having surface active properties as H2S scavenger
title_full_unstemmed Synthesis and evaluation of some amine compounds having surface active properties as H2S scavenger
title_short Synthesis and evaluation of some amine compounds having surface active properties as H2S scavenger
title_sort synthesis and evaluation of some amine compounds having surface active properties as h2s scavenger
topic Hydrogen sulfide scavenger
Micellization
Thermodynamic parameters
Minimum surface area
url http://www.sciencedirect.com/science/article/pii/S1110062114000579
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AT tahamarazek synthesisandevaluationofsomeaminecompoundshavingsurfaceactivepropertiesash2sscavenger
AT ahmedmalsabagh synthesisandevaluationofsomeaminecompoundshavingsurfaceactivepropertiesash2sscavenger
AT maamounmtkhattab synthesisandevaluationofsomeaminecompoundshavingsurfaceactivepropertiesash2sscavenger