Strain-induced superconductivity in RuO2(100) thin-films

Abstract Recently, superconductivity was discovered with a superconducting transition temperature (T c ) of 2 K in strained (110)-oriented RuO2 films grown on TiO2(110) single-crystal substrates. In this work, we predict and realize superconductivity in strained (100)-oriented RuO2 thin films grown...

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Bibliographic Details
Main Authors: Neha Wadehra, Benjamin Z. Gregory, Shuyuan Zhang, Noah Schnitzer, Yusuke Iguchi, Yilin Evan Li, Betül Pamuk, David A. Muller, Andrej Singer, Kyle M. Shen, Darrell G. Schlom
Format: Article
Language:English
Published: Nature Portfolio 2025-07-01
Series:Communications Materials
Online Access:https://doi.org/10.1038/s43246-025-00856-6
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Summary:Abstract Recently, superconductivity was discovered with a superconducting transition temperature (T c ) of 2 K in strained (110)-oriented RuO2 films grown on TiO2(110) single-crystal substrates. In this work, we predict and realize superconductivity in strained (100)-oriented RuO2 thin films grown on TiO2(100) single-crystal substrates. We show that while density functional theory predicts the T c of strained RuO2(100) films to be even higher than the RuO2(110) films, our transport and angle-resolved photoemission spectroscopy measurements find the T c to be about 1 K in strained RuO2(100) films grown on TiO2(100) substrates. Nonetheless, the thickness dependence of the T c follows a similar trend in both cases. Our scanning SQUID measurements reveal a local superfluid response, indicating a 100 mK inhomogeneity in T c over a 100 μm scale.
ISSN:2662-4443